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Recently, different experimental methods intended to detect the entangled two-photon absorption (ETPA) phenomenon in a variety of materials have been reported. The present work explores a different approach on which the ETPA process is…

Quantum Physics · Physics 2023-04-26 Freiman Triana-Arango , Gabriel Ramos-Ortiz , Roberto Ramírez-Alarcón

Recently, different experimental methods to investigate the entangled two-photon absorption (ETPA) process in a variety of materials have been reported. The present work reports on a different approach on which the ETPA process is detected…

Quantum Physics · Physics 2022-02-15 Freiman Triana-Arango , Gabriel Ramos-Ortiz , Roberto Ramírez-Alarcón

Nonlinear spectroscopy and microscopy techniques are ubiquitous in a wide range of applications across physics and biology. However, these usually rely on high-powered pulsed laser systems. A promising alternative is to exploit entangled…

Entangled two-photon absorption (ETPA) has recently become a topic of lively debate, mainly due to the apparent inconsistencies in the experimentally-reported ETPA cross sections of organic molecules. In this work, we provide a thorough…

The phenomenon of Entangled Two-Photon Absorption (ETPA) presents a persistent controversy in the literature, evidenced by a wide disparity in the reported values for the $\sigma_E$ cross-sections. Much of this discrepancy is attributed to…

Quantum Physics · Physics 2025-12-02 Pablo Yepiz-Graciano , Gabriel Ramos-Ortiz , Roberto Ramírez-Alarcón

Recent investigations suggest that the use of non-classical states of light, such as entangled photon pairs, may open new and exciting avenues in experimental two-photon absorption spectroscopy. Despite several experimental studies of…

Over the last 50 years entangled photon pairs have received attention for use in lowering the flux in two-photon absorption imaging and spectroscopy. Despite this, evidence for entangled two-photon absorption (ETPA) effects remain highly…

We introduce a method for determining the sensitivity of any given Entangled Two-Photon Absorption (ETPA) measurement. By modeling all signal and noise contributions to the measurement, we derive a single numerical value that describes the…

Quantum Physics · Physics 2025-12-23 René Pollmann , Franz Roeder , Christine Silberhorn , Benjamin Brecht

Entangled two-photon absorption (ETPA) may be a viable technique to continuously drive an excited state population in plasma for high-bandwidth spectroscopy measurements of localized plasma turbulence or impurity density. Classical…

Entangled two-photon absorption (eTPA) has been recognized as a potentially powerful tool for the implementation of ultra-sensitive spectroscopy. Unfortunately, there exists a general agreement in the quantum optics community that…

Quantum Physics · Physics 2025-01-31 Áulide Martínez-Tapia , Roberto de J. León-Montiel

Entangled two-photon absorption (ETPA) could form the basis of nonlinear quantum spectroscopy at very low photon fluxes, since, at sufficiently low photon fluxes, ETPA scales linearly with the photon flux. When different pairs start to…

Quantum Physics · Physics 2023-12-04 Frank Schlawin

While two-photon absorption (TPA) and other forms of nonlinear interactions of molecules with isolated time-frequency-entangled photon pairs (EPP) have been predicted to display a variety of fascinating effects, their potential use in…

It has been proposed that entangled two-photon absorption (E2PA) can be observed with up to 10 orders of magnitude lower photon flux than its classical counterpart. However, there is a significant controversy regarding the magnitude of this…

When a low flux of time-frequency-entangled photon pairs (EPP) illuminates a two-photon transition, the rate of two-photon absorption (TPA) can be enhanced considerably by the quantum nature of photon number correlations and frequency…

Two-photon absorption (TPA) and other nonlinear interactions of molecules with time-frequency-entangled photon pairs (EPP) has been predicted to display a variety of fascinating effects. Therefore, their potential use in practical…

Quantum Physics · Physics 2021-09-15 Michael G. Raymer , Tiemo Landes , Andrew H. Marcus

Entangled two-photon absorption spectroscopy (TPA) has been widely recognized as a powerful tool for revealing relevant information about the structure of complex molecular systems. However, to date, the experimental implementation of this…

Quantum Physics · Physics 2019-07-10 Roberto de J. León-Montiel , Jiří Svozilík , Juan P. Torres , Alfred B. U'Ren

We demonstrate how the Hong-Ou-Mandel (HOM) interference with polarization-entangled photons can be used to probe ultrafast dephasing. We can infer the optical properties like the real and imaginary parts of the complex susceptibility of…

The phenomena of subthreshold photoemission and absorption under coherent and entangled-photon-pair illumination are reviewed, and the generation and properties of entangled-photon pairs are surveyed. Three prominent forms of subthreshold…

Quantum Physics · Physics 2026-05-05 Malvin Carl Teich , Mark C. Booth , Francesco Lissandrin , Bahaa E. A. Saleh

Hong-Ou-Mandel (HOM) effect was long believed to be a two-photon interference phenomenon. It describes the fact that two indistinguishable photons mixed at a beam splitter will bunch together to one of the two output modes. Considering the…

Quantum Physics · Physics 2018-06-13 Li-Kai Yang , Han Cai , Tao Peng , Da-Wei Wang

In recent works we have explored a multi-photon extension of the celebrated two-photon Hong-Ou-Mandel (HOM) effect in which the quantum amplitudes for a two-photon input to a lossless, balanced 50:50 beamsplitter (BS) undergoes complete…

Quantum Physics · Physics 2025-01-10 Paul M. Alsing , Richard J. Birrittella
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