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We study the effect of electron-electron interactions in the optical conductivity of graphene under applied bias and derive a generalization of Elliot's formula, commonly used for semiconductors, for the optical intensity. We show that {\it…

Mesoscale and Nanoscale Physics · Physics 2010-07-29 N. M. R. Peres , R. M. Ribeiro , A. H. Castro Neto

Realizing strong nonlinear optical responses is a long-standing goal of both fundamental and technological importance. Recently significant efforts have focused on exploring excitons in solids as a pathway to achieving nonlinearities even…

Mesoscale and Nanoscale Physics · Physics 2023-06-21 Liuxin Gu , Lifu Zhang , Ruihao Ni , Ming Xie , Dominik S. Wild , Suji Park , Houk Jang , Takashi Taniguchi , Kenji Watanabe , Mohammad Hafezi , You Zhou

In quantum electrodynamics, optical processes are theoretically described by double-sided Feynman diagrams. This formalism is powerful in the case of molecules but proves inappropriate to account for light-matter interactions within complex…

Optics · Physics 2019-06-10 T. Noblet , C. Humbert

We study the linear optical absorption of bulk semiconductors in the presence of a homogeneous constant (dc) electric field with an approach suitable for including excitonic effects while working with many-band models. The absorption…

Mesoscale and Nanoscale Physics · Physics 2015-06-19 Federico Duque-Gomez , J. E. Sipe

We present a systematic theory of Coulomb interaction effects in the nonlinear optical processes in semiconductors using a perturbation series in the exciting laser field. The third-order dynamical response consists of phase-space filling…

Condensed Matter · Physics 2009-10-31 Th. Oestreich , K. Schoenhammer , L. J. Sham

The effects of the electron-phonon interaction on optical excitations can be understood in terms of exciton-phonon coupling, and require a careful treatment in low-dimensional materials with strongly bound excitons or strong electron-hole…

Materials Science · Physics 2022-02-17 Gabriel Antonius , Steven G. Louie

Recently, we have derived the changes in the absorption spectrum of an exciton when this exciton is photocreated close to a metal. The resolution of this problem -- which has similarities with Fermi edge singularities -- has been made…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 M. Combescot , O. Betbeder-Matibet

Excitons in a semiconductor monolayer form a collective resonance that can reflect resonant light with extraordinarily high efficiency. Here, we investigate the nonlinear optical properties of such atomistically thin mirrors and show that…

Mesoscale and Nanoscale Physics · Physics 2022-03-02 Valentin Walther , Lida Zhang , Susanne F. Yelin , Thomas Pohl

In this work we present a new procedure to compute optical spectra including excitonic effects and approximated quasiparticle corrections with reduced computational effort. The excitonic effects on optical spectra are included by solving…

Materials Science · Physics 2020-08-26 Filipe Matusalem , Marcelo Marques , Ivan Guilhon , Lara K. Teles

The optical response of two-dimensional materials is often significantly impacted by excitonic effects due to the reduced screening of attractive Coulomb interactions in low-dimensional systems. Accurate modeling of exciton formation and…

Materials Science · Physics 2026-03-09 Dmitry Tumakov , Daria Popova-Gorelova

Remarkable optical and electrical properties of two-dimensional (2D) materials, such as graphene and transition-metal dichalcogenide (TMDC) monolayers, offer vast technological potential for novel and improved optoelectronic nanodevices,…

Optics · Physics 2016-07-22 Martin Weismann , Nicolae C. Panoiu

Second-order nonlinear optical response allows to detect different properties of the system associated with the inversion symmetry breaking. Here, we use a second harmonic generation effect to investigate the alignment of a…

Mesoscale and Nanoscale Physics · Physics 2020-07-03 E. A. Stepanov , S. V. Semin , C. R. Woods , M. Vandelli , A. V. Kimel , K. S. Novoselov , M. I. Katsnelson

Excitons -- bound electron-hole pairs -- play a central role in light-matter interaction phenomena, and are crucial for wide-ranging applications from light harvesting and generation to quantum information processing. A long-standing…

Mesoscale and Nanoscale Physics · Physics 2023-08-15 Jenny Hu , Etienne Lorchat , Xueqi Chen , Kenji Watanabe , Takashi Taniguchi , Tony F. Heinz , Puneet A. Murthy , Thibault Chervy

We present a method, based on noncollinear second harmonic generation, to evaluate the non-zero elements of the nonlinear optical susceptibility. At a fixed incidence angle, the generated signal is investigated by varying the polarization…

The momentum-space signatures of excitons can be experimentally accessed through time-resolved (pump-probe) photoelectron spectroscopy. In this work, we develop a computational framework for exciton photoemission orbital tomography (exPOT)…

Techniques for coherent multidimensional optical spectroscopy have been developed and utilised to understand many different processes, including energy transfer in photosynthesis and many-body effects in semiconductor nanostructures.…

Optics · Physics 2017-01-24 Jonathan Tollerud , Jeffrey Davis

Motivated by the gigantic nonlinear optical response in the halogen-bridged Ni-compounds, the underlying electronic states of the compounds are examined in the one-dimensional two-band Hubbard model, by studying the current-current…

Strongly Correlated Electrons · Physics 2009-11-10 H. Matsueda , T. Tohyama , S. Maekawa

We present a theory of excitonic processes in gate controlled graphene quantum dots. The dependence of the energy gap on shape, size and edge for graphene quantum dots with up to a million atoms is predicted. Using a combination of…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 A. D. Guclu , P. Potasz , P. Hawrylak

Strong Coulomb interaction in atomically-thin transition metal dichalcogenides makes these systems particularly promising for studies of excitonic physics. Of special interest are the manifestations of the charged excitons, also known as…

Mesoscale and Nanoscale Physics · Physics 2020-08-26 M. M. Glazov

The concept of \textit{optical} exciton - a photo-excited bound electron-hole pair within a crystal - is routinely used to interpret and model a wealth of excited-state phenomena in semiconductors. Beside originating sub-band gap signatures…

Materials Science · Physics 2022-09-21 Fulvio Paleari , Andrea Marini