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The conformational and dynamical properties of active polymers in solution are determined by the nature of the activity, and the behavior of polymers with self-propelled, active Brownian particle-type monomers differs qualitatively from…

Soft Condensed Matter · Physics 2020-05-27 Aitor Martin-Gomez , Thomas Eisenstecken , Gerhard Gompper , Roland G. Winkler

Polymers exposed to shear flow exhibit a rich tumbling dynamics. While rigid rods rotate on Jeffery orbits, flexible polymers stretch and coil up during tumbling. Theoretical results show that in both of these asymptotic regimes the…

Soft Condensed Matter · Physics 2014-05-27 Philipp S. Lang , Benedikt Obermayer , Erwin Frey

By means of Brownian dynamics simulations we study the steady-state dynamic properties of a flexible active polymer in a poor solvent condition. Our results show that the effective diffusion constant of the polymer $D_{\rm eff}$ gets…

Soft Condensed Matter · Physics 2023-08-29 Suman Majumder , Subhajit Paul , Wolfhard Janke

We study the linear response of interacting active Brownian particles in an external potential to simple shear flow. Using a path integral approach, we derive the linear response of any state observable to initiating shear in terms of…

Statistical Mechanics · Physics 2019-04-12 Kiryl Asheichyk , Alexandre P. Solon , Christian M. Rohwer , Matthias Krüger

Self-consistent field approach is used to model a single end-tethered polymer chain on a substrate subject to various forces in three dimensions. Starting from a continuous Gaussian chain model, the following perturbations are considered:…

Periodic boundary conditions for planar mixed flows are implemented in the context of a multi-chain Brownian dynamics simulation algorithm. The effect of shear rate $\dot{\gamma}$, and extension rate $\dot{\epsilon}$, on the size of polymer…

Soft Condensed Matter · Physics 2020-07-03 Aashish Jain , Chandi Sasmal , Remco Hartkamp , B. D. Todd , J. Ravi Prakash

Nonequilibrium molecular dynamics simulations are used to study the shear thinning behavior of immiscible symmetric polymer blends. The phase separated polymers are subjected to a simple shear flow imposed by moving a wall parallel to the…

Soft Condensed Matter · Physics 2009-11-07 Sandra Barsky , Mark O. Robbins

Using molecular dynamics simulations we examine the dynamics of a family of model polymers with varying chain length and torsional potential barriers. We focus on features of the dynamics of polymers that are seen experimentally but absent…

Soft Condensed Matter · Physics 2019-06-11 Daniel Fragiadakis , C. Michael Roland

Nonlinear behavior of electro-osmosis in dilute non-adsorbing polymer solutions with low salinity is investigated with Brownian dynamics simulations and a kinetic theory. In the Brownian simulations, the hydrodynamic interaction between the…

Soft Condensed Matter · Physics 2015-06-19 Yuki Uematsu

We study how an active bath is transduced into the internal fluctuation spectrum of a semiflexible polymer. Starting from the statistics of active forces exerted by an explicit bath of active Brownian particles, we derive an effective…

Soft Condensed Matter · Physics 2026-04-14 Love Grover , Anil Kumar Dasanna , Abhishek Chaudhuri

We study the dynamics of an active Brownian particle with a nonlinear friction function located in a spatial cubic potential. For strong but finite damping, the escape rate of the particle over the spatial potential barrier shows a…

Statistical Mechanics · Physics 2012-04-02 P. S. Burada , B. Lindner

We develop a strong stretching approximation for a polymer brush made of self-avoiding polymer chains. The density profile of the brush and the distribution of the end monomer positions in stretching direction are computed and compared with…

Soft Condensed Matter · Physics 2021-05-26 Dirk Romeis , Michael Lang

The mechanical non-linear response of dense Brownian suspensions of polymer gel particles is studied experimentally and by means of numerical simulations. It is shown that the response to the application of a constant shear rate depends on…

Soft Condensed Matter · Physics 2022-10-05 Dmytro Kushnir , Céline Ruscher , Eckhard Bartsch , Fabrice Thalmann , Pascal Hébraud

The effect of fluctuating internal viscosity and hydrodynamic interactions on a range of rheological properties of dilute polymer solutions is examined using a finitely extensible dumbbell model for a polymer. Brownian dynamics simulations…

Soft Condensed Matter · Physics 2020-07-03 R. Kailasham , Rajarshi Chakrabarti , J. Ravi Prakash

We study the swelling of a flexible linear chain composed of active particles by analytical theory and computer simulation. Three different situations are considered: a free chain, a chain confined to an external harmonic trap, and a chain…

Soft Condensed Matter · Physics 2015-03-31 Andreas Kaiser , Sonja Babel , Borge ten Hagen , Christian von Ferber , Hartmut Löwen

An exact solution of coarse-grained polymer models with fluctuating internal friction and hydrodynamic interactions has not been proposed so far due to a one-to-all coupling between the connector vector velocities that precludes the…

Soft Condensed Matter · Physics 2024-06-19 R. Kailasham , Rajarshi Chakrabarti , J. Ravi Prakash

We study the dynamics of the phase behavior of a polymer blend in the presence of shear flow. By adopting a two fluid picture and using a generalization of the concept of material derivative, we construct kinetic equations that describe the…

Soft Condensed Matter · Physics 2009-10-30 Tao Sun , Anna C. Balazs , David Jasnow

The non-linear response of entangled polymers to shear flow is complicated. Its current understanding is framed mainly as a rheological description in terms of the complex viscosity. However, the full picture requires an assessment of the…

Computational Physics · Physics 2018-08-21 Airidas Korolkovas , Philipp Gutfreund , Max Wolff

We study the dynamics and conformation of polymers composed by active monomers. By means of Brownian dynamics simulations we show that when the direction of the self-propulsion of each monomer is aligned with the backbone, the polymer…

Soft Condensed Matter · Physics 2018-11-28 Valentino Bianco , Emanuele Locatelli , Paolo Malgaretti

Structure and dynamics of an active polymer on a smooth cylindrical surface are studied by Brownian dynamics simulations. The effect of active force on the polymer adsorption behavior and the combined effect of chain mobility, length N,…

Soft Condensed Matter · Physics 2024-08-21 Chen Shen , Chao-ran Qin , Tian-liang Xu , Kang Chen , Wen-de Tian