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Electric force microscopy was used to record the light-dependent impedance spectrum and the probe transient photoconductivity of a film of butylammonium lead iodide, BA$_{2}$PbI$_{4}$, a 2D Ruddlesden--Popper perovskite semiconductor. The…

Mesoscale and Nanoscale Physics · Physics 2020-06-02 Ali Moeed Tirmzi , Ryan P. Dwyer , Fangyuan Jiang , John A. Marohn

Two-dimensional (2D) Ruddlesden-Popper (RP) Metal Halides present unique and tunable properties. However, direct and oriented synthesis is challenging due to low formation energies that lead to rapid, uncontrolled growth during…

The versatile potential of lead halide perovskites and two-dimensional materials is merged in the Ruddlesen-Popper perovskites having outstanding optical properties. Here, the coherent spin dynamics in Ruddlesen-Popper (PEA)$_2$PbI$_4$…

Carrier spins in semiconductor nanocrystals are promising candidates for quantum information processing. Using a combination of time-resolved Faraday rotation and photoluminescence spectroscopies, we demonstrate optical spin polarization…

We have studied the possibly half metallic Co2FeSi full Heusler alloy by means of spin- and time-resolved photoemission spectroscopy. For excitation, the second and fourth harmonic of femtosecond Ti:sapphire lasers were used, with photon…

Materials Science · Physics 2016-08-16 J. -P. Wüstenberg , M. Cinchetti , M. Sánchez Albaneda , M. Bauer , M. Aeschlimann

We study the optically induced spin polarization, spin dephasing and diffusion in several high-mobility two-dimensional electron systems, which are embedded in GaAs quantum wells grown on (110)-oriented substrates. The experimental…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 R. Voelkl , M. Schwemmer , M. Griesbeck , S. A. Tarasenko , D. Schuh , W. Wegscheider , C. Schueller , T. Korn

We report on both experimental and theoretical study of conduction-electron spin polarization dynamics achieved by pulsed optical pumping at room temperature in GaAs(1-x)N(x) alloys with a small nitrogen content (x = 2.1, 2.7, 3.4%). It is…

Materials Science · Physics 2015-06-25 V. K. Kalevich , A. Yu. Shiryaev , E. L. Ivchenko , A. Yu. Egorov , L. Lombez , D. Lagarde , X. Marie , T. Amand

Metal halide perovskites (MHPs) exhibit pronounced spin-orbit coupling (SOC) as a result of their heavy metal constituents, leading to distinctive electronic properties such as Rashba type band splitting which make them promising candidates…

Materials Science · Physics 2025-12-09 Sushovan Sarkar , Koushik Gayen , Ashish Soni , Suman Kalyan Pal

Two dimensional Ruddlesden Popper (2D) RP hybrid perovskites exhibit substantially higher chemical and structural stability than their three dimensional (3D) counterparts, positioning them as promising candidates for next generation…

Owing to their exceptional semiconducting properties, hybrid inorganic-organic perovskites show great promise as photovoltaic absorbers. In these materials, long-range diffusion of charge carriers allows for most of the photogenerated…

Ruddlesden-Popper hybrid halide perovskite are quasi-two-dimensional materials with a layered structure and structural dynamics that are determined by the interplay between the organic and inorganic layers. While their optical properties…

We report an experimental study of the magnetic-field dependence of the optically pumped valley polarization in an epitaxial tungsten diselenide (WSe$_2$) monolayer grown by molecular-beam epitaxy (MBE) on a hexagonal boron nitride (hBN)…

Ultracold polar molecules (UPMs) are emerging as a novel and powerful platform for fundamental applications in quantum science. Here, we report characterization of the coherence between nuclear spin levels of ultracold ground-state…

Atomic Physics · Physics 2022-06-15 Junyu Lin , Junyu He , Mucan Jin , Guanghua Chen , Dajun Wang

Lead halide perovskites have emerged as platforms for exciton-polaritonic studies at room temperature thanks to their excellent photoluminescence efficiency and synthetic versatility. In this work we find proof of strong exciton-photon…

Materials Science · Physics 2024-05-07 Maximilian Black , Mehdi Asadi , Parsa Darman , Finja Schillmöller , Sara Darbari , Nahid Talebi

Layered lead halide A'2An-1PbnI3n+1 perovskites (2D LHPs) are attracting considerable attention as a more stable alternative with respect to APbI3 parent phases - a promising material for a new generation of solar cells. However, a critical…

Materials combining the optoelectronic functionalities of semiconductors with control of the spin degree of freedom are highly sought after for the advancement of quantum technology devices. Here, we report the paramagnetic…

Methylammonium lead triiodine (MAPbI$_3$) is a material representative of the hybrid organic-inorganic lead halide perovskites which attract currently great attention due to their photovoltaic efficiency and bright optoelectronic…

Materials Science · Physics 2022-06-08 E. Kirstein , D. R. Yakovlev , E. A. Zhukov , J. Höcker , V. Dyakonov , M. Bayer

Light-induced sliding ferroelectricity in two-dimensional van der Waals materials enables polarization control via relative layer motion. However, polarization switching occurs on the time scale of shear modes (tens of ps) and requires very…

Materials Science · Physics 2026-05-26 Xiangzhou Zhu , Stefano Mocatti , Matteo Calandra

We address nonradiative recombination pathways by leveraging surface passivation and dislocation management in micron-scale arrays of Ge crystals grown on deeply patterned Si substrates. The time decay photoluminescence (PL) at cryogenic…

We report the first study of the depolarization behavior of spin polarized 3He in a mixture of 3He-4He at a temperature below the 4He Lambda point in a deuterated TetraPhenyl Butadiene-doped deuterated PolyStyrene (dTPB-dPS) coated acrylic…

Atomic Physics · Physics 2008-11-26 Q. Ye , D. Dutta , H. Gao , K. Kramer , X. Qian , X. Zong , L. Hannelius , R. D. McKeown , B. Heyburn , S. Singer , R. Golub , E. Korobkina
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