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Theoretical framework for the isosteric heat of adsorption is developed treating the effects of the non-ideal gas behavior and the adsorbed phase volume. Rigorous thermodynamic treatment for the adsorbed phase volume is presented for…
Doppler broadening presents a major limitation for high-resolution spectroscopy and nonlinear optics in room-temperature atomic vapors. Here, we demonstrate the suppression of Doppler broadening accompanied by pronounced absorption on the…
The interaction of light with optical and mechanical systems is influenced by material properties, geometrical configurations, and surface topographies. Designing these systems necessitates a careful balance of conflicting requirements,…
For window applications in hot climates, it is desirable to have windows with high visible transparency, while maintaining strong reflectance in both the ultraviolet and near infrared, to minimize unwanted heat gain. Given that more than…
The effects of random distribution of magnetic impurities with concentration $x$ in a semiconductor alloy multilayer at a paramagnetic temperature are investigated by means of coherent potential approximation and tight-binding model. The…
Concentrating solar power, particularly parabolic trough system with solar concentrations less than 50, requires spectrally selective solar absorbers that are thermally stable at high temperatures of 400degC above to achieve high…
The disjoining pressure isotherm in foam films is theoretically studied and an important contribution of adsorption is discovered. On the basis of the interfacial thermodynamics an adsorption disjoining pressure component is derived, which…
For the development of nanoscale electronics and photonics using atomically thin two-dimensional (2D) materials, it is important to realize van der Waals (vdW) interfaces with low thermal resistance, to minimize performance reduction caused…
Vapor deposition on polycrystalline films can lead to staggering levels of compressive stress, exceeding even the yield strength of the films. Mysteriously, a significant part of this stress has a reversible nature: it disappears when the…
The ability to efficiently absorb thermal radiation within a small material volume is crucial for the realization of compact and high spatial resolution thermal imagers. Here we propose and experimentally demonstrate a compact plasmonic…
In recent years there has been great interest towards optical cavities as a tool to manipulate the properties and phases of embedded quantum materials. Due to the Purcell effect, a cavity changes the photon phase space and thus the rate of…
Controlling thermal expansion is an important, not yet resolved, and challenging problem in materials research. A conceptual design is introduced here for the first time, for the use of MOFs as platforms for controlling thermal expansion…
Panchromatic absorbing materials are widely regarded as a key strategy for enhancing solar energy utilization and photocurrent generation. However, in artificial molecular systems, broadening the absorption spectrum is often accompanied by…
In this paper, we report on the optical absorption in porous silicon. We model the absorption process assuming that porous silicon is a pseudo 1D material system having a distribution of band gaps. We show that in order to explain the…
The effects of chemical disorder on the electronic and optical properties of semiconductor alloy multilayers are studied based on the tight-binding theory and single-site coherent potential approximation. Due to the quantum confinement of…
We analyze the rate of two-photon absorption in tapered optical fibers with diameters less than the wavelength of the incident light. The rate of two-photon absorption is shown to be enhanced due to the small mode volume of the tapered…
A 20-fold increase over the single path optical absorption is demonstrated with a low loss medium placed in a resonant cavity. This has been applied to laser cooling of Yb:ZBLAN glass resulting in 90% absorption of the incident pump light.…
We study the atomic oxygen adsorption on Pb(111) surface by using density-functional theory within the generalized gradient approximation and a supercell approach. The atomic and energetic properties of purely on-surface and subsurface…
We investigate adsorption of a gas on the flat surface of a solid deformable adsorbent taking into account thermal fluctuations and analyze in detail the effect of thermal fluctuations on the adsorbent deformation in adsorption. The…
Future laser-interferometric gravitational wave detectors (GWDs) will potentially employ test mass mirrors from crystalline silicon and a laser wavelength of $1550\,\rm{nm}$, which corresponds to a photon energy below the silicon bandgap.…