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High-harmonic generation is a light up-conversion process occurring in a strong laser field, leading to coherent bursts of extreme ultrashort broadband radiation [1]. As a new perspective, we propose that ultrafast strong-field electronic…

The generation of high harmonics in laser-irradiated light homonuclear diatomics (H2+, N2 and O2) compared to that in atomic counterparts (of nearly identical binding energy) is studied within the velocity gauge version of conventional…

Atomic Physics · Physics 2009-11-11 Vladimir I. Usachenko , Pavel E. Pyak , Shih-I Chu

High-harmonic generation - the emission of high-frequency radiation by the ionization and subsequent recombination of an atomic electron driven by a strong laser field - is widely understood using a quasiclassical trajectory formalism,…

Quantum Physics · Physics 2020-07-29 Emilio Pisanty , Marcelo F. Ciappina , Maciej Lewenstein

Squeezing of optical fields, used as a powerful resource for many applications, and the radiation properties in the process of high harmonic generation have thus far been considered separately. In this Letter, we want to clarify that the…

Parametric oscillation is a fundamental concept that underlies nonlinear wave-matter interactions, leading to generation or amplification of new frequency components. Using a temporal modulation generated by the heterodyne interference of a…

Optics · Physics 2020-01-10 Xuexue Guo , Xingjie Ni

The quantum optical description of high-order harmonic generation where both the electrons of the generating medium and the driving and generated light fields are described quantum mechanically has been of significant interest in the past…

Quantum Physics · Physics 2025-02-05 Christian Saugbjerg Lange , Lars Bojer Madsen

High-harmonic generation (HHG) involves the up-conversion of a high-intensity driving field into its harmonic orders. This process is intrinsically non-classical, requiring from quantum mechanics for a complete explanation as, under…

Quantum Physics · Physics 2024-09-25 Javier Rivera-Dean

Quantum technologies are powered by platforms to generate complex non-classical states of matter or light to realize applications. We investigate the non-classical properties of high-harmonic generation in semiconductors, an emerging…

Quantum Physics · Physics 2026-03-18 David Theidel , Mackrine Nahra , Ilya Karuseichyk , Houssna Griguer , Mateusz Weis , Hamed Merdji

We present a theoretical model of high-harmonic generation from diatomic molecules. The theory includes effects of alignment as well as nuclear motion and is used to predict results for N$_2$, O$_2$, H$_2$ and D$_2$. The results show that…

Atomic Physics · Physics 2007-05-23 Christian Bruun Madsen , Lars Bojer Madsen

Quadratic optical parametric processes form the foundation for a variety of applications related to classical and quantum frequency conversion, which have attracted significant interest recently in on-chip implementation. These processes…

Optics · Physics 2018-09-19 Rui Luo , Yang He , Hanxiao Liang , Mingxiao Li , Qiang Lin

In this review, we compare different descriptions of photon-number statistics in harmonic generation processes within quantum, classical and semiclassical approaches. First, we study the exact quantum evolution of the harmonic generation by…

Quantum Physics · Physics 2007-05-23 Jiri Bajer , Adam Miranowicz

High-order harmonic generation (HHG) by hydrogenlike atoms/ions in the uniform periodic electric field, formed by the two linearly polarized counterpropagating laser beams of relativistic intensities, is studied. The relativistic quantum…

Atomic Physics · Physics 2011-06-14 H. K. Avetissian , A. G. Markossian , G. F. Mkrtchian

From the famous classical "simple man" model to the recent multichannel model for polyatomic molecules, this tutorial will guide you through the several landmarks in our understanding of high harmonic generation and high harmonic…

Atomic Physics · Physics 2013-04-10 Olga Smirnova , Misha Ivanov

We theoretically investigated the dependence of higher-order harmonic generation (HHG) in solid-state materials on the ellipticity of the electric field. We found that in the multiphoton absorption and ac Zener regimes, the intensity of HHG…

Materials Science · Physics 2016-12-28 T. Tamaya , A. Ishikawa , T. Ogawa , K. Tanaka

We develop a non-perturbative formulation based on the Green-function quantization method, that can describe spontaneous parametric down-conversion in the high-gain regime in nonlinear optical structures with arbitrary amount of loss and…

Quantum Physics · Physics 2023-12-13 Aleksa Krstić , Frank Setzpfandt , Sina Saravi

The generation of harmonics by atoms interacting with two circularly polarized and frequency related laser fields is addressed through ab initio numerical simulations. A detailed charaterization of a few specific harmonics is given. In…

Atomic Physics · Physics 2009-11-10 F. Ceccherini , N. Davini , D. Bauer , F. Cornolti

Quantum high-harmonic generation (HHG) is a prominent and growing field of research with potential capabilities of providing high photon-number entangled states of light. However, there is an open debate regarding the theory level required…

Quantum Physics · Physics 2026-03-16 Sebastián de-la-Peña , Heiko Appel , Angel Rubio , Ofer Neufeld

We address the process of generation of the photon-number entangled states of light in the stimulated nonlinear parametric down conversion process and build the simple model describing the generation, not involving the traditional…

Quantum Physics · Physics 2010-03-02 Oleksandr O. Gurin , Vladyslav C. Usenko , Constantin V. Usenko

This paper reports experimental evidence for phononic low-order to high-order harmonic conversion leading to high harmonic generation. Phononic high harmonic generation is mediated by a threshold dependent instability of a driven phonon…

Classical Physics · Physics 2018-04-24 Adarsh Ganesan , Cuong Do , Ashwin A. Seshia

Employing non-Hermitian Floquet theory, the strong-field process of high harmonic (HH) generation by a classical continuous-wave field irradiating ground-state atom is discovered to be controllable by placing the irradiated atom inside a…

Quantum Physics · Physics 2025-09-05 Zohar Amitay , Nimrod Moiseyev