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Exact conditions have long been used to guide the construction of density functional approximations. But hundreds of empirical-based approximations tailored for chemistry are in use, many of which neglect these conditions in their design.…

Chemical Physics · Physics 2023-08-15 Ryan Pederson , Kieron Burke

For materials of varying band gap, we compare energy levels of atomically localized defects calculated within a semilocal and a hybrid density-functional scheme. Since the latter scheme partially relieves the band gap problem, our study…

Materials Science · Physics 2008-07-30 Audrius Alkauskas , Peter Broqvist , Alfredo Pasquarello

Machine learning techniques are utilized to estimate the electronic band gap energy and forecast the band gap category of materials based on experimentally quantifiable properties. The determination of band gap energy is critical for…

Materials Science · Physics 2024-03-11 Sagar Prakash Barad , Sajag Kumar , Subhankar Mishra

We propose an experiment to measure the slow log(N) convergence to mean-field theory (MFT) around a dynamical instability. Using a density matrix formalism, we derive equations of motion which go beyond MFT and provide accurate predictions…

Atomic Physics · Physics 2016-09-08 Amichay Vardi , James R. Anglin

Mean field limits are an important tool in the context of large-scale dynamical systems, in particular, when studying multiagent and interacting particle systems. While the continuous-time theory is well-developed, few works have considered…

Systems and Control · Electrical Eng. & Systems 2023-12-12 Christian Fiedler , Michael Herty , Sebastian Trimpe

Stochastic density functional theory (sDFT) is becoming a valuable tool for studying ground state properties of extended materials. The computational complexity of describing the Kohn-Sham orbitals is replaced by introducing a set of random…

Chemical Physics · Physics 2021-06-16 Ming Chen , Roi Baer , Daniel Neuhauser , Eran Rabani

Machine-learned regression models represent a promising tool to implement accurate and computationally affordable energy-density functionals to solve quantum many-body problems via density functional theory. However, while they can easily…

Computational Physics · Physics 2022-11-08 Emanuele Costa , Giuseppe Scriva , Rosario Fazio , Sebastiano Pilati

The mean-field theory for lossy nonlinear composites, described by complex and field-dependent dielectric functions, is presented. By using the spectral representation of linear composites with identical microstructure, we develop…

Soft Condensed Matter · Physics 2007-05-23 K. W. Yu

Anisotropic patchy particles have become an archetypical statistical model system for associating fluids. Here we formulate an approach to the Kern-Frenkel model via classical density functional theory to describe the positionally and…

Statistical Mechanics · Physics 2024-06-12 Alessandro Simon , Jens Weimar , Georg Martius , Martin Oettel

Accurate approximations to density functionals have recently been obtained via machine learning (ML). By applying ML to a simple function of one variable without any random sampling, we extract the qualitative dependence of errors on…

Computational Physics · Physics 2015-01-29 Kevin Vu , John Snyder , Li Li , Matthias Rupp , Brandon F. Chen , Tarek Khelif , Klaus-Robert Müller , Kieron Burke

A method for beyond-mean-field calculations based on an energy density functional is described. The main idea is to map the energy surface for the nuclear quadrupole deformation, obtained from an energy density functional at the mean-field…

Nuclear Theory · Physics 2022-12-16 J. Ljungberg , J. Boström , B. G. Carlsson , A. Idini , J. Rotureau

In this paper, we study numerical approximations of the ground states in finite temperature density functional theory. We formulate the problem with respect to the density matrices and justify the convergence of the finite dimensional…

Numerical Analysis · Mathematics 2024-05-14 Ge Xu , Huajie Chen , Xingyu Gao

In principle, machine learning (ML) can be used to obtain any electronic property of a many-body system from its electron density within density functional theory. However, some physical quantities are highly sensitive to small variations…

Materials Science · Physics 2026-02-19 L. Arnstein , J. Wetherell , R. Lawrence , P. J. Hasnip , M. J. P. Hodgson

This paper studies a general class of stochastic population processes in which agents interact with one another over a network. Agents update their behaviors in a random and decentralized manner according to a policy that depends only on…

Probability · Mathematics 2023-07-21 Anirudh Sridhar , Soummya Kar

Modern density functional approximations achieve moderate accuracy at low computational cost for many electronic structure calculations. Some background is given relating the gradient expansion of density functional theory to the WKB…

Chemical Physics · Physics 2021-01-27 Kieron Burke

Given a sample $\{X_i\}_{i=1}^n$ from $f_X$, we construct kernel density estimators for $f_Y$, the convolution of $f_X$ with a known error density $f_{\epsilon}$. This problem is known as density estimation with Berkson error and has…

Methodology · Statistics 2014-07-30 James P. Long , Noureddine El Karoui , John A. Rice

We provide a review of recently-develop dynamical mean-field theory (DMFT) approaches to the general problem of strongly correlated electronic systems with disorder. We first describe the standard DMFT approach, which is exact in the limit…

Strongly Correlated Electrons · Physics 2023-02-16 E. Miranda , V. Dobrosavljevic

We review and refine the concept of a mean-field theory for the study of sandpile models, which are of central importance in the study of self-organized criticality. By considering the simple one-dimensional random walker with an absorbing…

Statistical Mechanics · Physics 2007-05-23 Matthew Stapleton , Kim Christensen

Kernel Density Estimation is a very popular technique of approximating a density function from samples. The accuracy is generally well-understood and depends, roughly speaking, on the kernel decay and local smoothness of the true density.…

Statistics Theory · Mathematics 2019-01-03 Maciej Skorski

For algorithms based on interacting particle systems that admit a mean-field description, convergence analysis is often more accessible at the mean-field level. In order to transfer convergence results obtained at the mean-field level to…

Probability · Mathematics 2025-11-03 Nicolai Jurek Gerber , Franca Hoffmann , Urbain Vaes