Related papers: A Blue-Detuned Magneto-Optical Trap of CaF Molecul…
Direct laser cooling and trapping of molecules to temperature below Doppler limit and density exceeding $10^8$ are challenging due to the sub-Doppler heating effects of molecular magneto-optical trap (MOT). In our previous paper [1], we…
We report the realization of a blue-detuned magneto-optical trap (BDM) of BaF molecules. The (1 + 1) type BDM and (1 + 2) type conveyor-belt MOT are explored. While the (1+1) BDM provides only weak trapping force, the conveyor-belt MOT…
Direct laser cooling of molecules has reached a phase space density exceeding 10$^{-6}$ in optical traps, but with rather small molecular numbers. To progress towards quantum degeneracy, a mechanism is needed that combines sub-Doppler…
We present the properties and advantages of a new magneto-optical trap (MOT) where blue-detuned light drives `type-II' transitions that have dark ground states. Using $^{87}$Rb, we reach a radiation-pressure-limited density exceeding…
In red-detuned magneto-optical traps (MOTs) of molecules, sub-Doppler heating competes with Doppler cooling, resulting in high temperature and low density. A solution is offered by the blue-detuned MOT where sub-Doppler cooling dominates…
We demonstrate significantly improved magneto-optical trapping of molecules using a very slow cryogenic beam source and RF modulated and DC magnetic fields. The RF MOT confines $1.1(3) \times 10^5$ CaF molecules at a density of $4(1) \times…
We demonstrate a blue-detuned magneto-optical trap (MOT) of a polyatomic molecule, calcium monohydroxide (CaOH). We identify a novel MOT frequency configuration that produces high spatial compression of the molecular cloud. This high…
We report optical trapping of laser-cooled molecules at sufficient density to observe molecule-molecule collisions for the first time in a bulk gas. SrF molecules from a red-detuned magneto-optical trap (MOT) are compressed and cooled in a…
We exploit red- and blue-detuned magneto optical trapping (MOT) of $^{87}$Rb benefitting from a simplified setup based on liquid crystal variable retarders (LCVR). To maintain the trapping forces when switching from a red- to a blue-detuned…
We present the properties of a magneto-optical trap (MOT) of CaF molecules. We study the process of loading the MOT from a decelerated buffer-gas-cooled beam, and how best to slow this molecular beam in order to capture the most molecules.…
Recent experiments have demonstrated direct cooling and trapping of diatomic and triatomic molecules in magneto-optical traps (MOTs). However, even the best molecular MOTs to date still have density $10^{-5}$ times smaller than in typical…
Calcium monofluoride (CaF) molecules are loaded into an optical dipole trap (ODT) and subsequently laser cooled within the trap. Starting with magneto-optical trapping, we sub-Doppler cool CaF and then load $150(30)$ CaF molecules into an…
We describe experiments demonstrating efficient transfer of molecules from a magneto-optical trap (MOT) into a conservative magnetic quadrupole trap. Our scheme begins with a blue-detuned optical molasses to cool SrF molecules to $\sim\!50$…
We study several new magneto-optical trapping configurations in $^{87}$Rb. These unconventional MOTs all use type-II transitions, where the angular momentum of the ground state is greater than or equal to that of the excited state, and they…
As a heavy molecule, barium monofluoride (BaF) presents itself as a promising candidate for measuring permanent electric dipole moment. The precision of such measurements can be significantly enhanced by utilizing a cold molecular sample.…
We report the experimental realization of a conveyor-belt magneto-optical trap for calcium monofluoride (CaF) molecules. The obtained highly-compressed cloud has a mean radius of 64(5) $\mu$m and a peak number density of $3.6(5) \times…
We demonstrate a three-dimensional magneto-optical trap (MOT) of a metal hydride molecule, CaH. We are able to scatter $\sim$$10^{4}$ photons with vibrational loss covered up to vibrational quantum number $\nu=2$. This allows us to laser…
We report magneto-optical trapping (MOT) of a polyatomic molecule, calcium monohydroxide (CaOH). The MOT contains $2.0(5)\times 10^4$ CaOH molecules at a peak density of $3.0(8)\times10^{6}$ cm$^{-3}$. CaOH molecules are further sub-Doppler…
Current dual-frequency magneto-optical traps for ultracold molecules are plagued by sub-Doppler heating effects, making them vastly inferior to standard atomic MOTs. Here we demonstrate theoretically that the sub-Doppler effects in such a…
Laser cooling is used to produce ultracold atoms and molecules for quantum science and precision measurement applications. Molecules are more challenging to cool than atoms due to their vibrational and rotational internal degrees of…