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Femtosecond optical pump-probe technique is used to study charge carrier dynamics in few-layer MoS2 samples fabricated by mechanical exfoliation. An ultrafast pump pulse excites carriers and differential reflection of a probe pulse tuned to…

Mesoscale and Nanoscale Physics · Physics 2011-11-01 Rui Wang , Brian A. Ruzicka , Nardeep Kumar , Matthew Z. Bellus , Hsin-Ying Chiu , Hui Zhao

The sensitivity of the displacement transducer pumped with a train of high-intensity laser pulses is estimated. Due to the multicomponent character of the pump a consideration of transformations of the signal and the noises between optical…

Optics · Physics 2007-05-23 Victor V. Kulagin

Laser treatment has emerged into a cornerstone of industrial manufacturing. This creates the demand to understand in detail the involved physical processes and their dynamics, to control the process, and to keep guard in-situ the laser…

Optics · Physics 2025-12-16 Jörn Bonse

Pump-probe microscopy is an emerging nonlinear imaging technique based on high repetition rate lasers and fast intensity modulation. Here we present new methods for pump-probe microscopy that keep the beam intensity constant and instead…

Optics · Physics 2021-04-07 Jun Jiang , David Grass , Yue Zhou , Warren S. Warren , Martin C. Fischer

We demonstrate femtosecond pump-probe transient absorption spectroscopy using a programmable dispersive filter as an ultra-fast delay line. Combined with fast synchronous detection this delay line allows for recording of 6 ps decay traces…

Optics · Physics 2018-06-22 Xavier Audier , Naveen Balla , Herve Rigneault

We demonstrate a femtosecond pump-probe spectrometer which utilizes a white light supercontinuum as input, and relies on mutual synchronization of acousto-optical chopper, pump-probe delay stage and the CCD camera to record shot-to-shot…

Chemical Physics · Physics 2022-12-27 Vivek N. Bhat , Asha S. Thomas , Vivek Tiwari

Optical pump-probe spectroscopy is a powerful tool to directly probe the carrier dynamics in materials down to sub-femtosecond resolution. To perform such measurement, while keeping the pump induced perturbation to the sample as small as…

We propose a novel method that uses the oscillation of an atomic excited wave packet observed through a pump-probe technique to accurately determine the zero time delay between a pair of ultrashort laser pulses. This physically-based…

Optics · Physics 2009-11-13 Qun Zhang , John W. Hepburn

We demonstrate pump-probe techniques, namely the Doppler spectrometry and the reflectometry in detail, which directly capture the time-resolved ultrafast evolution of high intensity femtosecond laser-driven hot, dense plasma. These…

A novel polarization-modulation transient method has been developed for studying fast anisotropic relaxation in electronic excited states of polyatomic and biologically relevant molecules under excitation with femtosecond laser pulses. The…

Chemical Physics · Physics 2020-05-12 Ioanna Gorbunova , Nikolay Bezverkhnii , Maxim Sasin , Idris Gagzhiev , Oleg Vasyutinskii

In this paper we describe the technical implementation of pump-probe cathodoluminescence microscopy (PP-CL), a novel technique for studying ultrafast dynamics in materials using combined excitation of electron and laser pulses. The PP-CL…

Instrumentation and Detectors · Physics 2021-12-07 Magdalena Solà-Garcia , Kelly W. Mauser , Nika van Nielen , Toon Coenen , Sophie Meuret , Albert Polman

The classical pump-probe scheme for experiments with femtosecond laser is proposed to use for study the inequality of forward and reversed transitions in optics.

Optics · Physics 2007-05-23 V. A. Kuz'menko

Time-resolved studies have so far relied on rapidly triggering a photo-induced dynamic in chemical or biological ions or molecules and subsequently probing them with a beam of fast moving photons or electrons that crosses the studied…

Chemical Physics · Physics 2021-03-19 Hazem Daoud , R. J. Dwayne Miller

Ultrafast optical pump-probe spectroscopy is a powerful tool to study dynamics in solid materials on femto- and picosecond timescales. In such experiments, a pump pulse induces dynamics inside a sample by impulsive light-matter interaction,…

We present a pump-probe technique for monitoring ultrafast polarizability changes. In particular, we use it to measure the plasma density created at the temporal focus of a self-compressing higher-order pump soliton in gas-filled…

The last decade has witnessed a rapid advancement in laser technology, enabling the direct monitoring and control of electronic motion on its natural attosecond to sub-femtosecond timescales. Ultrafast processes are conventionally studied…

Chemical Physics · Physics 2026-05-27 Torsha Moitra

The dynamics triggered by the impact of an ion onto a solid surface has been explored mainly by theoretical modeling or computer simulation to date. Results indicate that the microscopic non-equilibrium relaxation processes triggered by the…

Atomic Physics · Physics 2023-03-03 L. Kalkhoff , A. Golombek , M. Schleberger , K. Sokolowski-Tinten , A. Wucher , L. Breuer

We present an effective linear response approach to pump-probe femtosecond coherence spectroscopy in the well separated pulse limit. The treatment presented here is based on a displaced and squeezed state representation for the…

Chemical Physics · Physics 2009-11-06 Anand T. N. Kumar , Florin Rosca , Allan Widom , Paul M. Champion

A novel technique for measuring plasma conditions using monochromatic pump-broadband probe laser interactions has been experimentally demonstrated. Originally proposed in [J. Ludwig et al., Phys. Plasmas \textbf{26}, 113108 (2019)], this…

We have measured the evolution of the light intensity of a random laser during a nanosecond pump pulse. Relaxation oscillations in a titania random laser were observed in the time trace of the total emitted intensity. We compare our…

Optics · Physics 2007-05-23 Karen L. van der Molen , Allard P. Mosk , Ad Lagendijk
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