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Manganites are technologically important materials, used widely as solid oxide fuel cell cathodes: they have also been shown to exhibit electroresistance. Oxygen bulk diffusion and surface exchange processes are critical for catalytic…

Strongly Correlated Electrons · Physics 2011-10-05 Benjamin Bryant , Christoph Renner , Yusuke Tokunaga , Yoshinori Tokura , Gabriel Aeppli

Manganese(II) mobilised by mining activity poses a persistent water-quality challenge, yet the mechanisms by which low-cost sorbents, such as biochar, sequester Mn(II) remain poorly resolved. This study identifies the specific chemical…

The oxygen evolution reaction (OER) plays an important role in evaluating a photocatalyst and to understand its surface chemistry. In this work we present a comparative study of the OER on the oxide NaTaO$_3$ (113) surface and the…

Materials Science · Physics 2018-10-17 Hassan Ouhbi , Ulrich Aschauer

Currently explored rechargeable aqueous zinc-ion battery (RAZIB) cathode materials, such as $\alpha$-MnO$_{2}$, suffer from severe capacity fade when cycling at rates appropriate for grid-scale operation. Mn dissolution has been previously…

Chemical energy storage is an attractive solution to secure a sustainable energy supply. It requires an electrocatalyst to be implemented efficiently. In order to rationally improve the electrocatalyst materials and thereby the reaction…

Materials Science · Physics 2022-08-01 Marcel Risch , Dulce M. Morales , Javier Villalobos , Denis Antipin

Oxygen reduction catalysts frequently suffer from degradation under harsh operating conditions, and the limited understanding of the underlying mechanisms hampers the development of effective mitigation strategies. In this study, we…

Materials Science · Physics 2025-10-07 Huanhuan Yang , Guangfu Luo

The correlation between ex situ electronic conductivity, oxygen vacancy content, flat-band potential (Efb), and the oxygen evolution reaction (OER) activity for a wide range of perovskite compositions are investigated experimentally and…

Developing cost-effective and high-performance electrodes is critical for advancing hydrogen (H$_2$) production through electrochemical water splitting. In this study, we present a novel electrode design by depositing a $\beta$-MnO$_2$…

NiFe oxyhydroxide is one of the most promising oxygen evolution reaction (OER) catalysts for renewable hydrogen production, and deciphering the identity and reactivity of the oxygen intermediates on its surface is a key challenge but is…

Materials Science · Physics 2020-10-01 Yaming Hao , Yefei Li , Jianxiang Wu , Jinling Wang , Chenglin Jia , Tao Liu , Xuejing Yang , Zhipan Liu , Ming Gong

We report on in-situ resistivity measurements on GaMnAs during post-growth annealing in different atmospheres. A drop in the resistivity is observed when the GaMnAs is exposed to oxygen, which indicates that the passivation of Mn…

Strongly Correlated Electrons · Physics 2009-11-10 M. Malfait , J. Vanacken , W. Van Roy , G. Borghs , V. V. Moshchalkov

Lithium ion batteries often contain transition metal oxides like Li$_{x}$Mn$_2$O$_4$ ($0\leq x\leq2$). Depending on the Li content different ratios of Mn$^\text{III}$ to Mn$^\text{IV}$ ions are present. In combination with electron hopping…

Materials Science · Physics 2022-01-25 Marco Eckhoff , Knut Nikolas Lausch , Peter E. Blöchl , Jörg Behler

Two-dimensional (2D) monolayer pristine MoS$_2$ transition metal dichalcogenide (TMD) is the most studied material because of its promising aspects as nonprecious electrocatalyst for hydrogen evolution reaction (HER). Previous studies have…

Materials Science · Physics 2022-06-22 Joy Ekka , Shrish Nath Upadhyay , Frerich J. Keil , Srimanta Pakhira

The efficiency of $H_2$ production via water electrolysis is typically limited to the sluggish oxygen evolution reaction (OER). As such, significant emphasis has been placed upon improving the rate of OER through the anode catalyst. More…

The development of noble-metal free electrocatalysts is of high importance for clean energy conversion applications. MoS$_2$ has been considered as a promising low cost catalyst for the hydrogen evolution reaction (HER), however its…

The local atomic disorder and the electronic structure in the environment of manganese atoms in LaMnO_3 has been studied by x-ray absorption spectroscopy, over a temperature range (300K to 870K) covering the orbital ordering transition…

Strongly Correlated Electrons · Physics 2009-11-10 Raquel A. Souza , Narcizo M. Souza-Neto , Aline Y. Ramos , Helio C. N. Tolentino , Eduardo Granado

Synchrotron x-ray scattering measurements of the low-temperature structure of the single-layer manganese oxide La$_{1-x}$Sr$_{1+x}$MnO$_4$, over the doping range $0.33 \le x \le 0.67$, indicate the existence of three distinct regions: a…

Strongly Correlated Electrons · Physics 2009-11-07 S. Larochelle , A. Mehta , N. Kaneko , P. K. Mang , A. F. Panchula , L. Zhou , J. Arthur , M. Greven

The process of environmental oxidation is pivotal in determining the physical and chemical properties of two-dimensional (2D) materials. Its impact holds great significance for the practical application of these materials in nanoscale…

Materials Science · Physics 2024-03-20 Soumendra Kumar Das , Lokanath Patra , Prasanjit Samal , Pratap Kumar Sahoo

The lithium manganese oxide spinel Li$_x$Mn$_2$O$_4$, with $0\leq x\leq 2$, is an important example for cathode materials in lithium ion batteries. However, an accurate description of Li$_x$Mn$_2$O$_4$ by first-principles methods like…

Materials Science · Physics 2020-05-20 Marco Eckhoff , Peter E. Blöchl , Jörg Behler

Serial Femtosecond Crystallography at the X-ray Free Electron Laser (XFEL) sources enabled the imaging of the catalytic intermediates of the oxygen evolution reaction of Photosystem II. However, due to the incoherent transition of the…

Chemical Physics · Physics 2022-01-13 Muhamed Amin

This work highlights the potential of earth-abundant mixed-metal oxide catalysts for the acid-based oxygen evolution reaction. These catalysts offer numerous combinations of metal-centre compositions, which can enhance catalytic activity…

Applied Physics · Physics 2023-11-14 Erfan Fatehi , Manish Thadani , Gabriel Birsan , Robert W Black