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We investigate the effect on high-order harmonic generation of the distortion of molecular orbitals by the driving laser field. Calculations for high-order harmonic generation including orbital distortion are performed for N2. Our results…

Atomic Physics · Physics 2015-06-15 Maciej Dominik Śpiewanowski , Adam Etches , Lars Bojer Madsen

We perform a detailed analysis of high-order harmonic generation in diatomic molecules within the strong-field approximation, with emphasis on quantum-interference effects. Specifically, we investigate how the different types of electron…

Atomic Physics · Physics 2011-11-10 C. Figueira de Morisson Faria

We measure spectrally and spatially resolved high-order harmonics generated in argon using chirped multi-cycle laser pulses. Using a stable, high-repetition rate laser we observe detailed interference structures in the far-field. The…

By employing the exact diagonalization method, we investigate the high-harmonic generation (HHG) of the correlated systems under the strong laser irradiation. For the extended Hubbard model on a periodic chain, HHG close to the quantum…

Strongly Correlated Electrons · Physics 2022-03-07 Can Shao , Hantao Lu , Xiao Zhang , Chao Yu , Takami Tohyama , Ruifeng Lu

High-order harmonic generation (HHG) in isolated atoms and molecules has been widely utilized in extreme ultraviolet (XUV) photonics and attosecond pulse metrology. Recently, HHG has also been observed in solids, which could lead to…

Using one-dimensional simulations analyzed through the lens of open quantum systems, we study the photoelectron's strong-field dynamics from an atom surrounded by a scattering environment stochastically structured. We theoretically…

Quantum Physics · Physics 2026-05-21 Simon His , Camille Lévêque , Jérémie Caillat , Richard Taïeb , Jonathan Dubois

We study the high harmonic generation with vortex beams beyond the dipole approximation. To do so we employ the full minimal coupling approach to account for multipolar coupling without truncation and describe the full spatio-temporal…

Atomic Physics · Physics 2026-01-21 Esra Ilke Albar , Valeriia P. Kosheleva , Heiko Appel , Angel Rubio , Franco P. Bonafé

We investigate high-order harmonic spectra from aligned diatomic molecules in intense driving fields whose components have orthogonal polarizations. We focus on how the driving-field ellipticity influences structural interference patterns…

High-harmonic generation (HHG) in crystalline solids have been examined so far on the basis of one-body energy-band structures arising from electron itineracy in a periodic potential. Here, we show emergence of HHG signals which are…

Strongly Correlated Electrons · Physics 2020-04-22 Shohei Imai , Atsushi Ono , Sumio Ishihara

We consider several aspects of high-order harmonic generation in solids: the effects of elastic and inelastic scattering; varying pulse characteristics; and inclusion of material-specific parameters through a realistic band structure. We…

Other Condensed Matter · Physics 2013-02-07 A. F. Kemper , B. Moritz , J. K. Freericks , T. P. Devereaux

Here the role and influence of aberrations in optical imaging systems employing partially coherent complex scalar fields is studied. Imaging systems require aberrations to yield contrast in the output image. For linear shift-invariant…

Optics · Physics 2015-06-30 Mario A. Beltran , Marcus J. Kitchen , T. Petersen , David M. Paganin

The use of structured light to drive highly nonlinear processes in matter not only enables imprinting spatially-resolved properties onto short-wavelength radiation, but also opens alternative avenues for exploring the dynamics of nonlinear…

We present ab initio calculations using the $R$-matrix with time dependence (RMT) method for high-order harmonic generation (HHG) in argon in a short, intense pulse regime. The calculations employ a $6$-cycle $\sin^2$ pulse at $850$ nm with…

Atomic Physics · Physics 2026-04-23 Aaron T. Bondy , Klaus Bartschat

Backscattering of delocalized electrons has been recently established [Phys. Rev. A 105, L041101 (2022)] as a mechanism to enhance high-order harmonic generation (HHG) in periodic systems with broken translational symmetry. Here we study…

Atomic Physics · Physics 2022-07-12 Chuan Yu , Ulf Saalmann , Jan M. Rost

In recent publications, it has been shown that high-order harmonic generation can be manipulated by employing a time-delayed attosecond pulse train superposed to a strong, near-infrared laser field. It is an open question, however, which is…

Atomic Physics · Physics 2009-11-13 C. Figueira de Morisson Faria , P. Salieres

Toroidal vortex is a kind of novel and exotic structured light with potential applications in photonic topology and quantum information. Here, we present the study on high harmonic generation (HHG) from the interaction of the intense…

Optics · Physics 2024-10-10 Zijian Lyu , Yiqi Fang , Yunquan Liu

High-order frequency mixing in graphene using a two-color radiation field consisting of the fundamental and the second harmonic fields of an ultrashort linearly polarized laser pulse is studied. It is shown that the harmonics originated…

Mesoscale and Nanoscale Physics · Physics 2022-05-25 Hamlet K. Avetissian , Garnik F. Mkrtchian , Andreas Knorr

We investigate the high harmonic generation (HHG) in solids driven by laser fields with different ellipticities. The HHG spectra show a two-plateau structure within the energy gap between the valence band and the first conduction band.…

Optics · Physics 2018-06-01 Liang Li , Pengfei Lan , Xiaosong Zhu , Tengfei Huang , Peixiang Lu

We present an experimental technique using orbital angular momentum (OAM) in a fundamental laser field to drive High Harmonic Generation (HHG). The mixing of beams with different OAM allows to generate two laser foci tightly spaced to study…

Chemical Physics · Physics 2019-07-24 Jan Troßand Carlos A. Trallero-Herrero

High-order harmonic generation (HHG) in gases leads to short-pulse extreme ultraviolet (XUV) radiation useful in a number of applications, for example, attosecond science and nanoscale imaging. However, this process depends on many…