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The computational prediction of atomistic structure is a long-standing problem in physics, chemistry, materials, and biology. Within conventional force-field or {\em ab initio} calculations, structure is determined through energy…

Chemical Physics · Physics 2021-09-15 Dominik Lemm , Guido Falk von Rudorff , O. Anatole von Lilienfeld

Two-dimensional electronic spectroscopy has become one of the main experimental tools for analyzing the dynamics of excitonic energy transfer in large molecular complexes. Simplified theoretical models are usually employed to extract model…

Chemical Physics · Physics 2019-01-17 Mirta Rodríguez , Tobias Kramer

We propose machine learning (ML) models to predict the electron density -- the fundamental unknown of a material's ground state -- across the composition space of concentrated alloys. From this, other physical properties can be inferred,…

We train an equivariant machine learning model to predict energies and forces for a real-world study of hydrogen combustion under conditions of finite temperature and pressure. This challenging case for reactive chemistry illustrates that…

Chemical Physics · Physics 2023-06-16 Xingyi Guan , Joseph Heindel , Taehee Ko , Chao Yang , Teresa Head-Gordon

Serial Femtosecond Crystallography at the X-ray Free Electron Laser (XFEL) sources enabled the imaging of the catalytic intermediates of the oxygen evolution reaction of Photosystem II. However, due to the incoherent transition of the…

Chemical Physics · Physics 2022-01-13 Muhamed Amin

Sparsely annotated semantic segmentation (SASS) aims to train a segmentation network with coarse-grained (i.e., point-, scribble-, and block-wise) supervisions, where only a small proportion of pixels are labeled in each image. In this…

Computer Vision and Pattern Recognition · Computer Science 2022-03-23 Zhiyuan Liang , Tiancai Wang , Xiangyu Zhang , Jian Sun , Jianbing Shen

The near edge structure (XANES) in K-edge X-ray absorption spectroscopy (XAS) is a widely used tool for studying electronic and local structure in materials. The precise interpretation of these spectra with the help of calculations is hence…

Numerical simulations of high energy-density experiments require equation of state (EOS) models that relate a material's thermodynamic state variables -- specifically pressure, volume/density, energy, and temperature. EOS models are…

Data Analysis, Statistics and Probability · Physics 2024-02-26 Himanshu Sharma , Jim A. Gaffney , Dimitrios Tsapetis , Michael D. Shields

To accurately determine the nuclear equation of state (EoS) at finite baryon chemical potential ($\mu_B$) remains a challenging yet essential goal in the study of QCD matter under extreme conditions. In this study, we develop a deep…

Nuclear Theory · Physics 2025-01-20 Fu-Peng Li , Long-Gang Pang , Guang-You Qin

Superconducting transition-edge sensors (TESs) carried by X-ray telescopes are powerful tools for the study of neutron stars and black holes. Several methods, such as optimal filtering or principal component analysis, have already been…

Instrumentation and Methods for Astrophysics · Physics 2021-04-12 Paul Ripoche , Jeremy Heyl

Precisely determining the oxidation states of metal cations within variable-valence transition metal oxides remains a significant challenge, yet it is crucial for understanding and predicting the properties of these technologically…

Materials Science · Physics 2024-09-25 Hao Chen , Yun Liu , Hexin Zhang , Shengdi Zhao , Slavomir Nemsak , Haishan Liu , Miquel Salmeron

The design of high-entropy alloys (HEA) with desired properties is challenging due to their large compositional space. While various machine learning (ML) models can predict specific HEA solid-solution phases (SS), predicting high-entropy…

Materials Science · Physics 2023-06-27 Jie Qi , Diego Ibarra Hoyos , S. Joseph Poon

In this study, we explore the potential of machine learning for modeling molecular electronic spectral intensities as a continuous function in a given wavelength range. Since presently available chemical space datasets provide excitation…

Chemical Physics · Physics 2022-08-02 Prakriti Kayastha , Sabyasachi Chakraborty , Raghunathan Ramakrishnan

Analytical electron microscopy and spectroscopy of biological specimens, polymers, and other beam sensitive materials has been a challenging area due to irradiation damage. There is a pressing need to develop novel imaging and spectroscopic…

Machine Learning · Computer Science 2017-07-14 Yan Zhang , G. M. Dilshan Godaliyadda , Nicola Ferrier , Emine B. Gulsoy , Charles A. Bouman , Charudatta Phatak

Wildfires present intricate challenges for prediction, necessitating the use of sophisticated machine learning techniques for effective modeling\cite{jain2020review}. In our research, we conducted a thorough assessment of various machine…

Machine Learning · Computer Science 2024-04-03 Di Fan , Ayan Biswas , James Paul Ahrens

Resonant X-ray scattering (RXS) is a spectroscopy where both the power of site selective diffraction and the power of local absorption spectroscopy regarding atomic species are combined. By virtue of the dependence on the core level state…

Materials Science · Physics 2007-11-12 Yves Joly , Elena S. Nazarenko , José-Emilio Lorenzo , Sergio Di Matteo , Calogero R. Natoli

The real-space Green's function code FEFF has been extensively developed and used for calculations of x-ray and related spectra, including x-ray absorption (XAS), x-ray emission (XES), inelastic x-ray scattering, and electron energy loss…

Materials Science · Physics 2021-06-28 J. J. Kas , F. D. Vila , J. J. Rehr , C. D. Pemmaraju , T. S. Tan

Fast electrons spectromicroscopies enable to measure quantitatively the optical response of excitations with unrivaled spatial resolution. However, due to their inherently scalar nature, electron waves cannot access to polarization-related…

Optics · Physics 2021-05-26 Hugo Lourenço-Martins , Davy Gérard , Mathieu Kociak

We study theoretically resonant inelastic x-ray scattering (RIXS) at the Cu $L_3$-edge in a typical parent compound of high-$T_c$ cuprate superconductors La$_2$CuO$_4$ on the basis of a detailed electronic band structure. We construct a…

Strongly Correlated Electrons · Physics 2015-08-20 Takuji Nomura

This article examines the problem of Lithium-Sulfur (Li-S) battery state estimation. Such estimation is important for the online management of this energy-dense chemistry. The literature uses equivalent circuit models (ECMs) for Li-S state…

Systems and Control · Electrical Eng. & Systems 2021-02-17 Chu Xu , Timothy Cleary , Daiwei Wang , Guoxing Li , Christopher Rahn , Donghai Wang , Rajesh Rajamani , Hosam K. Fathy