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We theoretically demonstrate the quenching effect in below-threshold high harmonic generation (HHG) by using the time-dependent density-functional theory (TDDFT) and solving the time-dependent Schr\"{o}dinger equation (TDSE). It is shown…

Atomic Physics · Physics 2016-08-31 Xiaosong Zhu , Xi Liu , Pengfei Lan , Qingbin Zhang , Yueming Zhou , Min Li , Peixiang Lu

High-order harmonic generation (HHG), a robust tabletop source for producing attosecond pulses, has been extensively utilized in attosecond metrology. Traditionally, HHG driven by classical laser fields involves two typical quantum paths…

High harmonic generation (HHG) is a manifestation of the strongly nonlinear response of matter to intense laser fields and has, as the basis for coherent XUV sources a variety of applications. Recently, HHG from atoms in a phase and…

Optics · Physics 2020-05-20 Jonas Wätzel , Jamal Berakdar

The spectra produced by high-harmonic generation (HHG) typically exhibit well-defined peaks at odd integers times the laser frequency. However, in recent investigations of HHG from correlated materials, spectra exhibit signals at noninteger…

Atomic Physics · Physics 2024-06-05 Christian Saugbjerg Lange , Thomas Hansen , Lars Bojer Madsen

We investigate high-order harmonic generation (HHG) in graphene with a quantum master equation approach. The simulations reproduce the observed enhancement in HHG in graphene under elliptically polarized light [N. Yoshikawa et al, Science…

Materials Science · Physics 2021-02-03 Shunsuke A. Sato , Hideki Hirori , Yasuyuki Sanari , Yoshihiko Kanemitsu , Angel Rubio

The underlying physics behind the molecular harmonic emission in relatively long sin$^2$-like laser pulses is investigated. We numerically solved the full-dimensional electronic time-dependent Schr\"{o}dinger equation beyond the…

Atomic Physics · Physics 2016-09-21 H. Ahmadi , M. Vafaee , A. Maghari

The production of brighter coherent XUV radiation by intense laser pulses through the process of high-harmonic generation (HHG) is a central challenge in contemporary nonlinear optics. We study the generation and spatial propagation of high…

Optics · Physics 2025-06-03 Margarita Khokhlova , Vasily Strelkov

Applying the semiclassical model, we identify two connected effects in intraband high-harmonic generation (HHG): (1) propagation time from the point of emission at the source to the point of detection, (2) beyond-electric-dipole corrections…

Atomic Physics · Physics 2024-06-12 Simon Vendelbo Bylling Jensen , Lars Bojer Madsen

High harmonic generation (HHG) is used to measure the spectral phase of the recombination dipole matrix element (RDM) in argon over a broad frequency range that includes the 3p Cooper minimum (CM). The measured RDM phase agrees well with…

Atomic Physics · Physics 2015-06-17 S. B. Schoun , R. Chirla , J. Wheeler , C. Roedig , P. Agostini , L. F. DiMauro , K. J. Schafer , M. B. Gaarde

Acting as a highly nonlinear response to the strong laser field, high harmonic generation (HHG) naturally contains the fingerprints of atomic and electronic properties of materials. Electronic properties of a solid such as band structure…

Materials Science · Physics 2023-04-20 Shi-Qi Hu , Hui Zhao , Xin-Bao Liu , Da-Qiang Chen , Sheng Meng

High harmonic generation (HHG) is an extreme nonlinear process where intense pulses of light drive matter to emit high harmonics of the driving frequency, reaching the extreme ultraviolet (XUV) and x-ray spectral ranges. So far, the HHG…

High-harmonic generation (HHG) in strongly correlated Mott insulators is investigated using exact diagonalization and time-dependent density-matrix propagation of a laser-driven one-dimensional Hubbard chain. By projecting onto equilibrium…

Optics · Physics 2026-05-05 Tao-Yuan Du , Hui-Ru Li , Bo Li , Ruifeng Lu

The non-linear propagation of the intense near-infrared (NIR) driving field in wide bandgap materials pose a challenge and an opportunity to control the spectral properties of high harmonic generation (HHG) in solids. Here, we have…

Optics · Physics 2023-07-06 Mukhtar Hussain , Gareth O Williams , Tayyab Imran , Marta Fajardo

High harmonic emissions from crystalline solids contain rich information on the dynamics of electrons driven by intense infrared laser fields and have been intensively studied owing to their potential use as a probe of microscopic…

Materials Science · Physics 2023-05-01 K. Uchida , K. Tanaka

The solid-state harmonic generation (SSHG) derives from photocurrent coherence. The crystal symmetry, including point-group symmetry and time-reversal symmetry, constrains the amplitude and phase of the photocurrent, thus manipulates the…

Optics · Physics 2024-01-17 Chen Qian , Shicheng Jiang , Tong Wu , Hongming Weng , Chao Yu , Ruifeng Lu

This paper focuses on investigating high-order harmonic generation (HHG) in graphene quantum dots (GQDs) under intense near-infrared laser fields. To model the GQD and its interaction with the laser field, we utilize a mean-field approach.…

Mesoscale and Nanoscale Physics · Physics 2023-09-15 H. K. Avetissian , A. G. Ghazaryan , Kh. V. Sedrakian , G. F. Mkrtchian

In this paper, we investigate the effects of full electronic correlation on the high harmonic generation in the helium atom subjected to laser pulses of extremely high intensity. To do this, we perform real-time propagations of the helium…

Chemical Physics · Physics 2022-05-18 Aleksander P. Woźniak , Michał Przybytek , Maciej Lewenstein , Robert Moszyński

We theoretically investigate detuning-dependent properties of high-order harmonic generation (HHG) in monolayer transition metal dichalcogenides (TMDCs). In contrast to HHG in conventional materials, TMDCs show both parallel and…

Materials Science · Physics 2018-04-18 Tomohiro Tamaya , Satoru Konabe , Shiro Kawabata

High-harmonic generation (HHG) from solid state offers promising potential for attosecond optics with enhanced efficiency and compact configurations. However, Current implementations face critical limitations imposed by material damage…

Optics · Physics 2025-08-19 Qing-Guo Fan , Kang Lai , Wen-hao Liu , Lin-Wang Wang , Jun-Wei Luo , Zhi Wang

High-order harmonic generation (HHG) in gases leads to short-pulse extreme ultraviolet (XUV) radiation useful in a number of applications, for example, attosecond science and nanoscale imaging. However, this process depends on many…