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We study spin dynamics of ordered phases of Cs2CoBr4 in a magnetic field using electron spin resonance (ESR) technique and theoretical analysis. This material hosts weakly interacting distorted-triangular-lattice planes of spin-3/2 Co(2+)…

Strongly Correlated Electrons · Physics 2023-08-01 T. A. Soldatov , A. I. Smirnov , A. V. Syromyatnikov

We report the observation of a frequency shift and splitting of the electron spin resonance (ESR) mode of the low-dimensional S=1/2 frustrated antiferromagnet Cs2CuCl4 in the spin-correlated state below the Curie-Weiss temperature 4 K but…

Strongly Correlated Electrons · Physics 2015-03-18 K. Yu. Povarov , A. I. Smirnov , O. A. Starykh , S. V. Petrov , A. Ya. Shapiro

We report on high-field electron spin resonance (ESR) studies of magnetic excitations in the spin-1/2 triangular-lattice antiferromagnet Cs$_2$CuBr$_4$. Frequency-field diagrams of ESR excitations are measured for different orientations of…

Using electron-spin-resonance (ESR) technique we investigate the magnetic structure of CuCrO2, quasi-two-dimensional antiferromagnet with weakly distorted triangular lattice. Resonance frequencies and the excitation conditions in CuCrO2 at…

Strongly Correlated Electrons · Physics 2014-01-31 A. M. Vasiliev , L. A. Prozorova , L. E. Svistov , V. Tsurkan , V. Dziom , A. Shuvaev , Anna Pimenov , A. Pimenov

We study spin liquid in the frustrated diamond lattice antiferromagnet CoAl2O4 by means of single crystal neutron scattering in zero and applied magnetic field. The magnetically ordered phase appearing below TN=8 K remains nonconventional…

Magnetic interactions are generally believed to play a key role in mediating electron pairing for superconductivity in iron arsenides; yet their character is only partially understood. Experimentally, the antiferromagnetic (AF) transition…

The spin dynamics and magnetic excitations of the slightly distorted triangular s = 3/2 system alpha-CaCr2O4 are investigated by means of Raman spectroscopy and electron spin resonance (ESR) to elucidate its peculiar magnetic properties.…

The magnetic response of antiferromagnetic CsO2, coming from the p-orbital S=1/2 spins of anionic O2- molecules, is followed by 133Cs nuclear magnetic resonance across the structural phase transition occuring at Ts1=61 K on cooling. Above…

Strongly Correlated Electrons · Physics 2018-04-16 M. Klanjsek , D. Arcon , A. Sans , P. Adler , M. Jansen , C. Felser

Cs2CuCl4 is known to possess a quantum spin liquid phase with antiferromagnetic interaction below 2.8 K. We report the observation of a new metastable magnetic phase of the triangular frustrated quantum spin system Cs2CuCl4 induced by the…

Strongly Correlated Electrons · Physics 2017-12-18 Hyeong-Jin Kim , C. R. S. Haines , C. Liu , Sae Hwan Chun , Kee Hoon Kim , H. T. Yi , Sang-Wook Cheong , Siddharth S. Saxena

Although magnetically ordered at low temperatures, the spin-1/2 triangular antiferromagnet Cs_2CuCl_4 exhibits remarkable spin dynamics that strongly suggest proximity to a spin liquid phase. Here we address the question of whether a…

Strongly Correlated Electrons · Physics 2013-05-29 Jason Alicea , Matthew P. A. Fisher

Spin-orbit entangled magnetic dipoles, often referred to as pseudospins, provide a new avenue to explore novel magnetism inconceivable in the weak spin-orbit coupling limit, but the nature of their low-energy interactions remains to be…

Using magnetic neutron scattering we characterize an unusual low temperature phase in orthorhombic SrCuO2. The material contains zigzag spin ladders formed by pairs of S=1/2 chains (J=180 meV) coupled through a weak frustrated interaction…

Materials Science · Physics 2009-10-31 I. A. Zaliznyak , C. Broholm , M. Kibune , M. Nohara , H. Takagi

Motivated by a recent experiment on Cs2CuCl4, we study the spin dynamics of the spin-liquid phase of the spin-1/2 frustrated Heisenberg antiferromagnet on the anisotropic triangular lattice. There have been two different proposals for the…

Strongly Correlated Electrons · Physics 2009-11-10 Chung-Hou Chung , Klaus Voelker , Yong Baek Kim

We compare theoretical results for electron spin resonance (ESR) properties of the Heisenberg-Ising Hamiltonian with ESR experiments on the quasi-one-dimensional magnet Cu(py)$_2$Br$_2$ (CPB). Our measurements were performed over a wide…

We report a thorough theoretical study of the low temperature phase diagram of Cs_2CuCl_4, a spatially anisotropic spin S=1/2 triangular lattice antiferromagnet, in a magnetic field. Our results, obtained in a quasi-one-dimensional limit in…

Strongly Correlated Electrons · Physics 2015-03-17 Oleg A. Starykh , Hosho Katsura , Leon Balents

The three-dimensional frustrated spin lattice in MgCrGaO4, where Cr3+ ions occupy a pyrochlore-like network, exemplifies a quantum magnet with competing interactions, macroscopic degeneracy, and exotic low-energy excitations. Using…

Strongly Correlated Electrons · Physics 2026-03-17 U. Jena , S. Kundu , Suheon Lee , Q. Faure , F. Damay , S. Rols , Adam Berlie , S. Petit , Kwang-Yong Choi , P. Khuntia

Spin-1/2 Heisenberg antiferromagnetic frustrated spin chain systems display exotic ground states with unconventional excitations and distinct quantum phase transitions as the ratio of next-nearest-neighbor to nearest-neighbor coupling is…

The electron spin resonance (ESR) spectroscopy was employed to investigate the spin dynamics in triangular lattice antiferromagnets CuCr$_{1-x}$Mg$_{x}$O$_2$ with $x =$ 0 and 0.02. All spectra can be well fitted by a single Lorentzian…

Strongly Correlated Electrons · Physics 2012-07-16 Renwen Li , Zhe Qu , Wei Tong , Yuheng Zhang

Using neutron powder diffraction and Monte-Carlo simulations we show that a spin-liquid regime emerges at $all compositions in the diamond-lattice antiferromagnets Co(Al1-xCox)2O4. This spin-liquid regime induced by frustration due to the…

Strongly Correlated Electrons · Physics 2015-05-13 O. Zaharko , A. Cervellino , V. Tsurkan , N. B. Christensen , A. Loidl

We report low temperature electron spin resonance experimental and theoretical studies of an archetype $S=1/2$ strong-rung spin ladder material (C$_{5}$H$_{12}$N)$_{2}$CuBr$_{4}$. Unexpected dynamics is detected deep in the…

Strongly Correlated Electrons · Physics 2020-07-21 Yu. V. Krasnikova , S. C. Furuya , V. N. Glazkov , K. Yu. Povarov , D. Blosser , A. Zheludev
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