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Photoionization from energetically distinct electronic states may have a relative time delay of tens of attoseconds. Here we demonstrate that pulses of optical vortices allow measuring such attoseconds delays from magnetic sublevels, even…

Atomic Physics · Physics 2016-10-03 Jonas Wätzel , Jamal Berakdar

Plane-wave electrons undergo momentum transfer as they scatter off a target in overlapping spherical waves. The transferred momentum leads to target structural information to be encoded in angle and energy differential scattering. For…

Atomic and Molecular Clusters · Physics 2024-02-14 Aiswarya R. , Rasheed Shaik , Jobin Jose , Hari R. Varma , Himadri S. Chakraborty

Free-electron laser hard X-ray light sources can provide high fluence, femtosecond pulses, enabling the time-resolved probing of structural dynamics and elementary relaxation processes in molecules. Traditional X-ray elastic scattering from…

Chemical Physics · Physics 2016-11-23 Kochise Bennett , Markus Kowalewski , Shaul Mukamel

Ultrafast electron diffraction/microscopy technique enables us to investigate the nonequilibrium dynamics of crystal structures in the femtosecond-nanosecond time domain. However, the electron diffraction intensities are in general…

Materials Science · Physics 2024-07-10 Toshiya Shiratori , Jumpei Koga , Takahiro Shimojima , Kyoko Ishizaka , Asuka Nakamura

We demonstrate that spin-dependent electron diffraction is possible for a smooth range of transverse electron momenta in a two-photon Bragg scattering scenario of the Kapitza-Dirac effect. Our analysis is rendered possible by introducing a…

Quantum Physics · Physics 2024-01-19 Yang Wang , Sven Ahrens

Upon absorbing a photon, the ionized electron sails through the target force field in attoseconds to reach free space. This navigation probes details of the potential landscape that get imprinted into the phase of the ionization amplitude.…

Atomic Physics · Physics 2024-12-12 Sajad Azizi , Mohamed El-Amine Madjet , Zheng Li , Jan M. Rost , Himadri S. Chakraborty

Attosecond streaking of atomic photoemission holds the promise to provide unprecedented information on the release time of the photoelectron. We show that attosecond streaking phase shifts indeed contain timing (or spectral phase)…

In attosecond streaking, an electron is released by a short xuv pulse into a strong near infrared laser field. When the laser coupling between two states in the target is weak relative to the detuning, the streaking technique, which allows…

Atomic Physics · Physics 2015-05-19 Jan Conrad Baggesen , Lars Bojer Madsen

Bragg diffraction of an atomic wave packet in a retroreflective geometry with two counterpropagating optical lattices exhibits a light shift induced phase. We show that the temporal shape of the light pulse determines the behavior of this…

Quantum Physics · Physics 2016-12-21 Enno Giese , Alexander Friedrich , Sven Abend , Ernst M. Rasel , Wolfgang P. Schleich

A novel and universal interference structure is found in the photoelectron momentum distribution of atoms in intense infrared laser field. Theoretical analysis shows that this structure can be attributed to a new form of…

We theoretically investigate the scattering of an attosecond electron wave packet launched by an attosecond pulse under the influence of an infrared laser field. As the electron scatters inside a spatially extended system, the dressing…

Quantum Physics · Physics 2015-05-19 Justin Gagnon , Ferenc Krausz , Vladislav S. Yakovlev

We study Bragg scattering at 1D optical lattices. Cold atoms are confined by the optical dipole force at the antinodes of a standing wave generated inside a laser-driven high-finesse cavity. The atoms arrange themselves into a chain of…

Quantum Physics · Physics 2009-11-11 S. Slama , C. von Cube , A. Ludewig , M. Kohler , C. Zimmermann , Ph. W. Courteille

The shortest light pulses produced to date are of the order of a few tens of attoseconds, with central frequencies in the extreme ultraviolet range and bandwidths exceeding tens of eV. They are often produced as a train of pulses separated…

The dissociation dynamics of diatomic molecules interacting with (near) optical laser pulses of different duration is investigated by an elaborate discussion of the electric field of the laser and by a direct solution of the time-dependent…

Atomic Physics · Physics 2019-08-14 T. Fiedlschuster , J. Handt , E. K. U. Gross , R. Schmidt

Deviations from the perfect atomic arrangements in crystals play an important role in affecting their properties. Similarly, diffusion of such deviations is behind many microstructural changes in solids. However, observation of point defect…

Materials Science · Physics 2014-07-28 Jani Kotakoski , Clemens Mangler , Jannik C. Meyer

The elastic scattering of twisted electrons by diatomic molecules is studied within the framework of the non-relativistic first Born approximation. In this process, the coherent interaction of incident electrons with two molecular centers…

Atomic Physics · Physics 2018-10-17 A. V. Maiorova , S. Fritzsche , R. A. Mueller , A. Surzhykov

An unresolved issue in the theory of liquid crystals is the molecular basis of the electroclinic effect in the smectic-A phase. Recent x-ray scattering experiments suggest that, in a class of siloxane-containing liquid crystals, an electric…

Soft Condensed Matter · Physics 2009-11-07 J. V. Selinger , P. J. Collings , R. Shashidhar

Ultrashort electron pulses with a high average current provide a powerful means of enhancing time-resolved imaging and photon generation. In this study, we report the attosecond shaping of sub-relativistic electron beams using membranes in…

Recent progress in laser wakefield acceleration has led to the emergence of a new generation of electron and X-ray sources that may have enormous benefits for ultrafast science. These novel sources promise to become indispensable tools for…

We study the influence of the space and time dispersion on the frequency dependence of the wave vectors of electromagnetic waves propagating in three-dimensional photonic crystals. Two types of structures are considered: media with weak…

Other Condensed Matter · Physics 2007-05-23 F. Bass , V. Freilikher , O. Shefranova