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Time-dependent coupled-cluster method with time-varying orbital functions, called time-dependent optimized coupled- cluster (TD-OCC) method, is formulated for multielectron dynamics in an intense laser field. We have successfully derived…

Chemical Physics · Physics 2018-03-14 Takeshi Sato , Himadri Pathak , Yuki Orimo , Kenichi L. Ishikawa

We discuss possible avenues to study fission dynamics starting from a time-dependent mean-field approach. Previous attempts to study fission dynamics using the time-dependent Hartree-Fock (TDHF) theory are analyzed. We argue that different…

Nuclear Theory · Physics 2015-05-18 A. S. Umar , V. E. Oberacker , J. A. Maruhn , P. -G. Reinhard

We present the fully general time-dependent multiconfiguration self-consistent-field method to describe the dynamics of a system consisting of arbitrary different kinds and numbers of interacting fermions and bosons. The total wave function…

Atomic Physics · Physics 2017-10-11 Ryoji Anzaki , Takeshi Sato , Kenichi L. Ishikawa

The application of methods of time-dependent density functional theory (TDDFT) to systems of qubits provided the interesting possibility of simulating an assigned Hamiltonian evolution by means of an auxiliary Hamiltonian having different…

Quantum Physics · Physics 2012-03-08 Diego de Falco , Dario Tamascelli

We propose a gauge-invariant formulation of the channel orbital-based time-dependent configuration interaction singles (TDCIS) method [Phys. Rev. A 74, 043420 (2006)], one of the powerful ab initio methods to investigate electron dynamics…

Atomic Physics · Physics 2018-02-09 Takeshi Sato , Takuma Teramura , Kenichi L. Ishikawa

The dynamics of a many-body system coupled to an external environment represents a fundamentally important problem. To this class of open quantum systems pertains the study of energy transport and dissipation, dephasing, quantum measurement…

Strongly Correlated Electrons · Physics 2009-11-13 R. D'Agosta , M. Di Ventra

Warm dense matter (WMD) describes an intermediate phase, between condensed matter and classical plasmas, found in natural and man-made systems. In a laboratory setting, WDM needs to be created dynamically. It is typically laser or…

Plasma Physics · Physics 2022-03-14 Alexander J. White , Lee A. Collins , Katarina Nichols , S. X. Hu

The formalism of density functional theory (DFT) can be easily extended to the time dependent case (TDDFT). However, while in the static case the theory is well established and is expected to be, at least in principle, an exact approach for…

Condensed Matter · Physics 2007-05-23 Sandro Stringari

We present an implementation of a time-dependent multiconfiguration self-consistent-field (TD-MCSCF) method [R. Anzaki et al., Phys. Chem. Chem. Phys. 19, 22008 (2017)] with the full configuration interaction expansion for coupled…

Atomic Physics · Physics 2021-10-08 Yang Li , Takeshi Sato , Kenichi L. Ishikawa

We review time-dependent multiconfiguration self-consistent-field (TD-MCSCF) method and time-dependent optimized coupled-cluster (TD-OCC) method for first-principles simulations of high-field phenomena such as tunneling ionization and…

Chemical Physics · Physics 2022-11-21 Takeshi Sato , Himadri Pathak , Yuki Orimo , Kenichi L. Ishikawa

We present the theory, implementation, and benchmarking of a real-time time-dependent density functional theory (RT-TDDFT) module within the RMG code, designed to simulate the electronic response of molecular systems to external…

The time-dependent pair correlation functions for a degenerate ideal quantum gas of charged particles in a uniform magnetic field are studied on the basis of equilibrium statistics. In particular, the influence of a flat hard wall on the…

Condensed Matter · Physics 2018-08-16 L. G. Suttorp

The generator coordinate method (GCM) has been a well-known method to describe nuclear collective motions. In this method, one specifies {\it a priori} the relevant collective degrees of freedom as input of the method, based on empirical…

Nuclear Theory · Physics 2023-11-10 Moemi Matsumoto , Yusuke Tanimura , Kouichi Hagino

We describe an iterative formalism to compute influence functionals that describe the general quantum dynamics of a subsystem beyond the assumption of linear coupling to a quadratic bath. We use a space-time tensor network representation of…

Quantum Physics · Physics 2021-08-24 Erika Ye , Garnet Kin-Lic Chan

We describe the software package FELIX that solves the equations of the time-dependent generator coordinate method (TDGCM) in N-dimensions (N $\geq$ 1) under the Gaussian overlap approximation. The numerical resolution is based on the…

Computational Physics · Physics 2018-02-06 D. Regnier , M. Verrière , N. Dubray , N. Schunck

Optical processes in insulators and semiconductors, including excitonic effects, can be described in principle exactly using time-dependent density-functional theory (TDDFT). Starting from a linearization of the TDDFT semiconductor Bloch…

Materials Science · Physics 2015-05-13 V. Turkowski , C. A. Ullrich

Dynamical observables can often be described by time correlation functions (TCFs). However, efficiently calculating TCFs for complex quantum systems is a significant challenge, which generally requires solving the full dynamics of the…

Chemical Physics · Physics 2025-04-03 Wei Liu , Yu Su , Yao Wang , Wenjie Dou

The linear response approach to nuclear transport has been extended to pair correlations. The latter are treated within a mean field approximation to a pairing interaction with constant matrix elements $G$. The constraint of particle number…

Nuclear Theory · Physics 2009-10-31 F. A. Ivanyuk , H. Hofmann

We present a new application of the Generator Coordinate Method (GCM) as an electronic structure method for strong electron correlation in molecular systems. We identify spin fluctuations as an important generator coordinate responsible for…

Chemical Physics · Physics 2025-03-18 Amir Ayati , Hugh G. A. Burton , Patrick Bultinck , Stijn De Baerdemacker

The cornerstone of time-dependent (TD) density functional theory (DFT), the Runge-Gross theorem, proves a one-to-one correspondence between TD potentials and TD densities of continuum Hamiltonians. In all practical implementations, however,…

Mesoscale and Nanoscale Physics · Physics 2015-05-20 S. Kurth , G. Stefanucci