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We report a detailed experimental and theoretical study on the effect of hydrostatic pressure on the structural and magnetic aspects of the layered honeycomb antiferromagent $\alpha$-RuCl$_{3}$. Magnetic susceptibility measurements…

We report on a temperature-driven reversible change of the in-plane magnetic anisotropy of V$_2$O$_3$/Ni bilayers. This is caused by the rhombohedral to monoclinic structural phase transition of V$_2$O$_3$ at $T_C$ = 160 K. The in-plane…

We report magnetic, thermodynamic, thermal expansion, and on detailed optical experiments on the layered compound $\alpha$-RuCl$_3$ focusing on the THz and sub-gap optical response across the structural phase transition from the monoclinic…

Strongly Correlated Electrons · Physics 2018-11-09 S. Reschke , F. Mayr , S. Widmann , H. -A. Krug von Nidda , V. Tsurkan , M. V. Eremin , Seung-Hwan Do , K. -Y. Choi , Zhe Wang , A. Loidl

In RuCl$_3$, inelastic neutron scattering and Raman spectroscopy reveal a continuum of non-spin-wave excitations that persists to high temperature, suggesting the presence of a spin liquid state on a honeycomb lattice. In the context of the…

$\alpha$-RuCl$_3$, a well-known candidate material for Kitaev quantum spin liquid, is prone to stacking disorder due to the weak van der Waals bonding between the honeycomb layers. After a decade of intensive experimental and theoretical…

The majority of research on $\alpha$-RuCl$_3$ has focused on applying in-plane magnetic fields to suppress antiferromagnetic order and induce a quantum spin liquid (QSL). However, this effort has been complicated by the materials…

Strongly Correlated Electrons · Physics 2026-05-14 Hamza Nasir Daniel Balazs , Muhammad Nauman , Ezekiel Horsley , Subin Kim , Young-June Kim , K. A. Modic

Hexagonal-to-orthorhombic structural transitions in RAl$_3$C$_3$ have been studied by X-ray diffraction for R=Yb, Tm, Er, Dy, and Lu. We report how orthorhombic domains are controlled by adjusting external magnetic fields. It is shown that…

Materials Science · Physics 2015-11-11 T. Matsumura , Y. Hayashi , S. Takai , T. Otsubo , S. Matsuda , A. Ochiai

$\alpha$-RuCl$_3$ is a promising candidate material to realize the so far elusive quantum spin liquid ground state. However, at low temperatures, the coexistence of different exchange interactions couple the effective pseudospins into an…

We present high-resolution thermal-expansion and specific-heat measurements of single crystalline alpha-RuCl3. An extremely hysteretic structural transition expanding over 100 K is observed by thermal- expansion along both crystallographic…

Strongly Correlated Electrons · Physics 2018-09-26 Mingquan He , Xiao Wang , Liran Wang , Frédéric Hardy , Thomas Wolf , Peter Adelmann , Thomas Brückel , Yixi Su , Christoph Meingast

The pivotal role of magnetic anisotropy in stabilising two-dimensional (2D) magnetism has been widely accepted, however, direct correlation between magnetic anisotropy and long-range magnetic ordering in the 2D limit is yet to be explored.…

Strongly Correlated Electrons · Physics 2021-08-09 Minjie Zhang , Qifeng Hu , Chenqiang Hua , Man Cheng , Zhou Liu , Shijie Song , Fanggui Wang , Pimo He , Guang-Han Cao , Zhu-An Xu , Yunhao Lu , Jinbo Yang , Yi Zheng

Magnetic properties of high-quality Al-free nonsuperconducting GdBa_2Cu_3O_{6+y} single crystals grown by flux method have been studied. The magnetic anisotropy below the N\'eel temperature T_N~2.3K corresponds to the direction of Gd^{3+}…

Materials Science · Physics 2016-08-31 V. N. Narozhnyi , D. Eckert , G. Fuchs , V. Nekvasil , K. -H. Müller

A pseudo honeycomb system Li2RuO3 exhibits a second-order-like transition at temperature T=Tc=540 K to a low-T nonmagnetic phase with a significant lattice distortion forming Ru-Ru pairs. For this system, we have calculated the band…

Strongly Correlated Electrons · Physics 2015-05-13 Yoko Miura , Masatoshi Sato , Youichi Yamakawa , Tatsuro Habaguchi , Yoshiaki Ono

Powder X-ray diffraction (PXRD) and single-crystal neutron scattering were used to study in detail the structural properties of the Cs2CuCl(4-x)Br(x) series, good realizations of layered triangular antiferromagnets. Detailed…

The results of a single-crystal X-ray-diffraction study of the evolution of crystal structures of VI3 with temperature with emphasis on phase transitions are presented. Some related specific-heat and magnetization data are included. The…

The honeycomb Mott insulator $\alpha$-RuCl$_3$ loses its low-temperature magnetic order by pressure. We report clear evidence for a dimerized structure at $P>1$ GPa and observe the breakdown of the relativistic $j_{\rm eff}$ picture in this…

We have investigated low-temperature crystal structure of BiCh2-based compounds LaO1-xFxBiSSe (x = 0, 0.01, 0.02, 0.03, and 0.5), in which anomalous two-fold-symmetric in-plane anisotropy of superconducting states has been observed for x =…

We compute the rotational anisotropy of the free energy of $\alpha$-RuCl$_3$ in an external magnetic field. This quantity, known as the magnetotropic susceptibility, $k$, relates to the second derivative of the free energy with respect to…

Strongly Correlated Electrons · Physics 2023-12-07 Toshihiro Sato , B. J. Ramshaw , K. A. Modic , Fakher F. Assaad

The layered honeycomb magnet $\alpha$-RuCl$_3$ has attracted intense scrutiny as a prime candidate for realizing the Kitaev quantum spin liquid, yet a consensus on its microscopic Hamiltonian remains elusive due to the material's extreme…

The Kitaev material $\alpha$-RuCl$_3$ is among the most prominent candidates to host a quantum spin-liquid state endowed with fractionalized excitations. Recent experimental and theoretical investigations have separately revealed the…

We have investigated the structural, magnetic, thermodynamic, and charge transport properties of Mn1/3NbS2 single crystals through x-ray and neutron diffraction, magnetization, specific heat, magnetoresistance, and Hall effect measurements.…