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Two-photon absorption (TPA) and other nonlinear interactions of molecules with time-frequency-entangled photon pairs (EPP) has been predicted to display a variety of fascinating effects. Therefore, their potential use in practical…

Quantum Physics · Physics 2021-09-15 Michael G. Raymer , Tiemo Landes , Andrew H. Marcus

We experimentally demonstrate two-photon absorption (TPA) with broadband down-converted light (squeezed vacuum). Although incoherent and exhibiting the statistics of a thermal noise, broadband down-converted light can induce TPA with the…

Quantum Physics · Physics 2011-12-06 Barak Dayan , Avi Pe'er , Asher A. Friesem , Yaron Silberberg

Strong-field high-harmonic generation (HHG) is conventionally described semiclassically, with the driving laser treated as a classical field. This approximation becomes insufficient in nanoscale interaction geometries, where extreme spatial…

Quantum Physics · Physics 2026-05-22 Tsendsuren Khurelbaatar , R. T. Sang , Igor Litvinyuk

We introduce sum-frequency generation (SFG) as an effective physical two-photon detector for high power two-mode squeezed coherent states with arbitrary frequency separation, as produced by parametric oscillators well above the threshold.…

Optics · Physics 2013-10-30 Faina Shikerman , Avi Pe'er

We closely replicated and extended a recent experiment ("Spatial properties of entangled two-photon absorption," Phys. Rev. Lett. 129, 183601, 2022) that reportedly observed enhancement of two-photon absorption rates in molecular samples by…

Quantum Physics · Physics 2024-04-26 Tiemo Landes , Brian J. Smith , Michael G. Raymer

The excitation of atomic and molecular systems by propagating light in a two-photon state within the Wigner-Weisskopf approximation has been described using stochastic tools. The problem of a stochastic evolution of the quantum system,…

Quantum Physics · Physics 2025-02-19 Anita Dabrowska , Gniewomir Sarbicki

Photon subtraction is useful to produce nonclassical states of light addressed to applications in photonic quantum technologies. After a very accelerated development, this technique makes possible obtaining either single photons or optical…

Quantum Physics · Physics 2021-09-08 Oscar Rosas-Ortiz , Kevin Zelaya

A novel two-mode non-degenerate squeezed light is generated based on a four-wave mixing (4WM) process driven by two pump fields crossing at a small angle. By exchanging the roles of the pump beams and the probe and conjugate beams, we have…

Quantum Physics · Physics 2020-08-21 Xuan-Jian He , Jun Jia , Gao-Feng Jiao , L. Q. Chen , Weiping Zhang , Chun-Hua Yuan

We experimentally demonstrate sum-frequency generation (SFG) with entangled photon-pairs, generating as many as 40,000 SFG photons per second, visible even to the naked eye. The nonclassical nature of the interaction is exhibited by a…

Quantum Physics · Physics 2007-05-23 Barak Dayan , Avi pe'er , Asher A. Friesem , Yaron Silberberg

Stochastic electrodynamics is a classical theory which assumes that the physical vacuum consists of classical stochastic fields with average energy $\frac{1}{2}\hbar \omega$ in each mode, i.e., the zero-point Planck spectrum. While this…

Quantum Physics · Physics 2017-08-16 Theo M. Nieuwenhuizen , Matthew T. P. Liska

We study fluctuations of the metric in the postquantum theory of classical gravity, a covariant theory which couples a classical spacetime with quantum matter fields. Mathematical consistency requires spacetime to evolve stochastically.…

High Energy Physics - Theory · Physics 2026-05-08 Jonathan Oppenheim , Muhammad Sajjad

Bright squeezed vacuum (BSV) is a non-classical macroscopic state of light, which can be generated through high-gain parametric down-conversion or four-wave mixing. Although BSV is an important tool in quantum optics and has a lot of…

Optical fields provide an accessible platform to explore connections between classical and quantum mechanics. We introduce a group-theoretic framework based on the $\mathrm{su}(1,1)$ Lie algebra to construct classical analogs of…

Optics · Physics 2025-09-17 B. M. Rodríguez-Lara , F. E. Becerra

By means of quantum stochastic calculus we construct a model for an atom with two degenerate levels and stimulated by a laser and we compute its fluorescence spectrum; let us stress that, once the model for the unitary atom-field dynamics…

Quantum Physics · Physics 2009-11-07 Alberto Barchielli , Nicola Pero

We reveal that classical light diffraction in arrays of specially modulated coupled optical waveguides can simulate the quantum process of two-mode squeezing in nonlinear media, with the waveguide mode amplitudes corresponding the signal…

Optics · Physics 2013-05-28 Andrey A. Sukhorukov , Alexander S. Solntsev , John Sipe

A generalisation of Takens' delay-coordinate embedding theorem to stochastic systems, the Stochastic Embedding Sufficiency Theorem, is an inverse methodology enabling non-parametric recovery of both drift and diffusion fields from scalar…

Statistical Mechanics · Physics 2026-05-12 Carolina Garcia , Lucía Perea Durán , Agnese Venezia , Alex Conradie

Motivated by recent experiments, we study four-wave-mixing in an atomic double-{\Lambda} system driven by a far-detuned pump. Using the Heisenberg-Langevin formalism, and based on the microscopic properties of the medium, we calculate the…

Quantum Physics · Physics 2015-05-19 Q. Glorieux , R. Dubessy , S. Guibal , L. Guidoni , J. P. Likforman , T. Coudreau , E. Arimondo

We theoretically investigate the generation of two entangled beams of light in the process of single-pass type-I noncollinear frequency degenerate parametric downconversion with an ultrashort pulsed pump. We find the spatio-temporal…

Quantum Physics · Physics 2021-03-09 L. La Volpe , S. De , M. I. Kolobov , V. Parigi , C. Fabre , N. Treps , D. B. Horoshko

We derive equations for the strongly coupled system of light and dense atomic ensembles. The formalism includes an arbitrary internal level structure for the atoms and is not restricted to weak excitation of atoms by light. In the low light…

Atomic Physics · Physics 2016-06-07 Mark D. Lee , Stewart D. Jenkins , Janne Ruostekoski

Entangled photons offer two advantages for two-photon absorption spectroscopy. One of them, the linear scaling of two-photon absorption rate with the input photon flux, is only valid at very low photon fluxes and is therefore impractical.…

Quantum Physics · Physics 2022-01-26 Paula Cutipa , Maria V. Chekhova