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We configure and analyze a nanostructured device that hybridizes grating modes and surface plasmon resonances. The model uses an effective index of refraction that considers the volume fraction of the involved materials, and the propagation…

Passive parity-time-symmetric medium provides a feasible scheme to investigate non-Hermitian systems experimentally. Here, we design a passive PT-symmetric acoustic grating with a period equal to exact PT-symmetric medium. This treatment…

Classical Physics · Physics 2019-09-25 Yuzhen Yang , Han Jia , Yafeng Bi , Han Zhao , Jun Yang

We present a novel approach to transient Raman spectroscopy, which combines stochastic probe pulses and a covariance-based detection to measure stimulated Raman signals in alpha-quartz. A coherent broadband pump is used to simultaneously…

Nonequilibrium pump-probe time domain spectroscopies can become an important tool to disentangle degrees of freedom whose coupling leads to broad structures in the frequency domain. Here, using the time-resolved solution of a model…

We introduce a wide-field magneto-optical microscope to probe magnetization dynamics with femtosecond temporal and sub-micrometer spatial resolution. We carefully calibrate the non-linear dependency between the magnetization of the sample…

Raman spectroscopy is a useful experimental tool to investigate local deformation and structural changes in SiO$_2$-based glasses. Using a semi-classical modelling of Raman spectra in large samples of silica glasses, we show in this paper…

Disordered Systems and Neural Networks · Physics 2015-02-04 Nikita S. Shcheblanov , Boris Mantisi , Paolo Umari , Anne Tanguy

Pump-probe microscopy enables label-free imaging of structural and chemical features of samples. However, signals in pump-probe microscopy are typically small and often must be measured in the presence of large backgrounds. As a result,…

Near-field infrared spectroscopy by elastic scattering of light from a probe tip resolves optical contrasts in materials at dramatically sub-wavelength scales across a broad energy range, with the demonstrated capacity for chemical…

Grating magneto-optical traps are an enabling quantum technology for portable metrological devices with ultracold atoms. However, beam diffraction efficiency and angle are affected by wavelength, creating a single-optic design challenge for…

Spectroscopic mapping refers to the massive recording of spectra whilst varying an additional degree of freedom, such as: magnetic field, location, temperature, or charge carrier concentration. As this involves two serial tasks,…

Materials Science · Physics 2021-11-15 Berk Zengin , Jens Oppliger , Danyang Liu , Lorena Niggli , Tohru Kurosawa , Fabian Donat Natterer

Label-free microscopy exploits light scattering to obtain a three-dimensional image of biological tissues. However, light propagation is affected by aberrations and multiple scattering, which drastically degrade the image quality and limit…

We explore theoretically the feasibility of using frequency conversion by sum- or difference-frequency generation, enabled by three- wave-mixing, for selectively multiplexing orthogonal input waveforms that overlap in time and frequency.…

Nonlinear spectroscopy employs a series of laser pulses to interrogate dynamics in large interacting many-body systems, and has become a highly successful method for experiments in chemical physics. Current quantum optical experiments…

Quantum Physics · Physics 2016-10-19 Frank Schlawin , Manuel Gessner , Shaul Mukamel , Andreas Buchleitner

Atomically thin two-dimensional (2D) semiconductors are extensively investigated for opto-electronic applications that require strong light-matter interactions. In view of such applications, it is essential to understand how…

Materials Science · Physics 2022-11-16 Pieter Schiettecatte , Zeger Hens , Pieter Geiregat

A spatio-temporal metasurface is proposed to decompose in real time the temporal frequencies of electromagnetic waves into spatial frequencies onto a two-dimensional plane. The metasurface is analyzed and demonstrated using Fourier…

Optics · Physics 2014-12-30 Shulabh Gupta , Christophe Caloz

We present an alternative approach to pump-probe spectroscopy for measuring fast charge dynamics with an atomic force microscope (AFM). Our approach is based on coherent multifrequency lock-in measurement of the intermodulation between a…

Mesoscale and Nanoscale Physics · Physics 2019-01-30 Riccardo Borgani , David B. Haviland

Femtosecond optical pump-probe technique is used to study charge carrier dynamics in few-layer MoS2 samples fabricated by mechanical exfoliation. An ultrafast pump pulse excites carriers and differential reflection of a probe pulse tuned to…

Mesoscale and Nanoscale Physics · Physics 2011-11-01 Rui Wang , Brian A. Ruzicka , Nardeep Kumar , Matthew Z. Bellus , Hsin-Ying Chiu , Hui Zhao

Absorption of ultrashort laser pulses in a metallic grating deposited on a transparent sample launches coherent compression/dilatation acoustic pulses in directions of different orders of acoustic diffraction. Their propagation is detected…

Applied Physics · Physics 2018-02-14 Osamu Matsuda , Thomas Pezeril , Ievgeniia Chaban , Kentaro Fujita , Vitalyi Gusev

Pump-probe spectroscopy is central for exploring ultrafast dynamics of fundamental excitations, collective modes and energy transfer processes. Typically carried out using conventional diffraction-limited optics, pump-probe experiments…

Transient field-resolved spectroscopy enables studies of ultrafast dynamics in molecules, nanostructures, or solids with sub-cycle resolution, but previous work has so far concentrated on extracting the dielectric response at frequencies…