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The theoretical prediction of the rates of nonradiative processes in molecules is fundamental to assess their emissive properties. In this context, global harmonic models have been widely used to simulate vibronic spectra as well as…

Chemical Physics · Physics 2023-02-01 Michael Wenzel , Roland Mitric

The frozen Gaussian approximation (FGA) is an effective tool for modeling high frequency wave propagation. In previous works, the convergence of the FGA has established for strict hyperbolic systems. In this work, we derive the frozen…

Mathematical Physics · Physics 2019-11-04 James Hateley , Xu Yang

The development of new fluorescent molecules and dyes requires precise determination of their emission efficiency, which ultimately defines the potential of the developed materials. For this, the photoluminescence quantum yield (QY) is…

Instrumentation and Detectors · Physics 2018-07-27 Bart van Dam , Benjamin Bruhn , Gejza Dohnal , Katerina Dohnalova

The importance of considering near-field effects on photon recycling and spontaneous emission in a thermophotovoltaic device is investigated. Fluctuational electrodynamics is used to calculate external luminescence from a photovoltaic cell…

Optics · Physics 2017-08-02 John DeSutter , Rodolphe Vaillon , Mathieu Francoeur

We study a near-field thermophotonic (NF-TPX) refrigerating device, consisting of a lightemitting diode and a photovoltaic cell in close proximity. Calculations are performed in the frame of the detailed-balance approach. We study how…

Applied Physics · Physics 2025-09-26 Thomas Châtelet , Julien Legendre , Olivier Merchiers , Pierre-Olivier Chapuis

The conditions behind the sudden approximation are critically examined. The fuzzy band expression is derived in detail from first principles. We go beyond the sudden approximation to account for both extrinsic losses and interference…

Materials Science · Physics 2007-05-23 L. Hedin , J. D. Lee

Simulating vibrationally resolved electronic spectra of anharmonic systems, especially those involving double-well potential energy surfaces, often requires expensive quantum dynamics methods. Here, we explore the applicability and…

Chemical Physics · Physics 2022-05-12 Tomislav Begušić , Enrico Tapavicza , Jiří Vaníček

For the development and optimization of novel light emitting materials, such as fluorescent proteins, dyes and semiconductor quantum dots (QDs), a reliable and robust analysis of the emission efficiency is crucial. The emission efficiency…

We combine a high-resolution hydro-simulation of the LambdaCDM cosmology with two radiative transfer schemes (for continuum and line radiation) to predict the properties, spectra and spatial distribution of fluorescent Ly-alpha emission at…

Astrophysics · Physics 2009-11-10 Sebastiano Cantalupo , Cristiano Porciani , Simon J. Lilly , Francesco Miniati

Strong-field QED (SFQED) probability rates in the locally monochromatic approximation (LMA) have become an indispensable tool for simulations of processes like gamma-ray emission or electron-positron pair production in laser-particle…

High Energy Physics - Phenomenology · Physics 2025-06-06 Nikita Larin , Daniel Seipt

Advantage is taken of a complete and precise experimental study of the luminescent properties of yttrium aluminium garnet doped with Ce, previously accomplished by other authors, to confirm the accuracy of the invoked theoretical methods…

Materials Science · Physics 2017-04-14 Miguel Lagos , Rodrigo Paredes , César Retamal

A method for performing variable-width (thawed) Gaussian wavepacket (GWP) variational dynamics on machine-learned potentials is presented. Instead of fitting the potential energy surface (PES), the anharmonic correction to the global…

Chemical Physics · Physics 2024-12-17 Rami Gherib , Ilya G. Ryabinkin , Scott N. Genin

The purpose of this work is to generalize the frozen Gaussian approximation (FGA) theory to solve the 3-D elastic wave equation and use it as the forward modeling tool for seismic tomography with high-frequency data. FGA has been previously…

Geophysics · Physics 2018-12-05 James C. Hateley , Lihui Chai , Ping Tong , Xu Yang

Fluorescence recovery after photobleaching (FRAP) measurements offer an important tool for analyzing diffusion and binding processes. Confocal scanning laser microscopes that are used in FRAP experiments bleach regions with a radially…

Subcellular Processes · Quantitative Biology 2009-03-09 George D Tsibidis

We present a computationally efficient framework for predicting the excited-state properties of thermally activated delayed fluorescence (TADF) emitters, integrating extended tight-binding (\xtb), simplified Tamm-Dancoff approximation…

Computing accurate estimates of the Fourier transform of analog signals from discrete data points is important in many fields of science and engineering. The conventional approach of performing the discrete Fourier transform of the data…

Machine Learning · Statistics 2017-12-08 Luca Ambrogioni , Eric Maris

We report high-pressure photoluminescence, Raman scattering, and x-ray diffraction measurements on a lead-free halide perovskite $Cs_3Sb_2Br_9$. At about 3 GPa, an electronic transition manifests itself through a broad minimum in linewidth,…

In this study, the theoretical maximum efficiency $\eta_{max}$ and the Boltzmann-type factor giving the concentration ratio of excited-to-ground state pigment-molecules for photosynthetic systems under irradiation with arbitrary photon flux…

Statistical Mechanics · Physics 2025-12-17 Tetsuo Yabuki

The discrete Fourier transform is approximated by summing over part of the terms with corresponding weights. The approximation reduces significantly the requirement for computer memory storage and enhances the numerical computation…

Strongly Correlated Electrons · Physics 2015-03-19 Xin-Zhong Yan

We present a publicly-available code to generate sets of mock Lyman-$\alpha$ (\lya) forest data that have realistic large-scale correlations including those due to the Baryonic Acoustic Oscillations (BAO). The primary purpose of these mocks…

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