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We propose a continuous variable quantum state tomography protocol of electrons which result from the ionization of atoms or molecules by the absorption of extreme ultraviolet light pulses. Our protocol is benchmarked against a direct…

We theoretically propose a multidimensional high-harmonic echo spectroscopy technique which utilizes strong optical fields to resolve coherent electron dynamics spanning an energy range of multiple electron Volts. Using our recently…

Quantum coherence between electronic states of a photoionized molecule and the resulting process of ultrafast electron-hole migration have been put forward as a possible quantum mechanism of charge-directed reactivity governing the…

Entangled states of two coupled polar molecules controlled by laser pulses are studied theoretically. Schmidt decomposition is used to measure the degree of entanglement. By varying the pulse shape of the applied laser, transition from…

Atomic and Molecular Clusters · Physics 2007-05-23 Y. Y. Liao , Y. N. Chen , D. S. Chuu

Entangled coherent states play pivotal roles in various fields such as quantum computation, quantum communication, and quantum sensing. We experimentally demonstrate the generation of entangled coherent states with the two-dimensional…

Quantum Physics · Physics 2024-03-26 Honggi Jeon , Jiyong Kang , Jaeun Kim , Wonhyeong Choi , Kyunghye Kim , Taehyun Kim

We introduce and experimentally demonstrate a method, where the two intrinsic time scales of a molecule, the slow nuclear motion and the fast electronic motion, are simultaneously measured in a photo-electron photo-ion coincidence…

We produce oriented rotational wave packets in CO and measure their characteristics via high harmonic generation. The wavepacket is created using an intense, femtosecond laser pulse and its second harmonic. A delayed 800 nm pulse probes the…

The narrowing of electron and ion wave packets in the process of photoionization is investigated, with the electron-ion recoil fully taken into account. Packet localization of this type is directly related to entanglement in the joint…

Quantum Physics · Physics 2009-11-10 M. V. Fedorov , M. A. Efremov , A. E. Kazakov , K. W. Chan , C. K. Law , J. H. Eberly

We study formation and evolution of the electron wave-packets in the process of strong field ionization of various atomic targets. Our study is based on reformulating the problem in terms of conditional amplitudes, i.e., the amplitudes…

Atomic Physics · Physics 2023-10-18 I. A. Ivanov , A. S. Kheifets , Kyung Taec Kim

Precise quantum control and measurement of several harmonic oscillators, such as the modes of the electromagnetic field in a cavity or of mechanical motion, are key for their use as quantum platforms. The motional modes of trapped ions can…

We consider a model Hamiltonian describing the interaction of a single-mode radiation field with the atoms of a nonlinear medium, and study the dynamics of entanglement for specific non-entangled initial states of interest: namely, those in…

Quantum Physics · Physics 2007-07-01 C. Sudheesh , S. Lakshmibala , V. Balakrishnan

Light-induced molecular dynamics often involve the excitation of several electronic, vibrational, and rotational states. Since the ensuing electronic and nuclear motion determines the pathways and outcomes of photoinduced reactions, our…

Entanglement is one of the most intriguing aspects of quantum mechanics and lies at the heart of the ongoing Second Quantum Revolution, where it is a resource that is used in quantum key distribution, quantum computing and quantum…

Quantum Physics · Physics 2022-02-02 Lisa-Marie Koll , Laura Maikowski , Lorenz Drescher , Tobias Witting , Marc J. J. Vrakking

Projective measurements are a powerful tool for manipulating quantum states. In particular, a set of qubits can be entangled by measurement of a joint property such as qubit parity. These joint measurements do not require a direct…

We consider the use of a traveling wave probe to continuously measure the quantum state of an atom in free space. Unlike the more familiar cavity QED geometry, the traveling wave is intrinsically a multimode problem. Using an appropriate…

Quantum Physics · Physics 2009-11-07 Andrew Silberfarb , Ivan H. Deutsch

The detection of electron motion and electronic wavepacket dynamics is one of the core goals of attosecond science. Recently, choosing the nitric oxide (NO) molecule as an example, we have introduced and demonstrated a new experimental…

Atomic and Molecular Clusters · Physics 2015-04-17 Song Bin Zhang , Denitsa Baykusheva , Peter M. Kraus , Hans Jakob Wörner , Nina Rohringer

Recent technological advances allowed the coherent optical manipulation of high-energy electron wavepackets with attosecond precision. Here we theoretically investigate the collision of optically-modulated pulsed electron beams with atomic…

Atomic Physics · Physics 2021-04-21 Yuya Morimoto , Peter Hommelhoff , Lars Bojer Madsen

The magnetic focusing of electrons has proven its utility in fundamental studies of electron transport. Here we report the direct imaging of magnetic focusing of electron waves, specifically in a two-dimensional electron gas (2DEG). We see…

Mesoscale and Nanoscale Physics · Physics 2007-08-08 K. E. Aidala , R. E. Parrott , T. Kramer , E. J. Heller , R. M. Westervelt , M. P. Hanson , A. C. Gossard

We discuss techniques that allow for long coherence times in laser spectroscopy experiments with two trapped ions. We show that for this purpose not only entangled ions prepared in decoherence-free subspaces can be used but also a pair of…

Quantum Physics · Physics 2011-11-10 M. Chwalla , K. Kim , T. Monz , P. schindler , M. Riebe , C. F. Roos , R. Blatt

We describe a proof-of-principal experiment demonstrating a Fourier technique for measuring the shape of biphoton wavepackets. The technique is based on the use of synchronously driven fast modulators and slow (integrating) detectors.

Quantum Physics · Physics 2015-05-13 Chinmay Belthangady , Shengwang Du , Chih-Sung Chuu , G. Y. Yin , S. E. Harris