Related papers: Single molecule superradiance for optical cycling
We investigate superradiance of an ensemble of atoms coupled to an integrated superconducting LC-circuit. Particular attention is paid to the effect of inhomogeneous coupling constants. Combining perturbation theory in the inhomogeneity and…
Collective interaction of light with an atomic gas can give rise to superradiant instabilities. We experimentally study the sudden build-up of a reverse light field in a laser-driven high-finesse ring cavity filled with ultracold thermal or…
We examine the prospects for utilizing the optical bichromatic force (BCF) to greatly enhance laser deceleration and cooling for near-cycling transitions in small molecules. We discuss the expected behavior of the BCF in near-cycling…
Designing closed, laser-induced optical cycling transitions in trapped atoms or molecules is useful for quantum information processing, precision measurement, and quantum sensing. Larger molecules that feature such closed transitions are…
We report the cooling of an atomic ensemble with light, where each atom scatters only a single photon on average. This is a general method that does not require a cycling transition and can be applied to atoms or molecules which are…
We study the scattering properties of optical dipole-mode vector solitons recently predicted theoretically and generated in a laboratory. We demonstrate that such a radially asymmetric composite self-trapped state resembles ``a molecule of…
Molecular design principles provide guidelines for augmenting a molecule with a smaller group of atoms to realize a desired property or function. We demonstrate that these concepts can be used to create an optical cycling center that can be…
Several physical systems can be treated as a scattering process, and, for these processes, a natural observed quantity arises: the ratio between the reflected and incident intensities, known as the reflection coefficient. This dissertation…
Molecular predissociation is the spontaneous, nonradiative bond breaking process that can occur upon excitation. In the context of laser cooling, predissociation is an unwanted consequence of molecular structure that limits the ability to…
We demonstrate a 1D magneto-optical trap of the polar free radical calcium monohydroxide (CaOH). A quasi-closed cycling transition is established to scatter $\sim 10^3$ photons per molecule, predominantly limited by interaction time. This…
We investigate the physics of a gas of ultracold atoms coupled to three single-mode optical cavities and transversely pumped with a laser. Recent work has demonstrated that, for two cavities, the $\mathbb{Z}_{2}$ symmetries of each cavity…
Optical Bloch equations and rate equations serve as powerful tools to model light-matter interactions from textbook-like two-level atoms to the complex internal dynamics of molecules. A particular challenge in this context is posed by…
Cooling of molecules via free-space dissipative scattering of photons is thought not to be practicable due to the inherently large number of Raman loss channels available to molecules and the prohibitive expense of building multiple…
We theoretically investigate the collisions between ultracold polar molecules in the presence of two lasers ensuring a Raman resonant transition on individual molecules to suppress photon scattering, taking the example of bosonic…
Extremely fast rotating molecules carrying significantly more energy in their rotation than in any other degree of freedom are known as "super rotors". It has been speculated that super rotors may exhibit a number of unique properties.…
The majority of molecules proposed for laser cooling and trapping experiments have $\Sigma$-type ground states. Specifically, $^2\Sigma$ states have cycling transitions analogous to D1-lines in alkali-metal atoms while $^1\Sigma$ states…
We report direct laser cooling of a symmetric top molecule, reducing the transverse temperature of a beam of calcium monomethoxide (CaOCH$_3$) to $1.8\pm0.7$ mK while addressing two distinct nuclear spin isomers. These results open a path…
We are proposing to test experimentally the new idea of Enhanced Optical Cooling (EOC) in an electron storage ring. This experiment will confirm new fundamental processes in beam physics and will demonstrate new unique possibilities with…
Compared to purely atomic collisions, ultracold collisions involving molecules have the potential to support a much larger number of Fano-Feshbach resonances due to the huge amount of ro-vibrational states available. In order to handle such…
We create two molecular devices with superconducting junctions, using nickelocene molecules, single Fe atoms, and Pb electrodes at low temperature. We find contrasting behavior based on the coordination of the Fe atom: one device shows…