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Related papers: Solid-State $\rm ^{229}Th$ Nuclear Laser with Two-…

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We present a comprehensive theoretical investigation of hyperfine-resolved excitation and detection of the low-energy isomeric state of $^{229}$Th in trapped $^{229}\mathrm{Th}^{3+}$ ions. Using a quantum master equation approach, we…

Atomic Physics · Physics 2026-05-01 Wu Wang , Ke Zhang , Ke-Mi Xu , Shan-Gui Zhou

We propose a simple approach to measure the energy of the few-eV isomeric state in Th-229. To this end, U-229 nuclei are doped into VUV-transparent crystals, where they undergo alpha decay into Th-229, and, with a probability of 2%,…

Nuclear Experiment · Physics 2016-08-11 Simon Stellmer , Matthias Schreitl , Georgy Kazakov , Johannes Sterba , Thorsten Schumm

In the whole landscape of atomic nuclei, $^{229}$Th is currently the only known nucleus which could allow for the development of a nuclear-based frequency standard, as it possesses an isomeric state of just 7.6 eV energy above the ground…

Instrumentation and Detectors · Physics 2017-11-01 Lars von der Wense , Benedict Seiferle , Mustapha Laatiaoui , Peter G. Thirolf

The most probable candidate for the role of a nuclear optical standard is the 8.338-eV isomer of the 229mTh isotope of the thorium nucleus. Ways of using the resonance properties of the electron shell as an optical resonator to create…

Nuclear Theory · Physics 2023-07-19 F. F. Karpeshin , L. F. Vitushkin

The low-energy isomeric transition in Thorium-229 offers a unique interface between nuclear and atomic physics, presenting a resource for quantum technologies that is notably resilient to environmental decoherence. While early experiments…

Quantum Physics · Physics 2025-08-15 Jingbo Wang , Haixing Miao , Shiqian Ding , Dong E. Liu

The multi-photon excitation to the $8$-eV nuclear isomeric state $^{229\text{m}}$Th in the direct laser-nucleus interaction is investigated theoretically. We solve the time-dependent Schr\"odinger equation with the method which allows us to…

Nuclear Theory · Physics 2025-04-29 Weitao Liu , Yuanbin Wu

With an expected energy of 7.6(5) eV, $^{229}$Th possesses the lowest excited nuclear state in the landscape of all presently known nuclei. The energy corresponds to a wavelength of about 160 nm and would conceptually allow for an optical…

Instrumentation and Detectors · Physics 2017-04-27 Benedict Seiferle , Lars von der Wense , Mustapha Laatiaoui , Peter G. Thirolf

The process of internal conversion from excited electronic states is investigated theoretically for the case of the vacuum-ultraviolet nuclear transition of $^{229}{\mathrm Th}$. Due to the very low transition energy, the $^{229}{\mathrm…

Atomic Physics · Physics 2017-03-22 Pavlo V. Bilous , Georgy A. Kazakov , Iain D. Moore , Thorsten Schumm , Adriana Pálffy

We present a versatile laser system which provides more than 1.5W of narrowband light, tunable in the range from 455-463 nm. It consists of a commercial Titanium-Sapphire laser which is frequency doubled using resonant cavity second…

After nearly fifty years of searching, the vacuum ultraviolet $^{229}$Th nuclear isomeric transition has recently been directly laser excited [1,2] and measured with high spectroscopic precision [3]. Nuclear clocks based on this transition…

$^{229}$Th is the only nucleus currently under investigation for the development of a nuclear optical clock (NOC) of ultra-high accuracy. The insufficient knowledge of the first nuclear excitation energy of $^{229}$Th has so far hindered…

We propose a broadband, femtosecond two-photon excitation scheme for efficient population transfer to the ultra-narrow linewidth $1s2s\ ^1S_0$ metastable state in helium. Using $120$ nm vacuum ultraviolet (VUV) femtosecond laser pulses, we…

Atomic Physics · Physics 2026-01-13 Shashank Kumar , Justin D. Piel , Chris H. Greene , Niranjan Shivaram

Using resonant two-step laser excitation of trapped 232Th+ ions, we observe 43 previously unknown energy levels within the energy range from 7.3 to 8.3 eV. The high density of states promises a strongly enhanced electronic bridge excitation…

Atomic Physics · Physics 2013-08-01 O. A. Herrera-Sancho , N. Nemitz , M. V. Okhapkin , E. Peik

Population of the 8 eV $^{229m}$Th isomer via the second nuclear excited state at 29.19 keV by means of coherent x-ray pulses is investigated theoretically. We focus on two nuclear coherent population transfer schemes using partially…

Nuclear Theory · Physics 2022-07-13 Tobias Kirschbaum , Nikolay Minkov , Adriana Pálffy

The low-lying isomeric state of $^{229}$Th provides unique opportunities for high-resolution laser spectroscopy of the atomic nucleus. We determine the energy of this isomeric state by taking the absolute energy difference between the…

Here, we report the first demonstration of laser-induced conversion electron M\"{o}ssbauer spectroscopy of the $^{229}$Th nuclear isomeric state, which provides the ability to probe the nuclear transition in a material that is opaque to…

We describe a efficient way to photoionize strontium atoms in a linear radio-frequency trap. We use a 2-photon second order process to excite the autoionization resonance (4d2 + 5p2) 1D2. A doubled pulsed Ti:Saphire laser system is used at…

Quantum Physics · Physics 2007-12-04 E. Kirilov , S. Putterman

Experiments on one- and two-photon laser excitation of 232Th+ ions in a radiofrequency ion trap are reported. As the first excitation step, the strongest resonance line at 402 nm from the 6d^2 7s J=3/2 ground state to the 6d7s7p J=5/2 state…

Efficient production of nuclear isomers is critical for pioneering applications, like nuclear clocks, nuclear batteries, clean nuclear energy, and nuclear {\gamma}-ray lasers. However, due to small production cross sections and quick…

A continuous-wave laser source at 148.4 nm based on second-harmonic generation in randomly quasi-phase matched strontium tetraborate, SrB4O7, is demonstrated. It provides (1.3-0.6+0.7) nW of VUV power in a single pass for an incident UV…