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Multiple exciton generation (MEG) is a widely studied phenomenon in semiconductor nanocrystals and quantum dots wherein photo-excited carriers relax by generating additional electron-hole pairs. Here, we present the first experimental…

Materials Science · Physics 2023-10-27 S. R. Sahu , A. Tripathy , K. Dey , N. Mansuri , V. G. Sathe , D. K. Shukla

Multiple exciton generation (MEG) is a process in which more than one exciton is generated upon the absorption of a high energy photon, typically higher than two times the band gap, in semiconductor nanocrystals. It can be observed…

Utilizing the excess energy of photoexcitation that is otherwise lost as thermal effects can improve the efficiency of next-generation light-harvesting devices. Multiple exciton generation (MEG) in semiconducting materials yields two or…

Materials Science · Physics 2022-12-06 Ashish Soni , Dushyant Kushavah , Li-Syuan Lu , Wen-Hao Chang , Suman Kalyan Pal

We have shown theoretically that efficient multiple exciton generation (MEG) by a single photon can be observed in small nanocrystals (NCs). Our quantum simulations that include hundreds of thousands of exciton and multi-exciton states…

Mesoscale and Nanoscale Physics · Physics 2010-09-23 Wayne M. Witzel , Andrew Shabaev , C. Stephen Hellberg , Verne L. Jacobs , Alexander L. Efros

Multiple exciton generation (MEG) in nanometer-sized hydrogen-passivated silicon nanowires (NWs), and quasi two-dimensional nanofilms strongly depends on the degree of the core structural disorder as shown by the many-body perturbation…

Mesoscale and Nanoscale Physics · Physics 2014-11-25 Andrei Kryjevski , Dmitri Kilin

We show that bi-exciton formation can be highly efficient in a solar cell with the semiconductor absorber filled with an array of metallic nanoparticles having plasmonic resonance tuned to the semiconductor gap energy. This process can be…

Materials Science · Physics 2019-06-12 Jiantao Kong , Xueyuan Wu , Xin Wang , Michael J Naughton , Krzysztof Kempa

We study the coherent mixing between two-particle (single exciton) and four-particle (biexciton) states of a semiconductor nanocrystal resulting from the coulomb coupling between states with different numbers of electron-hole pairs. Using a…

Mesoscale and Nanoscale Physics · Physics 2016-02-26 P. Kowalski , P. Machnikowski

We use Boltzmann transport equation (BE) to study time evolution of a photo-excited state in a nanoparticle including phonon-mediated exciton relaxation and the multiple exciton generation (MEG) processes, such as exciton-to-biexciton…

Mesoscale and Nanoscale Physics · Physics 2017-11-22 Andrei Kryjevski , Deyan Mihaylov , Svetlana Kilina , Dmitri Kilin

The two-dimensional semiconductor MoS2 in its mono- and few-layer form is expected to have a significant exciton binding energy of several 100 meV, leading to the consensus that excitons are the primary photoexcited species. Nevertheless,…

Multiple exciton generation is a process in which more than one electron hole pair is generated per absorbed photon. It allows us to increase the efficiency of solar energy harvesting. Experimental studies have shown the multiple exciton…

Mesoscale and Nanoscale Physics · Physics 2016-08-11 Fikeraddis A. Damtie , Khadga J. Karki , Tõnu Pullerits , Andreas Wacker

Unique properties of lead chalcogenides have enabled multiple exciton generation (MEG) in their nanocrystals that can be beneficial in enhancing the efficiency of the third generation solar cells. Although the intrinsic electric field plays…

Atomic and Molecular Clusters · Physics 2017-09-07 Mahdi Gordi , Mohammad Kazem Moravvej-Farshi , Hamidreza Ramezani

Magnetoelectroluminescence (MEL) of organic semiconductor has been experimentally tuned by adopting blended emitting layer consisting of both hole and electron transporting materials. A theoretical model considering intermolecular quantum…

Materials Science · Physics 2015-05-14 B. F. Ding , Y. Yao , X. Y. Sun , Z. Y. Sun , X. D. Gao , Z. T. Xie , Z. J. Wang , X. M. Ding , Y. Z. Wu , X. F. Jin , C. Q. Wu , X. Y. Hou

Multiple exciton generation solar cells exhibit a low power conversion efficiency owing to nonradiative recombination even if numerous electron and hole pairs are generated per incident photon. This paper elucidates the non-idealities of…

Applied Physics · Physics 2021-04-14 Jongwon Lee

Although van der Waals layered transition metal dichalcogenides from transient absorption spectroscopy have successfully demonstrated an ideal carrier multiplication (CM) performance with an onset of nearly 2Eg,interpretation of the CM…

Mesoscale and Nanoscale Physics · Physics 2021-04-20 Jun Suk Kim , Minh Dao Tran , Sung-Tae Kim , Daehan Yoo , Sang-Hyun Oh , Ji-Hee Kim , Young Hee Lee

The population dynamics of single- and bi-exciton states in semiconductor nanocrystals is modeled numerically in the presence of Coulomb coupling between single- and two-exciton states and a dissipation channel in order to study the…

Mesoscale and Nanoscale Physics · Physics 2013-09-11 Maryam Azizi , Paweł Machnikowski

This paper reviews both experimental and theoretical work on nanostructures showing high quantum yields due to the phenomenon of multiple exciton generation. It outlines the aims and barriers to progress in identifying further such…

Mesoscale and Nanoscale Physics · Physics 2018-06-06 Nicholas Siemons , Alessio Serafini

In single-junction photovoltaic (PV) devices, the maximum achievable power conversion efficiency (PCE) is mainly limited by thermalization and transmission losses, because polychromatic solar irradiation cannot be matched to a single…

We present detailed analysis of the non-Poissonian population of excitons produced by MEG effect in quantum dots on the base of statistic theory of MEG and synergetic approach for chemical reactions. From the analysis we can conclude that a…

Quantum Physics · Physics 2015-05-28 N. N. Turaeva , B. L. Oksengendler , I. Uralov

The MEG II experiment searches for a charged-lepton-flavour-violating $\mu \to e \gamma$ with the target sensitivity of $6 \times 10^{-14}$. A liquid xenon calorimeter with VUV-sensitive photosensors measures photon position, timing, and…

An excitonic insulator phase is expected to arise from the spontaneous formation of electron-hole pairs (excitons) in semiconductors where the exciton binding energy exceeds the size of the electronic band gap. At low temperature, these…

Strongly Correlated Electrons · Physics 2022-09-02 Selene Mor , Marc Herzog , Claude Monney , Julia Stähler
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