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We present a continuum approach to model segregation of size-bidisperse granular materials in unsteady bounded heap flow as a prototype for modeling segregation in other time varying flows. In experiments, a periodically modulated feed rate…

Soft Condensed Matter · Physics 2022-08-02 Hongyi Xiao , Zhekai Deng , Julio M. Ottino , Paul B. Umbanhowar , Richard M. Lueptow

Molecular dynamics (MD) simulations are used to determine the diffusion coefficients, electrophoretic mobilities and electrical conductivity of a charged colloidal suspension in the salt-free regime as a function of the colloid charge. The…

Soft Condensed Matter · Physics 2010-12-16 Sorin Bastea

In this article, we demonstrate a method for inducing reversible crystal-to-crystal transitions in binary mixtures of soft colloidal particles. Through a controlled decrease of salinity and increasingly dominating electrostatic…

Soft Condensed Matter · Physics 2021-08-30 Jasper N. Immink , Maxime J. Bergman , J. J. Erik Maris , Joakim Stenhammar , Peter Schurtenberger

Dynamical heterogeneities in a colloidal fluid close to gelation are studied by means of computer simulations. A clear distinction between some fast particles and the rest, slow ones, is observed, yielding a picture of the gel composed by…

Soft Condensed Matter · Physics 2009-11-10 Antonio M. Puertas , Matthias Fuchs , Michael E. Cates

The liquid-liquid phase separation of a binary solvent can be arrested by colloidal particles trapped at the interface [K. Stratford et al., Science 309, 5744 (2005)]. We show experimentally that the colloidal network so formed can remain…

Soft Condensed Matter · Physics 2015-05-14 Eduardo Sanz , Kathryn A. White , Paul S. Clegg , Michael E. Cates

We study theoretically the evaporation-driven phase separation of a binary fluid mixture in a thin film deposited on a moving substrate, as occurs in meniscus-guided deposition for solution-processed materials. Our focus is on rapid…

Soft Condensed Matter · Physics 2024-07-01 René de Bruijn , Anton A. Darhuber , Jasper J. Michels , Paul van der Schoot

Colloidal particles are often seen as big atoms that can be directly observed in real space. They are therefore playing an increasingly important role as model systems to study processes of interest in condensed matter physics such as…

Phase transitions and collective dynamics of active colloidal suspensions are fascinating topics in soft matter physics, particularly for out-of-equilibrium systems, which can lead to rich rheological behaviours in the presence of steady…

Soft Condensed Matter · Physics 2023-01-16 A. Gülce Bayram , Fabian Jan Schwarzendahl , Hartmut Löwen , Luca Biancofiore

When a suspension freezes, a compacted particle layer builds up at the solidification front with noticeable implications on the freezing process. In a directional solidification experiment of monodispersed suspensions in thin samples, we…

Soft Condensed Matter · Physics 2019-05-08 Brice Saint-Michel , Marc Georgelin , Sylvain Deville , Alain Pocheau

We consider the dynamic wetting and dewetting processes of films and droplets of complex liquids on planar surfaces, focusing on the case of colloidal suspensions, where the particle interactions can be sufficiently attractive to cause…

Fluid Dynamics · Physics 2024-11-20 J. Zhang , D. N. Sibley , D. Tseluiko , A. J. Archer

When a drop containing colloidal particles evaporates on a surface, a circular stain made of these particles is often observed due to an internal flow toward the contact line. To hinder this effect, several approaches have been proposed…

Soft Condensed Matter · Physics 2016-01-06 François Boulogne , François Ingremeau , Julien Dervaux , Laurent Limat , Howard A. Stone

The thermodynamics of phase transitions of binary solutions into spatially inhomogeneous one-dimensional states is studied theoretically with taking into account nonlinear effects. It is shown that below the spinodal decomposition…

Statistical Mechanics · Physics 2022-03-18 Yu. M. Poluektov , A. A. Soroka

Molecular dynamics simulations are used to study fluidization of a vertically vibrated, three-dimensional shallow granular layer. As the container acceleration is increased above g, the granular temperature and root mean square particle…

Soft Condensed Matter · Physics 2007-08-01 Jennifer Kreft , Matthias Schroeter , Jack B. Swift , Harry L. Swinney

Using mesoscopic numerical simulations and analytical theory we investigate the coarsening of the solvent structure around a colloidal particle emerging after a temperature quench of the colloid surface. Qualitative differences in the…

Soft Condensed Matter · Physics 2018-04-18 Sutapa Roy , S. Dietrich , Anna Maciolek

We investigate the phase diagram of a two-component associating fluid mixture in the presence of selectively adsorbing substrates. The mixture is characterized by a bulk phase diagram which displays peculiar features such as closed loops of…

Statistical Mechanics · Physics 2009-11-07 J. M. Romero-Enrique , L. F. Rull , U. Marini Bettolo Marconi

We present a computer simulation study on the crystal nucleation process in suspensions of hard spheres, fully taking into account the solvent hydrodynamics. If the dynamics of collodial crystallization were purely diffusive, the crystal…

Soft Condensed Matter · Physics 2015-06-12 Marc Radu , Tanja Schilling

We investigate theoretically the bifurcation scenario for colloidal suspensions subject to a vertical temperature gradient taking into account the effect of sedimentation. In contrast to molecular binary mixtures, here the thermal…

Pattern Formation and Solitons · Physics 2015-05-13 A. Ryskin , H. Pleiner

Using a phase field crystal model we study the structure and dynamics of a drop of colloidal suspension during evaporation of the solvent. We model an experimental system where contact line pinning of the drop on the substrate is…

Soft Condensed Matter · Physics 2012-09-06 Nirmalendu Ganai , Arnab Saha , Surajit Sengupta

We present dynamical density functional theory results for the time evolution of the density distribution of a sedimenting model two-dimensional binary mixture of colloids. The interplay between the bulk phase behaviour of the mixture, its…

Soft Condensed Matter · Physics 2015-06-17 Alexandr Malijevsky , Andrew J. Archer

Drying suspensions often leave behind complex patterns of particulates, as might be seen in the coffee stains on a table. Here we consider the dynamics of periodic band or uniform solid film formation on a vertical plate suspended partially…

Soft Condensed Matter · Physics 2014-12-05 C. Nadir Kaplan , Ning Wu , Shreyas Mandre , Joanna Aizenberg , L. Mahadevan