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The ability in experiments to control the relative twist angle between successive layers in two-dimensional (2D) materials offers a new approach to manipulating their electronic properties; we refer to this approach as "twistronics". A…

Mesoscale and Nanoscale Physics · Physics 2017-02-22 Stephen Carr , Daniel Massatt , Shiang Fang , Paul Cazeaux , Mitchell Luskin , Efthimios Kaxiras

We derive electronic tight-binding Hamiltonians for strained graphene, hexagonal boron nitride and transition metal dichalcogenides based on Wannier transformation of {\it ab initio} density functional theory calculations. Our microscopic…

Mesoscale and Nanoscale Physics · Physics 2018-08-14 Shiang Fang , Stephen Carr , Miguel A. Cazalilla , Efthimios Kaxiras

When twisted to angles near 1{\deg}, graphene multilayers provide a new window on electron correlation physics by hosting gate-tuneable strongly-correlated states, including insulators, superconductors, and unusual magnets. Here we report…

We present a multi-scale density functional theory (DFT) informed molecular dynamics and tight-binding (TB) approach to capture the interdependent atomic and electronic structures of twisted bilayer graphene. We calibrate the flat band…

Mesoscale and Nanoscale Physics · Physics 2022-03-17 Nicolas Leconte , Srivani Javvaji , Jiaqi An , Appalakondaiah Samudrala , Jeil Jung

We study the electronic properties of twisted bilayers graphene in the tight-binding approximation. The interlayer hopping amplitude is modeled by a function, which depends not only on the distance between two carbon atoms, but also on the…

Mesoscale and Nanoscale Physics · Physics 2015-08-12 A. O. Sboychakov , A. L. Rakhmanov , A. V. Rozhkov , Franco Nori

Moir\'e superlattices in two-dimensional (2D) materials exhibit rich quantum phenomena, but ab initio modelling of these systems remains computationally prohibitive. Existing machine learning methods for accelerating density-functional…

Materials Science · Physics 2026-02-11 Zekun Lou , Alan M. Lewis , Mariana Rossi

In this article, we analyse the Bistritzer--MacDonald (BM) model (also known as the continuum model) of twisted bilayer graphene (TBG) with an additional external magnetic field. We provide an explicit semiclassical asymptotic expansion of…

Mathematical Physics · Physics 2024-01-05 Simon Becker , Jihoi Kim , Xiaowen Zhu

By virtue of being atomically thin, the electronic properties of heterostructures built from two-dimensional materials are strongly influenced by atomic relaxation. The atomic layers behave as flexible membranes rather than rigid crystals.…

Strongly Correlated Electrons · Physics 2025-01-07 Mohammed M. Al Ezzi , Gayani N. Pallewela , Christophe De Beule , E. J. Mele , Shaffique Adam

We derive a material-realistic real-space many-body Hamiltonian for twisted bilayer graphene from first principles, including both single-particle hopping terms for $p_z$ electrons and long-range Coulomb interactions. By disentangling low-…

Mesoscale and Nanoscale Physics · Physics 2022-01-24 Tom Westerhout , Mikhail I. Katsnelson , Malte Rösner

A detailed understanding of interacting electrons in twisted bilayer graphene (tBLG) near the magic angle is required to gain insights into the physical origin of the observed broken symmetry phases. Here, we present extensive atomistic…

Mesoscale and Nanoscale Physics · Physics 2020-07-02 Zachary A. H. Goodwin , Valerio Vitale , Xia Liang , Arash A. Mostofi , Johannes Lischner

We extend the low-energy effective two-band Hamiltonian for electrons in bilayer graphene (E. McCann, V. I. Fal'ko, Phys. Rev. Lett. 96 (2006) 86805) to include a spatially dependent electrostatic potential. We find that this Hamiltonian…

Mesoscale and Nanoscale Physics · Physics 2010-01-12 C. J. Poole

Staking layered materials revealed to be a very powerful method to tailor their electronic properties. It has indeed been theoretically and experimentally shown that twisted bilayers of graphene (tBLG) with a rotation angle $\theta$,…

Mesoscale and Nanoscale Physics · Physics 2020-07-01 Omid Faizy Namarvar , Ahmed Missaoui , Laurence Magaud , Didier Mayou , Guy Trambly de Laissardière

We consider the problem of numerically computing the quantum dynamics of an electron in twisted bilayer graphene. The challenge is that atomic-scale models of the dynamics are aperiodic for generic twist angles because of the…

Mathematical Physics · Physics 2024-02-27 Tianyu Kong , Diyi Liu , Mitchell Luskin , Alexander B. Watson

Twisted bilayer graphene exhibits isolated, relatively flat electronic bands near charge neutrality when the interlayer rotation is tuned to specific magic angles. These small misalignments, typically below 1.1{\deg}, result in long-period…

Mesoscale and Nanoscale Physics · Physics 2026-03-26 Antonio Palamara , Michele Pisarra , Antonello Sindona

In this paper, the electronic properties of 30{\deg} twisted double bilayer graphene, which loses the translational symmetry due to the incommensurate twist angle, are studied by means of the tight-binding approximation. We demonstrate the…

Materials Science · Physics 2020-09-14 Guodong Yu , Zewen Wu , Zhen Zhan , Mikhail I. Katsnelson , Shengjun Yuan

Understanding the dynamics of excitons in two dimensional semiconductors requires a theory that incorporates the essential physics distinct from their three-dimensional counterparts. In addition to the modified dielectric environment,…

Mesoscale and Nanoscale Physics · Physics 2019-01-30 Pengke Li , Ian Appelbaum

Motivated by the recent observation of correlated insulator states and unconventional superconductivity in twisted bilayer graphene, we study the dependence of electron correlations on the twist angle and reveal the existence of strong…

Strongly Correlated Electrons · Physics 2019-09-18 Zachary A. H. Goodwin , Fabiano Corsetti , Arash A. Mostofi , Johannes Lischner

We present efficient angle-dependent low-energy Hamiltonians to describe the properties of the twisted bilayer graphene (tBLG) heterostructure, based on {\it ab initio} calculations of mechanical relxation and electronic structure. The…

Mesoscale and Nanoscale Physics · Physics 2019-08-02 Shiang Fang , Stephen Carr , Ziyan Zhu , Daniel Massatt , Efthimios Kaxiras

We provide a formal derivation of a reduced model for twisted bilayer graphene (TBG) from Density Functional Theory. Our derivation is based on a variational approximation of the TBG Kohn-Sham Hamiltonian and asymptotic limit techniques. In…

Mesoscale and Nanoscale Physics · Physics 2023-04-14 Eric Cancès , Louis Garrigue , David Gontier

The recently realized bilayer graphene system with a twist angle of $30^\circ$ offers a new type of quasicrystal which unites the dodecagonal quasicrystalline nature and graphene's relativistic properties. Here, we introduce a concise…

Mesoscale and Nanoscale Physics · Physics 2019-05-10 Pilkyung Moon , Mikito Koshino , Young-Woo Son
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