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IV-VI semiconductor SnSe has been known as the material with record high thermoelectric performance.The multiple close-to-degenerate valence bands in the electronic band structure has been one of the key factors contributing to the high…

A single crystal monolith of La0.9Sr0.1FeO3 and thin pulsed laser deposited film of La0.8Sr0.2Fe0.8Ni0.2O3 were subject to angle integrated valence band photoemission spectroscopy in ultra high vacuum and conductivity experiments in ambient…

Strongly Correlated Electrons · Physics 2011-06-07 A. Braun , B. S. Mun , Y. Sun , Z. Liu , R. Mäder , S. Erat , X. Zhang , S. S. Mao , E. Pomjakushina , K. Conder , L. J. Gauckler , T. Graule

Many properties of layered materials change as they are thinned from their bulk forms down to single layers, with examples including indirect-to-direct band gap transition in 2H semiconducting transition metal dichalcogenides as well as…

We investigate the electronic structure of CaFe$_2$As$_2$ using high resolution photoemission spectroscopy. Experimental results exhibit three energy bands crossing the Fermi level making hole pockets around the $\Gamma$-point. Temperature…

Superconductivity · Physics 2014-04-03 G. Adhikary , D. Biswas , N. Sahadev , R. Bindu , N. Kumar , S. K. Dhar , A. Thamizhavel , K. Maiti

The interaction between localized f and itinerant conduction electrons is crucial in the electronic properties of heavy fermion and valence fluctuating compounds. Using high-resolution angle-resolved photoemission spectroscopy, we…

The temperature-dependent electronic structures of heavy fermion compound CeB$_{6}$ are investigated thoroughly by means of the combination of density functional theory and single-site dynamical mean-field theory. The band structure,…

Strongly Correlated Electrons · Physics 2017-05-03 Haiyan Lu , Li Huang

Photoemission experiments involve the motion of an electron near a conducting surface. This necessarily generates heat by ohmic losses from eddy currents. This inelastic scattering of the electrons will result in a downward shift in…

Strongly Correlated Electrons · Physics 2007-05-23 Robert Haslinger , Robert Joynt

The remarkable properties of (1T-)TiSe$_2$ among the transition metal dichalcogenides have attracted the attention of many researchers due to its peculiar behavior during the charge density wave (CDW) transition. Therefore, it is highly…

Materials Science · Physics 2024-02-08 Shin-ichiro Tanaka , Shigemasa Suga , Keiji Ueno , Keisuke Fukutani , Fumihiko Matsui

We have conducted temperature dependent Angle Resolved Photoemission Spectroscopy (ARPES) study of the electronic structure of n-, p- type PbTe, PbSe and PbS, which are pre- mier thermoelectric materials. Our ARPES measurements on them…

A combined experimental and theoretical study of very-low-energy electron diffraction at the (0001) surface of 2H-NbSe2 is presented. Electron transmission spectra have been measured for energies up to 50 eV above the Fermi level with k||…

Strongly Correlated Electrons · Physics 2009-11-07 E. E. Krasovskii , W. Schattke , V. N. Strocov , R. Claessen

We have conducted temperature dependent Angle Resolved Photoemission Spectroscopy (ARPES) study of the electronic structures of PbTe, PbSe and PbS. Our ARPES data provide direct evidence for the \emph{light} hole upper valence bands (UVBs)…

Strongly Correlated Electrons · Physics 2018-05-10 J. Zhao , C. D. Malliakas , K. Wijayaratne , V. Karlapati , N. Appathurai , D. Y. Chung , S. Rosenkranz , M. G. Kanatzidis , U. Chatterjee

The pressure-dependent relation between Eu valence and lattice structure in model compound EuO is studied with synchrotron-based x-ray spectroscopic and diffraction techniques. Contrary to expectation, a 7% volume collapse at $\approx$ 45…

Strongly Correlated Electrons · Physics 2015-06-04 N. M. Souza-Neto , J. Zhao , E. E. Alp , G. Shen , S. V. Sinogeikin , G. Lapertot , D. Haskel

We report $^{31}$P NMR measurements under various magnetic fields up to 7 T for the intermediate valence compound EuNi$_2$P$_2$, which shows heavy electronic states at low temperatures. In the high-temperature region above 40 K, the Knight…

Complex materials encompassing different phases of matter can display new photoinduced metastable states differing from those attainable under equilibrium conditions. These states can be realized when energy is injected in the material…

Strongly Correlated Electrons · Physics 2024-06-27 Wibke Bronsch , Manuel Tuniz , Denny Puntel , Alessandro Giammarino , Fulvio Parmigiani , Yang-hao Chan , Federico Cilento

An underestimation of the fundamental band gap values by the density functional theory within the local density approximation and associated approaches is a well-known challenge of ab-initio electronic structure computations. Motivated by…

Strongly Correlated Electrons · Physics 2023-08-24 Giuseppe Cuono , Raghottam M. Sattigeri , Carmine Autieri , Tomasz Dietl

We report a photoemission and x-ray absorption study on Au1-xPtxTe2 (x = 0 and 0.35) triangular lattice in which superconductivity is induced by Pt substitution for Au. Au 4f and Te 3d core-level spectra of AuTe2 suggests a valence state of…

The localized-to-itinerant transition of f electrons lies at the heart of heavy-fermion physics, but has only been directly observed in single-layer Ce-based materials. Here, we report a comprehensive study on the electronic structure and…

Strongly Correlated Electrons · Physics 2019-02-18 Q. Yao , D. Kaczorowski , P. Swatek , D. Gnida , C. H. P. Wen , X. H. Niu , R. Peng , H. C. Xu , P. Dudin , S. Kirchner , Q. Y. Chen , D. W. Shen , D. L. Feng

We present a comprehensive study of the photon energy dependence of the valence band photoemission yield in the prototype Mott-Hubbard oxide V2O3. The analysis of our experimental results, covering an extended photon energy range (20-6000…

Our valence band photoelectron spectroscopic studies show a temperature dependent spectral weight transfer near the Fermi level in the Fe-based superconductor FeSe1-xTex. Using theoretical band structure calculations we have shown that the…

Superconductivity · Physics 2015-06-22 P. Mishra , H. Lohani , R. A. Zargar , V. P. S. Awana , B. R. Sekhar

The Kondo model predicts that both the valence at low temperatures and its temperature dependence scale with the characteristic energy T_K of the Kondo interaction. Here, we study the evolution of the 4f occupancy with temperature in a…

Strongly Correlated Electrons · Physics 2018-06-19 K. Kummer , C. Geibel , C. Krellner , G. Zwicknagl , C. Laubschat , N. B. Brookes , D. V. Vyalikh