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Dual-comb spectroscopy enables broadband, high-resolution measurements with microsecond temporal resolution, but extending this capability to the 10~12.5 $\mu$m molecular fingerprint region remains technically challenging, particularly for…

Optics · Physics 2026-04-30 Pei-Ling Luo , I-Yun Chen

We devise a new detection technique for mid-infrared multi-heterodyne spectroscopy. As an experimental implementation, mid-infrared light interrogates a gas sample in the 3-$\mu$m region of the fundamental CH, OH, NH stretch in molecules…

Optics · Physics 2020-03-17 Zaijun Chen , Theodor W. Hänsch , Nathalie Picqué

Dual-comb spectroscopy is a rapidly developing technique enabling ultraprecise broadband optical diagnostics of atoms and molecules. This powerful tool typically requires two phase-locked femtosecond lasers, yet it has been shown that it…

Dual comb spectroscopy allows for high-resolution spectra to be measured over broad bandwidths, but an essential requirement for coherent integration is the availability of a phase reference. Usually, this means that the combs' phase and…

Optics · Physics 2016-06-01 David Burghoff , Yang Yang , Qing Hu

Coherent Raman microscopy provide label-free imaging by interrogating the intrinsic vibration of biomolecules. Nevertheless, trade-off between high chemical-specificity and high imaging-speed currently exists in transition from spectroscopy…

Optics · Physics 2017-10-11 Kun Chen , Tao Wu , Tao Chen , Tian Zhou , Haoyun Wei , Yan Li

Frequency comb spectroscopy provides broadband access to molecular fingerprints with mode-defined spectral resolution. However, its deployment in non-cooperative gas sensing remains challenging because conventional implementations require…

Light detection and ranging (LIDAR) is critical to many fields in science and industry. Over the last decade, optical frequency combs were shown to offer unique advantages in optical ranging, in particular when it comes to fast distance…

We demonstrate dual-comb spectroscopy based on difference frequency generation of frequency-agile near-infrared frequency combs, produced with the help of electro-optic modulators. The combs have a remarkably flat intensity distribution and…

Dual-comb spectroscopy has demonstrated remarkable capabilities for rapid and sensitive measurements; however, significant challenges still exist in generating high-power, mutually coherent mid-infrared combs. Here we demonstrate that a…

Optical two-dimensional coherent spectroscopy (2DCS) has become a powerful tool for studying energy level structure, dynamics, and coupling in many systems including atomic ensembles. Various types of two-dimensional (2D) spectra, including…

Atomic Physics · Physics 2022-05-25 Jieli Yan , Stephen Revesz , Danfu Liang , Hebin Li

Frequency combs, spectra of evenly-spaced narrow phase-coherent laser lines, have revolutionized precision measurements. On-chip frequency comb generators hold much promise for fully-integrated instruments of time and frequency metrology.…

To meet climate targets, the IPCC underscores the necessity of technologies capable of removing gigatonnes of CO2 annually, with Geological Carbon Storage (GCS) playing a central role. GCS involves capturing CO2 and injecting it into deep…

Computational Physics · Physics 2025-02-12 Abhinav Prakash Gahlot , Felix J. Herrmann

There is a growing urgency to track greenhouse gasses with the resolution, precision and accuracy needed to support independent verification of $CO_2$ fluxes at local to global scales. The current generation of space-based sensors, however,…

Atmospheric and Oceanic Physics · Physics 2026-05-27 Aaron Sonabend-W , Sean Campbell , John Platt , Christopher Van Arsdale , Anna M. Michalak

Dual-comb ranging has emerged as an effective technology for long-distance metrology, providing absolute distance measurements with high speed, precision, and accuracy. Here, we demonstrate a dual-comb ranging method that utilizes a…

Laser-based range measurement systems (LIDAR) are important in many application areas including autonomous vehicles, robotics, manufacturing, formation-flying of satellites, and basic science. Coherent laser ranging systems using dual…

Optics · Physics 2018-02-27 Myoung-Gyun Suh , Kerry Vahala

Breath analysis enables rapid, non-invasive diagnostics, as well as long-term monitoring, of human health through the identification and quantification of exhaled biomarkers. Here, for the first time, we demonstrate the remarkable…

Chemical Physics · Physics 2022-06-07 Qizhong Liang , Ya-Chu Chan , P. Bryan Changala , David J. Nesbitt , Jun Ye , Jutta Toscano

Spectroscopic ellipsometry is a means to investigate optical and dielectric material responses. Conventional spectroscopic ellipsometry has trade-offs between spectral accuracy, resolution, and measurement time. Polarization modulation has…

Attosecond light sources based on high-order harmonic generation (HHG) constitute to date the only table-top solution for producing coherent broadband radiation covering the spectral range from the extreme ultraviolet to the soft X-rays.…

We present a new type of dual optical frequency comb source capable of scaling applications to high measurement speeds while combining high average power, ultra-low noise operation, and a compact setup. Our approach is based on a…

We report a high-energy, bidirectional, dissipative soliton mode-locked fiber laser operating in the 1550 nm normal-dispersion regime. By leveraging intracavity dispersion management and a Lyot filtering mechanism, the laser achieves…

Optics · Physics 2026-02-17 Mingjun Wang , Zhangru Shi , Anshuang Wang , Bowen Li
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