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Despite recent numerical evidence, one of the fundamental theoretical mysteries of polaritonic chemistry is how and if collective strong coupling can induce local changes of the electronic structure to modify chemical properties. Here we…

When the light interacts with matters in a lossy cavity, in the standard cavity quantum electrodynamics, the dissipation of cavity fields is characterized simply by the strengths of the two couplings: the light-matter interaction and the…

Quantum Physics · Physics 2014-02-17 Motoaki Bamba , Tetsuo Ogawa

The standard description of cavity-modified molecular reactions typically involves a single (resonant) mode, while in reality the quantum cavity supports a range of photon modes. Here we demonstrate that as more photon modes are accounted…

Mesoscale and Nanoscale Physics · Physics 2020-07-15 Norah M. Hoffmann , Lionel Lacombe , Angel Rubio , Neepa T. Maitra

Modern research in optical physics has achieved quantum control of strong interactions between a single atom and one photon within the setting of cavity quantum electrodynamics (cQED). However, to move beyond current proof-of-principle…

Quantum Physics · Physics 2011-08-15 D. J. Alton , N. P. Stern , Takao Aoki , H. Lee , E. Ostby , K. J. Vahala , H. J. Kimble

Polaritonic chemistry exploits strong light-matter coupling between molecules and confined electromagnetic field modes to enable new chemical reactivities. In systems displaying this functionality, the choice of the cavity determines both…

Optics · Physics 2022-08-25 Jacopo Fregoni , Francisco J. García-Vidal , Johannes Feist

Circuit quantum electrodynamics allows one to probe, manipulate and couple superconducting quantum bits using cavity photons at an exquisite level. One of its cornerstones is the possibility to achieve the strong coupling which allows one…

Mesoscale and Nanoscale Physics · Physics 2018-10-24 L. E Bruhat , T. Cubaynes , J. J. Viennot , M. C. Dartiailh , M. M. Desjardins , A. Cottet , T. Kontos

We study theoretically the interaction between two photons in a nonlinear cavity. The photons are loaded into the cavity via a method we propose here, in which the input/output coupling of the cavity is effectively controlled via a tunable…

Quantum Physics · Physics 2020-04-29 Mikkel Heuck , Kurt Jacobs , Dirk R. Englund

We present a quantum theory for a fully coupled hybrid optomechanical system where all mutual couplings between a two-level atom, a confined photon mode and a mechanical oscillator mode are considered. In such a configuration, new quantum…

Quantum Physics · Physics 2017-03-01 Juan Restrepo , Ivan Favero , Cristiano Ciuti

Single atoms coupled to a cavity offer unique opportunities as quantum optomechanical devices because of their small mass and strong interaction with light. A particular regime of interest in optomechanics is that of "single-photon strong…

Quantum Physics · Physics 2022-04-01 Javier Argüello-Luengo , Darrick E. Chang

This article reviews theoretical methods developed in the last decade to understand cavity quantum electrodynamics in the ultrastrong-coupling regime, where the strength of the light-matter interaction becomes comparable to the photon…

Quantum Physics · Physics 2020-06-05 Alexandre Le Boité

Cavity quantum electrodynamics (cavity QED) describes the coherent interaction between matter and an electromagnetic field confined within a resonator structure, and is providing a useful platform for developing concepts in quantum…

Polaritonic chemistry offers the possibility of modifying molecular properties and even influencing chemical reactivity through strong coupling between vibrational transitions and confined light modes in optical cavities. Despite…

Chemical Physics · Physics 2025-05-16 Thomas Schnappinger , Markus Kowalewski

The prospect of laser cooling of polyatomic molecules has opened a new avenue in the search for the electric dipole moment of the electron (eEDM). An upper bound on the eEDM would probe new physics arising from beyond the Standard Model of…

Atomic Physics · Physics 2019-06-12 V. S. Prasannaa , N. Shitara , A. Sakurai , M. Abe , B. P. Das

Plasmonic nanocavities enable the confinement of molecules and electromagnetic fields within nano-metric volumes. As a consequence, the molecules experience a remarkably strong interaction with the electromagnetic field, to such an extent…

Chemical Physics · Physics 2021-09-01 Jacopo Fregoni , Tor S. Haugland , Silvio Pipolo , Tommaso Giovannini , Henrik Koch , Stefano Corni

Molecular cavity optomechanical systems, featuring ultrahigh vibrational frequencies and strong light-matter interactions, hold significant promise for advancing applications in quantum science and technology. Specifically, by introducing…

Optics · Physics 2025-12-25 Jian Tang , Baijun Li , Bin Yin , Tian-Xiang Lu , Ran Huang , Franco Nori , Hui Jing

We consider the photoassociation of a low-density gas of quantum-degenerate trapped fermionic atoms into bosonic molecules in a spherically symmetric harmonic potential. For a dilute system and the photoassociation coupling energy small…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Takahiko Miyakawa , Pierre Meystre

We compute the ab-initio electron density beyond the strict Born-Oppenheimer approximation in crystalline LiH and LiD with density functional methods. By taking into account the quantum mechanical nature of the nuclei, an aspect absent in…

Materials Science · Physics 2026-03-13 Ville J. Härkönen

We propose and analyze a scheme for photon trapping in an optical resonator coupled with two-level atoms. We show that when the cavity is excited by two identical light fields from two ends of the cavity respectively, the output light from…

Optics · Physics 2015-08-19 G. S. Agarwal , Yifu Zhu

Achieving strong coupling between light and matter is usually a challenge in Cavity Quantum Electrodynamics (cQED), especially in solid state systems. For this reason is useful taking advantage of alternative approaches to reach this…

Mesoscale and Nanoscale Physics · Physics 2018-03-07 J. E. Ramírez-Muñoz , J. P. Restrepo Cuartas , H. Vinck-Posada

We give a new reduction of a general diatomic molecular Hamiltonian, without modifying it near the collision set of nuclei. The resulting effective Hamiltonian is the sum of a smooth semiclassical pseudodifferential operator (the…

Mathematical Physics · Physics 2015-06-26 André Martinez , Vania Sordoni
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