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Molecular nanowires in which a single molecule bonds chemically to two metal electrodes and forms a stable electrically conducting bridge between them have been studied intensively for more than a decade. However the experimental…

Chemical Physics · Physics 2012-08-21 Firuz Demir , George Kirczenow

Quantum reflection is a pure wave phenomena that predicts reflection of a particle at a changing potential for cases where complete transmission occurs classically. For a chemical bond, we find that this effect can lead to non-classical…

The hydrogen molecule contains the basic ingredients to understand the chemical bond, i.e, a pair of electrons. We show a step to understand The Correspondence Principle for chaotic system in the Chemical World. The hydrogen molecule is…

Chaotic Dynamics · Physics 2007-05-23 A. Lopez-Castillo

The lowest-lying states of LiH have been widely used to develop and calibrate many different methods in quantum mechanics. In this paper we show that the electron-transfer processes occurring in these two states are a difficult test for…

Metallization and dissociation are key transformations in diatomic molecules at high densities particularly significant for modeling giant planets. Using X-ray absorption spectroscopy and atomistic modeling, we demonstrate that in halogens,…

The metal-insulator transition (MIT) of VO2 is discussed with particular emphasis on the structural instability of the rutile compounds toward dimerization. Ti substitution experiments reveal that the MIT is robust up to 20% Ti…

Strongly Correlated Electrons · Physics 2022-02-01 Zenji Hiroi

Trions are a three-particle bound state of electrons and holes. Experimental realization of a trion liquid in the degenerate quantum limit would open a wide range of phenomena in quantum many-body physics. However, trions have been observed…

Mesoscale and Nanoscale Physics · Physics 2023-12-21 Phuong X. Nguyen , Raghav Chaturvedi , Liguo Ma , Patrick Knuppel , Kenji Watanabe , Takashi Taniguchi , Kin Fai Mak , Jie Shan

Conjugated polymers are soft, one-dimensional conductors that admit complex interactions between their polymeric, conformational degrees of freedom and their electronic ones. The presence of extended electronic states along their backbone…

Soft Condensed Matter · Physics 2011-07-29 Jeremy D. Schmit , Alex J. Levine

We study electron transport through single-molecule junctions formed by an octanethiol molecule bonded with the thiol anchoring group to a gold electrode and the opposing methyl endgroup to a carbon tip. Using the scanning tunneling…

We measure and theoretically determine the effect of molecular rotational splitting on Zeeman relaxation rates in collisions of cold Triplet-Sigma molecules with helium atoms in a magnetic field. All four stable isotopomers of the imidogen…

In order to control the dimensionality and the topology of the arrangement of magnetic Ru ions, NaCl-type lithium ruthenates have been investigated. Three types of lithium ruthenates, Li$_{3}$RuO$_{4}$, Li$_{2}$RuO$_{3}$, and…

Materials Science · Physics 2007-05-23 Makoto Soma , Hirohiko Sato

We first argue that the covalent bond and the various closed-shell interactions can be thought of as symmetry broken versions of one and the same interaction, viz., the multi-center bond. We use specially chosen molecular units to show that…

Strongly Correlated Electrons · Physics 2017-06-16 Jon C. Golden , Vinh Ho , Vassiliy Lubchenko

A theoretical study proposes the atomic configuration of electron-beam irradiated C$_{60}$ thin films. We examined the electronic structure and electron-transport properties of the C$_{60}$ clusters using density-functional calculations and…

Materials Science · Physics 2015-05-28 Tomoya Ono , Shigeru Tsukamoto

Ilmenites $AB$O$_3$ provide a platform for electron correlation and magnetism on alternatively stacked honeycomb layers of edge-sharing $A$O$_6$ or $B$O$_6$ octahedra. When $A$ and $B$ are $3d$ transition metals, strong electron correlation…

Strongly Correlated Electrons · Physics 2024-02-12 Seong-Hoon Jang , Yukitoshi Motome

Coulomb interactions can have a decisive effect on the ground state of electronic systems. The simplest system in which interactions can play an interesting role is that of two electrons on a string. In the presence of strong interactions…

Mesoscale and Nanoscale Physics · Physics 2013-10-24 S. Pecker , F. Kuemmeth , A. Secchi , M. Rontani , D. C. Ralph , P. L. McEuen , S. Ilani

Unusual chemical bonds are proposed. Each bond is almost covalent but is characterized by the thread of a small radius $\sim 0.6\times 10^{-11}$cm, between two nuclei in a molecule. The main electron density is concentrated outside the…

Chemical Physics · Physics 2015-01-07 B. Ivlev

Highly conductive molecular junctions were formed by direct binding of benzene molecules between two Pt electrodes. Measurements of conductance, isotopic shift in inelastic spectroscopy and shot noise compared with calculations provide…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 M. Kiguchi , O. Tal , S. Wohlthat , F. Pauly , M. Krieger , D. Djukic , J. C. Cuevas , J. M. van Ruitenbeek

The internal electric field of a Rydberg atom electron can bind a polar molecule to form a giant ultralong-range stable polyatomic molecule. Such molecules not only share their properties with Rydberg atoms, they possess huge permanent…

Atomic Physics · Physics 2015-05-27 Seth T. Rittenhouse , M. Mayle , P. Schmelcher , H. R. Sadeghpour

We show that the dipole-dipole interaction between three identical Rydberg atoms can give rise to bound trimer states. The microscopic origin of these states is fundamentally different from Efimov physics. Two stable trimer configurations…

Atomic Physics · Physics 2018-06-29 Martin Kiffner , Wenhui Li , Dieter Jaksch

We investigate the formation of trimers in an infinite one-dimensional lattice model of hard-core particles with single-particle hopping $t$ and and nearest-neighbour two-body $U$ and three-body $V$ interactions of relevance to Rydberg…

Quantum Physics · Physics 2021-01-12 Arthur Christianen , John Sous