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An in situ study of deformation, fracture, and fatigue behavior of silicon as a lithium-ion battery electrode material is presented. Thin films (100-200 nm) of silicon are cycled in a half-cell configuration with lithium metal foil as…

Lithium ion batteries have been a central part of consumer electronics for decades. More recently, they have also become critical components in the quickly arising technological fields of electric mobility and intermittent renewable energy…

Computational Physics · Physics 2021-11-15 Chiara Panosetti , Simon B. Anniés , Cristina Grosu , Stefan Seidlmayer , Christoph Scheurer

When State of Charge, State of Health, and parameters of the Lithium-ion battery are estimated simultaneously, the estimation accuracy is hard to be ensured due to uncertainties in the estimation process. To improve the estimation…

Systems and Control · Electrical Eng. & Systems 2024-12-20 Ziyou Song , Jun Hou , Xuefeng Li , Xiaogang Wu , Xiaosong Hu , Heath Hofmann , Jing Sun

Lithium-ion battery degradation estimation using fast and noninvasive techniques is a crucial issue in the circular economy framework of this technology. Currently, most of the approaches used to establish the battery-state (i.e., State of…

Signal Processing · Electrical Eng. & Systems 2021-10-28 Simon Montoya-Bedoya , Miguel Bernal , Laura A. Sabogal-Moncada , Hader V. Martinez-Tejada , Esteban Garcia-Tamayo

Battery degradation is governed by complex and randomized cyclic conditions, yet existing modeling and prediction frameworks usually rely on rigid, unchanging protocols that fail to capture real-world dynamics. The stochastic electrical…

Signal Processing · Electrical Eng. & Systems 2025-04-08 Yuqi Li , Han Zhang , Xiaofan Gui , Zhao Chen , Yu Li , Xiwen Chi , Quan Zhou , Shun Zheng , Ziheng Lu , Wei Xu , Jiang Bian , Liquan Chen , Hong Li

With the importance of Li-ion and emerging alternative batteries to our electric future, predicting new sustainable materials, electrolytes and complete cells that safely provide high performance, long life, energy dense capability is…

Materials Science · Physics 2022-07-26 Alex Grant , Colm O'Dwyer

Charge transport processes at interfaces which are governed by complex interfacial electronic structure play a crucial role in catalytic reactions, energy storage, photovoltaics, and many biological processes. Here, the first soft X-ray…

To develop a high-density and long-life lithium-ion battery, a technology is needed that allows non-destructive visualization of the spatial distribution of deteriorated parts after cycle test. In the present study, we measured the…

Chemical Physics · Physics 2021-05-26 Shogo Suzuki , Hideaki Okada , Kai Yabumoto , Seiju Matsuda , Yuki Mima , Noriaki Kimura , Kenjiro Kimura

Silicon suboxide is currently considered as a unique candidate for lithium ion batteries anode materials due to its considerable capacity. However, no adequate information exist about the role of oxygen content on its performance. To this…

Materials Science · Physics 2017-03-28 Obaidur Rahaman , Bohayra Mortazavi , Timon Rabczuk

We present a coupled continuum formulation for the electrostatic, chemical, thermal, mechanical and fluid physics in battery materials. Our treatment is at the particle scale, at which the active particles held together by carbon-binders,…

Computational Physics · Physics 2018-07-26 Zhenlin Wang , Krishna Garikipati

Photoelectrochemical impedance spectroscopy (PEIS) is a useful tool for the characterization of photoelectrodes for solar water splitting. However, the analysis of PEIS spectra often involves a priori assumptions that might bias the…

Chemical Physics · Physics 2020-12-10 Dino Klotz , Daniel A. Grave , Hen Dotan , Avner Rothschild

Electrochemical impedance spectroscopy (EIS) is an effective method for studying the electrochemical systems. The interpretation of EIS is the biggest challenge in this technology, which requires reasonable modeling. However, the modeling…

Data Analysis, Statistics and Probability · Physics 2019-07-04 Shan Zhu , Xinyang Sun , Yuxuan Wang , Naiqin Zhao , Junwei Sha

Lithium-ion batteries have found their way into myriad sectors of industry to drive electrification, decarbonization, and sustainability. A crucial aspect in ensuring their safe and optimal performance is monitoring their energy levels. In…

Systems and Control · Electrical Eng. & Systems 2025-01-13 Hao Tu , Manashita Borah , Scott Moura , Yebin Wang , Huazhen Fang

X-ray photoelectron diffraction is a powerful tool for determining the structure of clean and adsorbate-covered surfaces. Extending the technique into the ultrafast time domain will open the door to studies as diverse as the direct…

Electrochemical degradation of solid electrolytes is a major roadblock in the development of solid-state batteries, and the formed solid-solid interphase (SSI) plays a key role in the performance of solid-state batteries. In this study, by…

X-ray Computed Tomography (X-ray CT) is a well-known non-destructive imaging technique where contrast originates from the materials' absorption coefficients. Novel battery characterization studies on increasingly challenging samples have…

Photoionization spectra of Se have been studied by step-wise resonance laser ionization. The Rydberg series 4s$^2$4p$^3$($^4$S)np $^3$P$_{0,1,2}$ and 4s$^2$4p$^3$($^4$S)np $^5$P$_{1,2,3}$ were measured via different excitation schemes.…

Atomic Physics · Physics 2021-02-03 R. Li , Y. Liu , M. Mostamand , J. Lassen

We present the electro-thermal characterization of transition-edge sensor (TES) detectors suspended on Si membranes fabricated using a silicon-on-insulator (SOI) wafer. The use of an all-silicon fabrication platform, in contrast to the more…

Lithium intercalated anatase used in Li-ion batteries has some special features: coexistence of Li-rich and Li-poor phases as well as two possible positions for Li ions in the oxygen tetrahedron. A theoretical description of the compound…

Materials Science · Physics 2009-07-06 O. V. Velychko , I. V. Stasyuk

The morphologies of crystalline lithium peroxide (Li2O2) discharge products in Li-O2 batteries have been shown to exhibit a dependency on subtle variations within the battery cell-operating environment including exposure to ambient air,…

Materials Science · Physics 2016-06-22 Hariharan Katharajan , Kumar Virwani , A. David Erpelding , Jeannette M. Garcia
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