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Solar water splitting has attracted much attention as a clean and renewable route to produce hydrogen fuel. Since the oxygen evolution half-reaction (OER) requires high overpotentials, much research has focused on finding catalyst materials…

Materials Science · Physics 2019-06-03 Maria Bouri , Ulrich Aschauer

We report a theoretical study on resonant x-ray emission spectra (RXES) in the whole energy region of the Mn $L_{2,3}$ white lines for three prototypical Mn/Ag(001) systems: (i) a Mn impurity in Ag, (ii) an adsorbed Mn monolayer on Ag, and…

Strongly Correlated Electrons · Physics 2016-08-31 M. Taguchi , P. Kruger , J. C. Parlebas , A. Kotani

Two-dimensional (2D) materials offer a valuable platform for manipulating and studying chemical reactions at atomic level, owing to the ease of controlling their microscopic structure at the nanometer scale. While extensive research has…

This work reports the synthesis, the physicochemical characterization and the electrochemical studies of new electrocatalysts (ECs) for the oxygen reduction reaction (ORR) that: (i) are based on a hierarchical graphene-based support; and…

This study presents a novel approach for the degradation of tetracycline (TC) in pig manure wastewater using magnet-ite-based magnetic nanofibers (MNFs) as heterogeneous Fenton-like catalysts. The MNFs, composed of polyacrylonitrile (PAN)…

Resonant soft x-ray diffraction has been used to probe the temperature dependent orbital and magnetic structure of $\mathrm{LaSr_{2}Mn_{2}O_7}$. Previous crystallographic studies have shown that this material has almost no MnO$_{6}$ oxygen…

Strongly Correlated Electrons · Physics 2007-05-23 S. B. Wilkins , N. Stojic , T. A. W. Beale , N. Binggeli , P. Bencok , S. Stanescu , J. F. Mitchell , P. Abbamonte , P. D. Hatton , M. Altarelli

The spinel-structured lithium manganese oxide (LiMn$_2$O$_4$) is a material currently used as cathode for secondary lithium-ion batteries, but whose properties are not yet fully understood. Here, we report a computational investigation of…

Materials Science · Physics 2018-03-14 David Santos-Carballal , Phuti E. Ngoepe , Nora H. de Leeuw

LiMn2O4 (LMO), cathodes present large stability when cycled in aqueous electrolytes, contrasting its behavior in conventional organic electrolytes in Lithium-ion batteries (LIBs). To elucidate the mechanisms underlying this distinctive…

Atomically thin van der Waals magnetic materials have not only provided a fertile playground to explore basic physics in the two-dimensional (2D) limit but also created vast opportunities for novel ultrafast functional devices. Here we…

Mesoscale and Nanoscale Physics · Physics 2024-08-20 F. Michael Bartram , Meng Li , Liangyang Liu , Zhiming Xu , Yongchao Wang , Mengqian Che , Hao Li , Yang Wu , Yong Xu , Jinsong Zhang , Shuo Yang , Luyi Yang

We have studied detailed nucleosynthesis in the shocked surface layers of an Oxygen-Neon-Magnesium core collapse supernova with an eye to determining if the conditions are suitable for r process nucleosynthesis. We find no such conditions…

Astrophysics · Physics 2009-11-13 R. D. Hoffman , B. Muller , H. -T. Janka

Double-exchange mechanisms in RE$_{1-x}$AE$_{x}$MnO$_{3}$ manganites (where RE is a trivalent rare-earth ion and AE is a divalent alkali-earth ion) relies on the strong exchange interaction between two Mn$^{3+}$ and Mn$^{4+}$ ions through…

Understanding how light modifies long-range order in quantum materials is key to improving our ability to control functionality. However, this is challenging if the response is heterogeneous. Here we address the most common form of…

Electrocatalytic water splitting, which produces hydrogen and oxygen through water electrolysis, is a promising method for generating renewable, carbon-free alternative fuels. However, its widespread adoption is hindered by the high costs…

Materials Science · Physics 2024-12-23 Kajjana Boonpalit , Nongnuch Artrith

The defect chemistry and thermal oxidation of lanthanide (Ln) incorporated-UO2 are critical for understanding and predicting their behavior as enhanced fuels, mixed oxide (MOX) fuels, spent nuclear fuels (SNF), and particles for safeguard…

The synthesis of new 'Pt-free' electrocatalysts (ECs) for the oxygen reduction reaction (ORR) is reported. The ECs are characterized by a hierarchical 'core-shell' morphology; the 'core' is made of graphene, that is covered by a cratered,…

Transition metal oxides have been extensively studied and utilized as efficient catalysts. However, the strongly correlated behavior which often results in intriguing emergent phenomena in these materials has been mostly overlooked in…

MXenes with versatile chemistry and superior electrical conductivity are prevalent candidate materials for energy storage and catalysts. Inspired by recent experiments of hybridizing MXenes with carbon materials, here we theoretically…

Materials Science · Physics 2018-05-14 Si Zhou , Xiaowei Yang , Wei Pei , Nanshu Liu , Jijun Zhao

Using x-ray and neutron scattering, we have studied the structural and magnetic properties of the single-layer manganite La{1-x}Sr{1+x}MnO4 (0 < x < 0.7). Single crystals were grown by the traveling-solvent floating-zone method at 18 La/Sr…

Strongly Correlated Electrons · Physics 2009-11-10 S. Larochelle , A. Mehta , L. Lu , P. K. Mang , O. P. Vajk , N. Kaneko , J. W. Lynn , L. Zhou , M. Greven

Structural investigation on $Co_{3-x}Mn_xTeO_6$; ($0 \lt x \le 2$) solid solutions as a function of Mn concentration using Synchrotron X-ray diffraction (SXRD) and XANES measurements are presented. Phase diagram obtained from Rietveld…

Materials Science · Physics 2014-04-08 Harishchandra Singh , A. K. Sinha , Haranath Ghosh , M. N. Singh , Parasmani Rajput

Manganese metallocenes larger than the experimentally produced sandwiched MnBz$_2$ compound are studied using several density functional theory methods. First, we show that the lowest energy structures have Mn clusters surrounded by benzene…

Materials Science · Physics 2017-08-02 Tomás Alonso-Lanza , Jhon W. González , Faustino Aguilera- Granja , Andrés Ayuela