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A thermodynamic argument has been developed which relates the chirality of the constituents of a mixture of enantiomers to the system excess volume, and thereby to its Gibbs free enthalpy. A specific connection is shown between the excess…

Statistical Mechanics · Physics 2007-05-23 J. F. Kenney , Ulrich K. Deiters

The homochirality of biomolecules remains one of the outstanding puzzles concerning the beginning of life. Chiral amplification of a randomly perturbed racemic mixture of chiral molecules is a well-accepted prerequisite for all routes to…

Chemical Physics · Physics 2022-10-12 Uri Hananel , Assaf Ben-Moshe , Haim Diamant , Gil Markovich

The stability and conservation properties of a recently proposed polymerization model are studied. The achiral (racemic) solution is linearly unstable once the relevant control parameter (here the fidelity of the catalyst) exceeds a…

Biomolecules · Quantitative Biology 2007-05-23 A. Brandenburg , A. C. Andersen , S. Höfner , M. Nilsson

Understanding the condensed-phase behavior of chiral molecules is important in biology, as well as in a range of technological applications, such as the manufacture of pharmaceuticals. Here, we use molecular dynamics simulations to study a…

Statistical Mechanics · Physics 2023-12-27 Pablo M. Piaggi , Roberto Car , Frank H. Stillinger , Pablo G. Debenedetti

A Monte Carlo study of the late time growth of $L1_2$ ordered domains on a fcc $A_3B$ binary alloy is presented. The energy of the alloy has been modeled by a nearest neighbor interaction Ising hamiltonian. The system exhibits a fourfold…

Condensed Matter · Physics 2009-10-28 Carlos Frontera , Eduard Vives , Teresa Castán , Antoni Planes

We present a differential rate equation model of chiral polymerization based on a simple copolymerization scheme in which the enantiomers are added to, or removed from, the homochiral or heterochiral chains (reversible stepwise isodesmic…

Quantitative Methods · Quantitative Biology 2017-08-23 Celia Blanco , David Hochberg

Diffusion effect on chirality selection in a two-dimensional reaction-diffusion model is studied by the Monte Carlo simulation. The model consists of achiral reactants A which turn into either of the chiral products, R or S, in a solvent of…

Statistical Mechanics · Physics 2007-07-20 Ryo Shibata , Yukio Saito , Hiroyuki Hyuga

We introduce and numerically solve a mathematical model of the experimentally established mechanisms responsible for the symmetry breaking transition observed in the chiral crystallization experiments reported by I. Weissbuch, L. Addadi, L.…

Biomolecules · Quantitative Biology 2017-09-13 Celia Blanco , David Hochberg

Detection of chiral molecules requires amplification of chirality to measurable levels. Typically, amplification mechanisms are considered at the microscopic scales of individual molecules and their aggregates. Here we demonstrate chirality…

Soft Condensed Matter · Physics 2015-07-28 Chenhui Peng , Oleg D. Lavrentovich

We present a fast Monte-Carlo algorithm for simulating epitaxial surface growth, based on the continuous-time Monte-Carlo algorithm of Bortz, Kalos and Lebowitz. When simulating realistic growth regimes, much computational time is consumed…

Materials Science · Physics 2009-11-11 J. P. DeVita , L. M. Sander , P. Smereka

The real-time dynamics of chiral phase transition is investigated in a two-flavor ($N_f=2$) soft-wall AdS/QCD model. To understand the dynamics of thermalization, we quench the system from initial states deviating from the equilibrium…

High Energy Physics - Phenomenology · Physics 2023-04-19 Xuanmin Cao , Jingyi Chao , Hui Liu , Danning Li

Starting from the chemical master equation, we employ field theoretic techniques to derive Langevin-type equations that exactly describe the stochastic dynamics of the Frank chiral amplification model with spatial diffusion. The intrinsic…

Populations and Evolution · Quantitative Biology 2007-05-23 David Hochberg , Maria-Paz Zorzano

Liquid crystal mesophases of achiral molecules are normally achiral, yet in a few materials they spontaneously segregate and form right- and left-handed chiral domains. One mechanism that drives chiral segregation is molecular shape…

Soft Condensed Matter · Physics 2026-01-16 Matthew J. Deutsch , Robin L. B. Selinger , Paul van der Schoot

In this work we report on kinetic Monte-Carlo calculations of resistive switching and the underlying growth dynamics of filaments in an electrochemical metallization device consisting of an Ag/TiO2/Pt sandwich-like thin film system. The…

Competing phases or interactions in complex many-particle systems can result in free energy barriers that strongly suppress thermal equilibration. Here we discuss how extended ensemble Monte Carlo simulations can be used to study the…

Statistical Mechanics · Physics 2007-05-23 S. Trebst , D. A. Huse , E. Gull , H. G. Katzgraber , U. H. E. Hansmann , M. Troyer

Local scale invariance (LSI) has been recently proposed as a possible extension of the dynamical scaling in systems at the critical point and during phase ordering. LSI has been applied inter alia to provide predictions for the scaling…

Statistical Mechanics · Physics 2009-11-11 Michel Pleimling , Andrea Gambassi

We study the QCD phase diagram in the strong coupling limit with fluctuation effects by using the auxiliary field Monte-Carlo method. We apply the chiral angle fixing technique in order to obtain finite chiral condensate in the chiral limit…

High Energy Physics - Lattice · Physics 2016-01-26 Terukazu Ichihara , Akira Ohnishi , Takashi Z. Nakano

We develop a coarse grained (CG) approach for efficiently simulating calcium dynamics in the endoplasmic reticulum membrane based on a fine stochastic lattice gas model. By grouping neighboring microscopic sites together into CG cells and…

Chemical Physics · Physics 2015-06-15 Chuansheng Shen , Hanshuang Chen

Recently the first chemical systems which show the amplification of enantiometric excess (ee) was found. Inspired by these experiments, we propose a few chemical reaction models in a closed system. The reactions consist of autocatalytic…

Biological Physics · Physics 2007-05-23 Yukio Saito , Hiroyuki Hyuga

Mandelic acid is an enantiomer of interest in many areas, in particular for the pharmaceutical industry. One of the approaches to produce enantiopure mandelic acid is through crystallization from an aqueous solution. We propose in this…

Fluid Dynamics · Physics 2023-03-22 Q. Tan , S. A. Hosseini , A. Seidel-Morgenstern , D. Thevenin , H. Lorenz
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