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Plasmons in nanostructured metals are widely utilized to trigger strong light--matter interactions with quantum light sources. While the nonclassical behavior of such quantum emitters (QEs) is well-understood in this context, the role of…

A rigorous account of quantum nonlocal effects is paramount for understanding the optical response of metal nanostructures and for designing plasmonic devices at the nanoscale. Here, we present a scheme for retrieving the quantum surface…

Mesoscale and Nanoscale Physics · Physics 2023-09-06 P. A. D. Gonçalves , F. Javier García de Abajo

Surface plasmons on metals can concentrate light into sub-nanometric volumes and on these near atomic length scales the electronic response at the metal interface is smeared out over a Thomas-Fermi screening length. This nonlocality is a…

Mesoscale and Nanoscale Physics · Physics 2015-06-16 Yu Luo , A. I. Fernandez-Dominguez , Aeneas Wiener , S. A. Maier , J. B. Pendry

We study the effect of electron spill-out and of nonlocality on the propagation of light inside a gap between two semi-infinite metallic regions. We compare the predictions of a local response model taking into account only the spill-out,…

Optics · Physics 2021-11-01 M. Khalid , O. Morandi , E. Mallet , P. A. Hervieux , G. Manfredi , A. Moreau , C. Ciracì

We explore theoretically how nonlocal corrections in the description of the metal affect the strong coupling between excitons and plasmons in typical examples where nonlocal effects are anticipated to be strong, namely small metallic…

Mesoscale and Nanoscale Physics · Physics 2018-01-18 Christos Tserkezis , Martijn Wubs , N. Asger Mortensen

Historically, the field of plasmonics has been relying on the framework of classical electrodynamics, with the local-response approximation of material response being applied even when dealing with nanoscale metallic structures. However,…

Noble metal nanostructures are ubiquitous elements in nano-optics, supporting plasmon modes that can focus light down to length scales commensurate with nonlocal effects associated with quantum confinement and spatial dispersion in the…

As the dimensions of plasmonic structures or the field confinement length approach the mean free path of electrons, mesoscopic optical response effects, including nonlocality, electron density spill-in or spill-out, and Landau damping, are…

Optics · Physics 2024-06-07 Weixiang Ye

Non-local effects in the optical response of noble metals are shown to produce significant blueshift and near-field quenching of plasmons in nanoparticle dimers, nanoshells, and thin metal waveguides. Compared with a local description…

Other Condensed Matter · Physics 2012-11-13 F. Javier Garcia de Abajo

Inspired by recent measurements on individual metallic nanospheres that can not be explained with traditional classical electrodynamics, we theoretically investigate the effects of nonlocal response by metallic nanospheres in three distinct…

Mesoscale and Nanoscale Physics · Physics 2014-03-07 Thomas Christensen , Wei Yan , Søren Raza , Antti-Pekka Jauho , N. Asger Mortensen , Martijn Wubs

Over the last three decades, plasmonics using metallic nanostructures has become central to nanophotonics research. Recently, its targets have been extended to nonlinear optical phenomena. In a nonlinear regime, quantum mechanical effects,…

Optics · Physics 2023-01-04 Takashi Takeuchi , Kazuhiro Yabana

Particle plasmons in metal nanoparticles have primarily been investigated through the use of local optical response approximations. However, as nanoparticle size approaches the average distance of electrons to the metal surface, mesoscopic…

Optics · Physics 2023-06-28 Weixiang Ye

We provide theoretical and numerical tools to quantitatively study the impact of nonlocality arising from free electrons in metals on the optical properties of metallo-dielectric multilayers. Though effects due to nonlocality are in general…

Collective optical excitations, such as localized surface plasmons in metallic nanoparticles and Mie resonances in high-index dielectrics, play a central role in nanoscale light--matter interactions. When such optical modes interact with…

Plasmon-exciton polaritons provide exciting possibilities to control light-matter interactions at the nanoscale by enabling closer investigation of quantum optical effects and facilitating novel technologies based, for instance, on…

Mesoscale and Nanoscale Physics · Physics 2020-02-25 Grigorios P. Zouros , Georgios D. Kolezas , N. Asger Mortensen , Christos Tserkezis

We analyze dispersion properties of metal-dielectric nanostructured metamaterials. We demonstrate that, in a sharp contrast to the results for the corresponding effective medium, the structure demonstrates strong optical nonlocality due to…

The plasmon response of metallic nanostructures is anticipated to exhibit nonlocal dynamics of the electron gas when exploring the true nanoscale. We extend the local-response approximation (based on Ohm's law) to account for a general…

Mesoscale and Nanoscale Physics · Physics 2014-03-04 N. Asger Mortensen

A local model of the dielectric response of a metal predicts that singular surfaces, such as sharp-edged structures, have a continuous absorption spectrum and extreme concentration of energy at the singularity. Here we show that nonlocality…

Mesoscale and Nanoscale Physics · Physics 2019-04-24 Fan Yang , Yao-Ting Wang , Paloma Arroyo Huidobro , John B Pendry

The electronic environment causes decoherence and dissipation of the collective surface plasmon excitation in metallic nanoparticles. We show that the coupling to the electronic environment influences the width and the position of the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Guillaume Weick , Gert-Ludwig Ingold , Rodolfo A. Jalabert , Dietmar Weinmann

Plasmon resonance, with strong coupling of light to electrons at a metal-dielectric interface, allows light confinement and control at subwavelength scale. It's fundamentally limited by the inherent mobility of the electrons, leading to the…

Optics · Physics 2019-02-20 Evgenii E. Narimanov
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