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The anions C$_7$N$^-$ and C$_{10}$H$^-$ are the two longest of the linear (C,N)-bearing and (C,H)-bearing chains which have so far been detected in the Interstellar Medium. In order to glean information on their collision-induced rotational…

We present an extensive range of quantum calculations for the state-changing rotational dynamics involving two simple molecular anions which are expected to play some role in evolutionary analysis of chemical networks in the Interstellar…

Chemical Physics · Physics 2020-10-28 Jan Franz , Barry Mant , Lola González-Sánchez , Roland Wester , Franco A. Gianturco

Among all closed-shell species observed in molecular clouds, molecules with C$_{3v}$ symmetry play a crucial role, as their rotational spectroscopy allows them to behave as a gas thermometer. In the interstellar medium, methyl cyanide…

Astrophysics of Galaxies · Physics 2023-09-22 M. Ben Khalifa , P. J. Dagdigian , J. Loreau

Modeling environments that are not in local thermal equilibrium, such as protoplanetary disks or planetary atmospheres, with molecular spectroscopic data from space telescopes requires knowledge of the rate coefficients of rovibrationally…

Atomic Physics · Physics 2023-10-10 Taha Selim , Ad van der Avoird , Gerrit C. Groenenboom

We investigate the relative efficiencies of low-temperature chemical reactions in the Interstellar medium (ISM) with H$^-$ anion reacting in the gas phase with cyanopolyyne neutral molecules, leading to the formation of anionic C$_x$N$^-$…

Chemical Physics · Physics 2018-07-31 F. A. Gianturco , M. Satta , E. Yurtsever , R. Wester

Interstellar aromatic molecules such as polycyclic aromatic hydrocarbons and polycyclic nitrogen and oxygen bearing molecules are thought to be abundant in the interstellar medium. In this class of molecules, benzonitrile ($c$-C$_6$H$_5$CN)…

Astrophysics of Galaxies · Physics 2024-01-19 M. Ben Khalifa , J. Loreau

Modeling of molecular emission from interstellar clouds requires the calculation of rates for excitation by collisions with the most abundant species. The present paper focuses on the calculation of rate coefficients for rotational…

Astrophysics of Galaxies · Physics 2015-05-18 E. Sarrasin , D. Ben Abdallah , M. Wernli , A. Faure , J. Cernicharo , F. Lique

Recent astronomical observations revealed an increasing molecular complexity in the interstellar medium through the detection of a series of large cyclic carbon species. To correctly interpret these detections, a complex analysis is…

Atomic and Molecular Clusters · Physics 2024-06-05 Sándor Demes , Cheikh Tidiane Bop , Malek Ben Khalifa , François Lique

Two different ab initio potential energy surfaces are employed to investigate the efficiency of the rotational excitation channels for the polar molecular ion HeH$^+$ interacting with He atoms. We further use them to investigate the quantum…

Among the numerous molecular systems found in the interstellar medium (ISM), vinyl cyanide is the first identified olephinic nitrile. While it has been observed in various sources, its detection in Sgr B2 is notable as the 2$_{11}$-2$_{12}$…

Astrophysics of Galaxies · Physics 2025-06-23 Karina Sogomonyan , Malek Ben Khalifa , Jérôme Loreau

New calculations for rotational excitation of cyanoacetylene by collisions with hydrogen molecules are performed to include the lowest 38 rotational levels of HC3N and kinetic temperatures to 300 K. Calculations are based on the interaction…

Astrophysics of Galaxies · Physics 2016-06-15 A. Faure , F. Lique , L. Wiesenfeld

Rate coefficients for collisional processes such as rotational and vibrational excitation are essential inputs in many astrophysical models. When rate coefficients are unknown, they are often estimated using known values from other systems.…

Astrophysics of Galaxies · Physics 2015-06-22 Kyle M. Walker , B. H. Yang , P. C. Stancil , N. Balakrishnan , R. C. Forrey

We report new observations of molecular anions with the Yebes 40m and IRAM 30m telescopes toward the cold dense clouds TMC-1 CP, Lupus-1A, L1527, L483, L1495B, and L1544. We detected for the first time C3N- and C5N- in Lupus-1A and C4H- and…

Astrophysics of Galaxies · Physics 2023-09-13 M. Agundez , N. Marcelino , B. Tercero , I. Jimenez-Serra , J. Cernicharo

We report the first identification in space of HC$_3$N$^+$, the simplest member of the family of cyanopolyyne cations. Three rotational transitions with half-integer quantum numbers from $J$=7/2 to 11/2 have been observed with the Yebes 40m…

Astrophysics of Galaxies · Physics 2024-07-03 C. Cabezas , M. Agúndez , Y. Endo , B. Tercero , N. Marcelino , P. de Vicente , J. Cernicharo

Ammonia is one of the most widely observed molecules in space, and many observations are able to resolve the hyperfine structure due to the electric quadrupole moment of the nitrogen nucleus. The observed spectra often display anomalies in…

Astrophysics of Galaxies · Physics 2023-09-06 J. Loreau , A. Faure , F. Lique , S. Demes , P. J. Dagdigian

In light of its ubiquitous presence in the interstellar gas, the chemistry and reactivity of the HCO+ ion requires special attention. The availability of up-to-date collisional data between this ion and the most abundant perturbing species…

Astrophysics of Galaxies · Physics 2022-01-13 F. Tonolo , L. Bizzocchi , M. Melosso , F. Lique , L. Dore , V. Barone , C. Puzzarini

The modelling of emission spectra of molecules seen in interstellar clouds requires the knowledge of collisional rate coefficients. Among the commonly observed species, N$_2$H$^+$ is of particular interest since it was shown to be a good…

Astrophysics of Galaxies · Physics 2015-06-23 François Lique , Fabien Daniel , Laurent Pagani , Nicole Feautrier

We report extensive theoretical calculations on the rotation-inversion excitation of interstellar ammonia (NH3) due to collisions with atomic and molecular hydrogen (both para- and ortho-H2). Close-coupling calculations are performed for…

Chemical Physics · Physics 2018-11-29 N. Bouhafs , C. Rist , F. Daniel , F. Dumouchel , F. Lique , L. Wiesenfeld , A. Faure

Radiative charge exchange collisions between a carbon atom C(${}^3$P) and a helium ion He+, both in their ground state, are investigated theoretically. Detailed quantum chemistry calculations are carried out to obtain potential energy…

Atomic Physics · Physics 2017-01-25 James F. Babb , B. M. McLaughlin

Cyanopolyynes are among the largest and most commonly observed interstellar Complex Organic Molecules in star-forming regions. They are believed to form primarily in the gas-phase, but their formation routes are not well understood. We…

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