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A new theoretical approach to the description of the attosecond streaking measurements of atomic photoionization is presented. It is a fully quantum mechanical description based on numerical solving of the time-dependent Schroedinger…

Atomic Physics · Physics 2007-05-23 A. K. Kazansky , N. M. Kabachnik

Tunneling plays a central role in the interaction of matter with intense laser pulses, and also in time-resolved measurements on the attosecond timescale. A strong laser field influences the binding potential of an electron in an atom so…

We study the temporal aspects of laser-assisted extreme ultraviolet (XUV) photoionization using attosecond pulses of harmonic radiation. The aim of this paper is to establish the general form of the phase of the relevant transition…

To measure and control the electron motion in atoms and molecules by the strong laser field on the attosecond time scale is one of the research frontiers of atomic and molecular photophysics. It involves many new phenomena and processes and…

Atomic Physics · Physics 2022-03-30 Chao Chen , Jiayin Che , Shang Wang , Guoguo Xin , Yanjun Chen

Attosecond photoemission or photoionization delays are a unique probe of the structure and the electronic dynamics of matter. However, spectral congestion and spatial delocalization of valence electron wave functions set fundamental limits…

Using extreme-ultraviolet attosecond-pulse-trains, we investigate the photoionization dynamics of a Helium atom in the presence of moderately-strong (~10^12 W/cm^2) femtosecond laser pulses. The electronic structure of a laser-dressed atom…

Atomic Physics · Physics 2011-08-02 Niranjan Shivaram , Henry Timmers , Xiao-Min Tong , Arvinder S. Sandhu

Shape resonances in physics and chemistry arise from the spatial confinement of a particle by a potential barrier. In molecular photoionization, these barriers prevent the electron from escaping instantaneously, so that nuclei may move and…

Imaging in real time the complete dynamics of a process as fundamental as photoemission has long been out of reach due to the difficulty of combining attosecond temporal resolution with fine spectral and angular resolutions. Here, we…

Tremendous advances in laser pump-probe techniques open the door for the observation in real time of ultrafast \textit{electronic} processes. Particularly attractive is the visualization of interatomic processes where one can follow the…

Atomic and Molecular Clusters · Physics 2007-05-23 Alexander I. Kuleff , Lorenz S. Cederbaum

Attosecond dynamics in strong-field tunnel ionization are encoded in intricate holographic patterns in the photoelectron momentum distributions (PMDs). These patterns show the interference between two or more superposed quantum electron…

We provide a brief review of how phase space techniques are explored within strong-field and attosecond science. This includes a broad overview of the existing landscape, with focus on strong-field ionisation and rescattering, high-order…

Atomic Physics · Physics 2021-07-28 H. Chomet , C. Figueira de Morisson Faria

Tunneling and over-barrier ionization are the primary processes of strong-field ionization of atoms and molecules. While the dynamics of tunneling ionization have been extensively studied, exploration of over-barrier ionization dynamics has…

Atomic Physics · Physics 2025-09-03 Yongzhe Ma , Qingcao Liu , Hongcheng Ni , Jian Wu

Recently two emerging areas of research, attosecond and nanoscale physics, have started to come together. Attosecond physics deals with phenomena occurring when ultrashort laser pulses, with duration on the femto- and sub-femtosecond time…

Time-resolved investigations of ultrafast electronic and molecular dynamics were not possible until recently. The typical time scale of these processes is in the picosecond to attosecond realm. The tremendous technological progress in…

Atomic Physics · Physics 2013-05-14 Stefan Pabst

Attosecond streaking, as a measurement technique, was originally conceived as a means to characterize attosecond light pulses, which is a good approximation if the relevant transition matrix elements are approximately constant within the…

Atomic Physics · Physics 2015-05-19 Vladislav S. Yakovlev , Justin Gagnon , Nicholas Karpowicz , Ferenc Krausz

Photoionization as a half-scattering process is not instantaneous. Usually, time delays in photoionization are of the order of few tens of attoseconds (1 as = 10$^{-18}$ s). While going from a single atom to a nano-object, one can expect…

Streaking of photoelectrons has long been used for the temporal characterization of attosecond extreme ultraviolet pulses. When the time-resolved photoelectrons originate from a coherent superposition of electronic states, they carry an…

Chemical Physics · Physics 2016-07-27 Markus Kowalewski , Kochise Bennett , Jérémy R. Rouxel , Shaul Mukamel

Photoelectron spectroscopy is a powerful method that provides insight into the quantum mechanical properties of a wide range of systems. The ionized electron wavefunction carries information on the structure of the bound orbital, the ionic…

We report attosecond-scale probing of the laser-induced dynamics in molecules. We apply the method of high-harmonic spectroscopy, where laser-driven recolliding electrons on various trajec- tories record the motion of their parent ion.…

The intermediate domain of strong-field ionization between the tunneling and the multiphoton regimes is investigated using the strong field approximation and the imaginary-time method. An intuitive model for the dynamics is developed which…

Quantum Physics · Physics 2015-06-22 M. Klaiber , K. Z. Hatsagortsyan , C. H. Keitel