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We describe the ground- and excited-state electronic structure of bulk MnO and NiO, two prototypical correlated electron materials, using coupled cluster theory with single and double excitations (CCSD). As a corollary, this work also…

A low concentration of cobalt clusters with a fcc structure and containing almost one thousand atoms are embedded in two different metallic matrices: platinum and niobium. Samples have been prepared using a co-deposition technique. Cobalt…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 M. Jamet , M. Negrier , V. Dupuis , J. Tuaillon-Combes , P. Melinon , A. Perez , W. Wernsdorfer , B. Barbara , J. Vogel , B. Baguenard

We fabricate high-quality c-axis oriented epitaxial YBa$_2$Cu$_3$O$_{7-x}$ films with 15% of yttrium atoms replaced by terbium (YTBCO) and study their electrical properties. The Tb substitution reduces the charge carrier density resulting…

Superconductivity · Physics 2023-11-17 M. Lyatti , I. Kraiem , T. Röper , I. Gundareva , G. Mussler , D. Grützmacher , T. Schäpers

Within a first principles framework, we study the electronic structure of the recently synthesized polymeric coordination compound Cu(II)-2,5-bis(pyrazol-1-yl)-1,4-dihydroxybenzene (CuCCP), which has been suggested to be a good realization…

Structural, elastic and thermal properties of cementite (Fe$_3$C) were studied using a Modified Embedded Atom Method (MEAM) potential for iron-carbon (Fe-C) alloys. Previously developed Fe and C single element potentials were used to…

The electronic ground states of the actinide dioxides AnO2 (with An=U, Np, Pu, Am, and Cm) are investigated employing first-principles calculations within the framework of the local density approximation +U (LDA+U) approach, implemented in…

Strongly Correlated Electrons · Physics 2014-10-22 Michi-To Suzuki , Nicola Magnani , Peter M. Oppeneer

We report density functional study of alternate fullerene-like cage structures and finite closed capped single-wall nanotubes of aluminum nitride. The cages and nanotubes studied are modeled as Al24N24, Al28N28, Al32N32, Al36N36, Al48N48,…

Materials Science · Physics 2009-11-11 Rajendra R. Zope , Brett I. Dunlap

We demonstrate that configurational electronic entropy, previously neglected, in {\it ab initio} thermodynamics of materials can qualitatively modify the finite-temperature phase stability of mixed-valence oxides. While transformations from…

Materials Science · Physics 2015-11-17 Fei Zhou , Thomas Maxisch , Gerbrand Ceder

By means of density functional theory the electronic structure of the MgB2 superconductor was characterised and compared with that of the related iso-structural systems: AlB2, ZrB2, NbB2, and TaB2. Using the full-potential linearized…

Superconductivity · Physics 2009-11-07 Pablo de la Mora , Miguel Castro , Gustavo Tavizon

We study the electronic and magnetic structure of carbon and nitrogen impurities and interstitials in rutile TiO${_2}$. To this end we perform \textit{ab-initio} calculations of a 48-atom supercell employing the VASP code. In order to…

Materials Science · Physics 2015-01-22 Jacqueline Atanelov , Christoph Gruber , Peter Mohn

The nudged-elastic band (NEB) method is modified with concomitant two climbing images (C2-NEB) to find a transition state (TS) in complex energy landscapes, such as those with serpentine minimal energy path (MEP). If a single climbing image…

Computational Physics · Physics 2017-11-28 Nikolai A. Zarkevich , Duane D. Johnson

In accordance with a relation between the lattice parameter c and the concentration of holes p, which has been found earlier for the YBa2Cu3O6+d compound, we obtain the p parameter in the same manner for the solid solution Nd1.2Ba1.8Cu3O6+d…

Materials Science · Physics 2018-01-03 A. V. Fetisov , S. Kh. Estemirova

Adiabatic mixed quantum/classical molecular dynamics simulations were used to generate snapshots of the hydrated electron (e-) in liquid water at 300 K. Water cluster anions that include two complete solvation shells centered on the e- were…

Data Analysis, Statistics and Probability · Physics 2016-09-28 Ilya A. Shkrob , William J. Glover , Ross E. Larsen , Benjamin J. Schwartz

We present a comprehensive theoretical study of the electronic structures of the Yb atom and the Yb$_2$ molecule, respectively, focusing on their ground and lowest-lying electronically excited states. Our study includes various…

The electronic structure of the nitrogenase metal cofactors is central to nitrogen fixation. However, the P-cluster and iron molybdenum cofactor, each containing eight irons, have resisted detailed characterization of their electronic…

Chemical Physics · Physics 2020-01-08 Zhendong Li , Sheng Guo , Qiming Sun , Garnet Kin-Lic Chan

The equation of state, structural behavior and phase stability of {\alpha}-uranium have been investigated up to 1.3 TPa using density functional theory, adopting a simple description of electronic structure that neglects the spin-orbit…

Materials Science · Physics 2015-05-28 S. Adak , H. Nakotte , P. F. de Châtel , B. Kiefer

The alloying effect on the lattice parameters, isostructural mixing enthalpies and ductility of the ternary nitride systems Cr1-xTMxN (TM=Sc, Y; Ti, Zr, Hf; V, Nb, Ta; Mo, W) in the cubic B1 structure has been investigated using…

Materials Science · Physics 2014-07-10 Liangcai Zhou , David Holec , Paul. H. Mayrhofer

In this study, we investigate effects of boron substitution on the structural and electronic properties of small tungsten clusters using density functional theory (DFT). We construct a series of tungsten boride clusters by replacing…

Materials Science · Physics 2025-12-17 Akshata M. Waghmare , Sajeev S. Chacko , Balasaheb J. Nagare

We present a comprehensive density functional theory (DFT) study of the electronic, magnetic, and topological properties of the layered pnictides EuMnXBi2 (X = Mn, Fe, Co, Zn), focusing in particular on the relatively unexplored Bi-based…

Materials Science · Physics 2026-04-07 Deep Sagar , Abhishek Sharma , Arti Kashyap

We present a systematic first-principles study of substitutional 3d transition-metal (TM) defects in CsPbI3 using the spin-polarized GGA+U framework. TM incorporation is generally energetically favorable and induces lattice distortions that…

Materials Science · Physics 2025-12-18 Misbah Shaheen , Sheharyar Pervez