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Double perovskites containing heavy transition metal ions are an important family of compounds for the study of the interplay between electron correlation and spin-orbit coupling. Here, by combining magnetic susceptibility, heat capacity,…

The coupling between antiferromagnetic spins and infrared-active phonons in solids is responsible for many intriguing phenomena and is a field of intense research with extensive potential applications in the modern devices based on…

Microscopic coupling between the electron spin and the lattice vibration is responsible for an array of exotic properties from morphic effects in simple magnets to magnetodielectric coupling in multiferroic spinels and hematites.…

Materials Science · Physics 2022-07-22 Mingqiang Gu , Y. H. Bai , G. P. Zhang , Thomas F. George

Temperature dependent Raman scattering measurements have been performed to explore unusual coupling between magnetism and crystal structure in doped pyrochlore iridate Y$_2$(Ir$_{1-x}$Ru$_x$)$_2$O$_7$ with $x$ = 0.0, 0.05 and 0.2. The…

Strongly Correlated Electrons · Physics 2019-02-20 Harish Kumar , V. G. Sathe , A. K. Pramanik

Raman scattering measurements on BiFeO3 single crystals show an important coupling between the magnetic order and lattice vibrations. The temperature evolution of phonons shows that the lowest energy E and A1 phonon modes are coupled to the…

Strongly Correlated Electrons · Physics 2010-10-12 P. Rovillain , M. Cazayous , Y. Gallais , A. Sacuto , R. P. S. M. Lobo , D. Lebeugle , D. Colson

Temperature and magnetic field studies of the elastic constants of the chromium spinel CdCr_2O_4 show pronounced anomalies related to strong spin-phonon coupling in this frustrated antiferromagnet. A detailed comparison of the longitudinal…

Strongly Correlated Electrons · Physics 2015-05-20 Subhro Bhattacharjee , S. Zherlitsyn , O. Chiatti , A. Sytcheva , J. Wosnitza , R. Moessner , M. E. Zhitomirsky , P. Lemmens , V. Tsurkan , A. Loidl

Nickel orthoborate $Ni_{3}(BO_{3})_{2}$ having a complex orthorhombic structure $P_{nnm}$ (#58, Z=2) of the kotoite type is known for quite a long time as an antiferromagnetic material below $T_{N}$ = 46 K, but up to now its physical…

We present Raman spectroscopy results backed by first-principles calculations and investigate the nature of possible spin-phonon coupling (SPC) in a Gd-doped Y$_2$CoMnO$_6$ (YGCMO) double perovskite oxide. The influence of Gd substitution,…

Materials Science · Physics 2025-08-20 Anasua Khan , Debdatta Banerjee , Divya Rawat , T. K Nath , Ajay Soni , Swastika Chatterjee , A. Taraphder

We have calculated spin relaxation rates in parabolic quantum dots due to the phonon modulation of the spin-orbit interaction in presence of an external magnetic field. Both, deformation potential and piezoelectric electron-phonon coupling…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 A. M. Alcalde , Qu Fanyao , G. E. Marques

We performed a Raman scattering study of thin films of LiTi$_2$O$_4$ spinel oxide superconductor. We detected four out of five Raman active modes, with frequencies in good accordance with our first-principles calculations. Three T$_{2g}$…

Superconductivity · Physics 2017-09-13 D. Chen , Y. -L. Jia , T. -T. Zhang , Z. Fang , K. Jin , P. Richard , H. Ding

Spin-orbit interaction is an important vehicle for spin relaxation. At finite temperature lattice vibrations modulate the spin-orbit interaction and thus generate a mechanism for spin-phonon coupling, which needs to be incorporated in any…

Materials Science · Physics 2018-09-26 Subhayan Roychoudhury , Stefano Sanvito

In ABO3 perovskites, oxygen octahedron rotations are common structural distortions that can promote large ferroelectricity in BiFeO3 with an R3c structure [1], but suppress ferroelectricity in CaTiO3 with a Pbnm symmetry [2]. For many…

Materials Science · Physics 2016-04-05 Hongwei Wang , Jianguo Wen , Dean J. Miller , Qibin Zhou , Mohan Chen , Ho Nyung Lee , Karin M. Rabe , Xifan Wu

Superconducting and normal-state properties of the beta-pyrochlore oxide KOs2O6 are studied by means of thermodynamic and transport measurements. It is shown that the superconductivity is of conventional s-wave type and lies in the…

Superconductivity · Physics 2009-11-13 Z. Hiroi , S. Yonezawa , Y. Nagao , J. Yamaura

The Iridium-based oxides are the subject of great recent interest due to the non-conventional physics that may emerge from the strong spin-orbit coupling present in 5d ions. Here, we explore the coupling between Ir and Co in the…

Materials Science · Physics 2025-11-18 C. A. S. Vieira , B. J. Santos , J. G. Duque , E. M. Bittar , L. Bufaiçal

Magnetic relaxation in coordination compounds is largely dominated by the interaction of the spin with phonons. Large zero-field splitting and exchange coupling values have been empirically found to strongly suppress spin relaxation and…

The interplay between spin dynamics and lattice vibration has been suggested as an important part of the puzzle of high-temperature superconductivity. Here we report the strong interaction between spin fluctuation and phonon in SmFeAsO, a…

Superconductivity · Physics 2010-10-29 L. Zhang , P. F. Guan , D. L. Feng , X. H. Chen , S. S. Xie , M. W. Chen

Type-II multiferroics, where spin interactions induce a ferroelectric polarization, are interesting for new device functionalities due to large magnetoelectric coupling. We report on a new type of multiferroicity in the quadruple-perovskite…

Magnetic frustrations and degeneracies profoundly affect ground-state magnetic properties emerging from competing exchange interactions. Controlling such frustrations using orbital and phonon engineering via the Kugel-Khomskii-type…

The low frequency lattice vibrations and relaxations are investigated in single crystals of the four 3D hybrid organolead perovskites, MAPbBr$_3$, FAPbBr$_3$, MAPbI$_3$, and $\alpha$-FAPbI$_3$, at the Brillouin zone center using Raman and…

First-principles calculations of the epitaxial-strain phase diagram of perovskite SrCoO$_{3}$ are presented. Through combination of the large spin-phonon coupling with polarization-strain coupling and coupling of the band gap to the polar…

Materials Science · Physics 2012-09-10 Jun Hee Lee , Karin M. Rabe
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