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A theory of pump-probe spectroscopy is developed in which optical fields drive two-quantum, Raman-like transitions between ground state sublevels. Three fields are incident on an ensemble of atoms. Two of the fields act as the pump field…

Atomic Physics · Physics 2009-11-06 P. R. Berman , B. Dubetsky

We present three dimensional time-dependent calculations of ionization of arbitrarily spatially oriented H$_2^+$ by attosecond, intense, high-frequency laser fields. The ionization probability shows a strong dependence on both the…

Atomic Physics · Physics 2007-05-23 S. Selsto , M. Forre , J. P. Hansen , L. B. Madsen

The relative population of the fine structure sublevels of an atom's ground state is affected by radiative transitions induced by an anisotropic radiation flux. This causes the alignment of atomic angular momentum. In terms of observational…

Astrophysics · Physics 2008-11-26 Huirong Yan , A. Lazarian

Photonic Integrated Circuits (PIC)s are a promising contender for quantum information technologies. The spectral purity of photons is one of the key attributes of PIC photon-pair sources. The dual-pulse pump manipulation technique [1]…

Quantum Physics · Physics 2024-04-08 Lukas Rodda , Ben M. Burridge , Jorge Barreto , Imad I. Faruque

High-harmonic spectroscopy driven by circularly-polarized laser pulses and their counter-rotating second harmonic is a new branch of attosecond science which currently lacks quantitative interpretations. We extend this technique to the…

Atomic Physics · Physics 2019-09-04 Denitsa Baykusheva , Simon Brennecke , Manfred Lein , Hans Jakob Wörner

SABRE (Signal Amplification by Reversible Exchange) methods provide a simple, fast, and cost-effective method to hyperpolarize a wide variety of molecules in solution, and have been demonstrated with protons and, more recently, with…

Chemical Physics · Physics 2022-02-14 Xiaoqing Li , Jacob R. Lindale , Shannon L. Eriksson , Warren S. Warren

The quantum dynamics of a system of Rb atoms, modeled by a V-type three-level system interacting with intense probe and pump pulses, are studied. The time-delay-dependent transient-absorption spectrum of an intense probe pulse is thus…

Atomic Physics · Physics 2018-02-14 Vadim Becquet , Stefano M. Cavaletto

A novel mechanism of asymmetric frequency conversion is investigated in nonlinear dispersive devices driven parametrically with a biharmonic pump. When the relative phase between the first and second harmonics combined in a two-tone pump is…

Mesoscale and Nanoscale Physics · Physics 2014-12-17 Archana Kamal , Ananda Roy , John Clarke , Michel H. Devoret

The influence of pump coherence on the entanglement produced in spontaneous parametric down-conversion (SPDC) is important to understand, both from a fundamental perspective, and from a practical standpoint for controlled generation of…

Quantum Physics · Physics 2023-04-13 Cheng Li , Boris Braverman , Girish Kulkarni , Robert W. Boyd

This paper presents an overview of the radiative transfer problem of calculating the spectral line intensity and polarization that emerges from a (generally magnetized) astrophysical plasma composed of atoms and molecules whose excitation…

Solar and Stellar Astrophysics · Physics 2015-05-14 J. Trujillo Bueno

Demixing of binary fluids subjected to slow temperature ramps shows repeated waves of nucleation which arise as a consequence of the competition between generation of supersaturation by the temperature ramp and relaxation of supersaturation…

Statistical Mechanics · Physics 2012-10-16 Izabella J. Benczik , Jürgen Vollmer

An ab initio simulation of strong-field photodissociation of diatomic molecules was developed, inspired by recent dissociation experiments of F2-. The transition between electronic states was modeled, including the laser pulse and…

Atomic Physics · Physics 2020-06-26 Bar Ezra , Shimshon Kallush , Ronnie Kosloff

A three-dimensional semiclassical model is used to study double ionization of Ar when driven by a near-infrared and near-single-cycle laser pulse for intensities ranging from 0.85$\times$10$^{14}$ W/cm$^{2}$ to 5$\times$10$^{14}$…

Atomic Physics · Physics 2017-02-15 A. Chen , M. Kübel , B. Bergues , M. F. Kling , A. Emmanouilidou

A narrow elliptic ring containing an electron threaded by a magnetic field B is studied. When the ring is highly flattened, the increase of B would lead to a big energy gap between the ground and excited states, and therefore lead to a…

Other Condensed Matter · Physics 2007-05-23 Shuping Situ , Yanzhang He , Chengguang Bao

Charge collection measurements performed on heavily irradiated p-spray dofz pixel sensors with a grazing angle hadron beam provide a sensitive determination of the electric field within the detectors. The data are compared with a complete…

Exact and asymptotic lineshape expressions are derived from the semi-classical density matrix representation describing a set of closed three-level atomic or molecular states including decoherences, relaxation rates and light-shifts. An…

Atomic Physics · Physics 2012-11-22 Thomas Zanon , Emeric de Clercq , Ennio Arimondo

We report a combined theoretical and experimental study of the spectral and polarization dependence of near resonant radiation coherently backscattered from an ultracold gas of 85Rb atoms. Measurements in an approximately 6 MHz range about…

Quantum Physics · Physics 2009-11-10 D. V. Kupriyanov , I. M. Sokolov , N. V. Larionov , P. Kulatunga , C. I. Sukenik , S. Balik , M. D. Havey

We investigate analytical expressions for the upper and lower bounds for the ionization probability through ultra-intense shortly pulsed laser radiation. We take several different pulse shapes into account, including in particular those…

Quantum Physics · Physics 2009-10-30 C. Figueira de Morisson Faria , A. Fring , R. Schrader

We predict new end-of-pulse behavior in high-field atomic double ionization. Calculations of atomic electron trajectories in short intense laser pulses confirm our analysis of elliptical polarization. We exhibit a four-band structure in ion…

Atomic Physics · Physics 2010-08-20 Xu Wang , J. H. Eberly

Experimental and numerical investigation of single-beam and pump-probe interaction with a resonantly absorbing dense extended medium under strong and weak field-matter coupling is presented. Significant probe beam amplification and conical…