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Large-scale density functional theory (DFT) calculations provide a powerful tool to investigate the atomic and electronic structure of materials with complex structures. This article reviews a large-scale DFT calculation method, the…

Materials Science · Physics 2022-08-31 Ayako Nakata , David R. Bowler , Tsuyoshi Miyazaki

Direct air capture (DAC) with solid sorbents such as metal-organic frameworks (MOFs) is a promising approach for negative carbon emissions. Computational materials screening can help identify promising materials from the vast chemical space…

Materials Science · Physics 2025-06-12 Logan M. Brabson , Andrew J. Medford , David S. Sholl

Metal-organic frameworks (MOFs) are an incredibly diverse group of highly porous hybrid materials, which are interesting for a wide range of possible applications. For a reliable description of many of their properties accurate…

Materials Science · Physics 2024-11-26 Sandro Wieser , Egbert Zojer

Software quality assurance activities become increasingly difficult as software systems become more and more complex and continuously grow in size. Moreover, testing becomes even more expensive when dealing with large-scale systems. Thus,…

Software Engineering · Computer Science 2023-10-27 Xhulja Shahini , Domenic Bubel , Andreas Metzger

The enormous structural and chemical diversity of metal-organic frameworks (MOFs) forces researchers to actively use simulation techniques on an equal footing with experiments. MOFs are widely known for outstanding adsorption properties, so…

Materials Science · Physics 2021-11-22 Vadim V. Korolev , Yurii M. Nevolin , Thomas A. Manz , Pavel V. Protsenko

Highly accurate force fields are a mandatory requirement to generate predictive simulations. In this regard, Machine Learning Force Fields (MLFFs) have emerged as a revolutionary approach in computational chemistry and materials science,…

Materials Science · Physics 2025-03-11 Carlos A. Vital , Román J. Armenta-Rico , Huziel E. Sauceda

We investigate Machine-Learned Force Fields (MLFFs) trained on approximate Density Functional Theory (DFT) and Coupled Cluster (CC) level potential energy surfaces for the carbon diamond and lithium hydride solids. We assess the accuracy…

System specific neural force fields (NFFs) have gained popularity in computational chemistry. One of the most popular datasets as a bencharmk to develop NFFs models is the MD17 dataset and its subsequent extension. These datasets comprise…

Machine Learning · Computer Science 2024-03-07 Zihan Pengmei , Junyu Liu , Yinan Shu

Machine Learning (ML) based prognostics and health monitoring (PHM) tools provide new opportunities for manufacturers to operate and maintain their equipment in a risk-optimized manner and utilize it more sustainably along its lifecycle.…

Machine Learning · Computer Science 2024-05-15 Christoph Netsch , Till Schöpe , Benedikt Schindele , Joyam Jayakumar

Machine learning (ML) is increasingly becoming a common tool in computational chemistry. At the same time, the rapid development of ML methods requires a flexible software framework for designing custom workflows. MLatom 3 is a program…

Machine-learned interatomic potentials (MLIPs) and force fields (i.e. interaction laws for atoms and molecules) are typically trained on limited data-sets that cover only a very small section of the full space of possible input structures.…

Numerical Analysis · Mathematics 2022-09-13 Christoph Ortner , Yangshuai Wang

The increased availability of computing time, in recent years, allows for systematic high-throughput studies of material classes with the purpose of both screening for materials with remarkable properties and understanding how structural…

Materials Science · Physics 2023-11-28 Robin Hilgers , Daniel Wortmann , Stefan Blügel

Software fault prediction (SFP) is a critical task in software engineering, enabling early identification of faults in modules to improve software quality and reduce maintenance costs. This research investigates the combined effects of…

Software Engineering · Computer Science 2026-05-19 Ahmad Nauman Ghazi , Nagajyothi Devarapalli , Ashir Javeed , Sadi Alawadi , Fahed Alkhabbas , Khalid AlKharabsheh

Machine learning software, deep neural networks (DNN) software in particular, discerns valuable information from a large dataset, a set of data. Outcomes of such DNN programs are dependent on the quality of both learning programs and…

Machine Learning · Computer Science 2019-11-27 Shin Nakajima

Simulating atomic-scale processes, such as protein dynamics and catalytic reactions, is crucial for advancements in biology, chemistry, and materials science. Machine learning force fields (MLFFs) have emerged as powerful tools that achieve…

Chemical Physics · Physics 2024-12-30 Lars L. Schaaf , Ilyes Batatia , Christoph Brunken , Thomas D. Barrett , Jules Tilly

Machine learning force fields (MLFFs) have emerged as a sophisticated tool for cost-efficient atomistic simulations approaching DFT accuracy, with recent message passing MLFFs able to cover the entire periodic table. We present an invariant…

Present Large Language Models (LLM) self-training methods always under-sample on challenging queries, leading to inadequate learning on difficult problems which limits LLMs' ability. Therefore, this work proposes a difficulty-aware…

Computation and Language · Computer Science 2025-03-13 Boyang Xue , Qi Zhu , Hongru Wang , Rui Wang , Sheng Wang , Hongling Xu , Fei Mi , Yasheng Wang , Lifeng Shang , Qun Liu , Kam-Fai Wong

Fast and accurate molecular force field (FF) parameterization is still an unsolved problem. Accurate FFs are not generally available for all molecules, like novel druglike molecules. While methods based on quantum mechanics (QM) exist to…

Chemical Physics · Physics 2019-08-06 Raimondas Galvelis , Stefan Doerr , Joao M. Damas , Matt J. Harvey , Gianni De Fabritiis

A key challenge in security analysis is the manual evaluation of potential security weaknesses generated by static application security testing (SAST) tools. Numerous false positives (FPs) in these reports reduce the effectiveness of…

Cryptography and Security · Computer Science 2025-07-15 Jonas Wagner , Simon Müller , Christian Näther , Jan-Philipp Steghöfer , Andreas Both

Electronic structure methods offer in principle accurate predictions of molecular properties, however, their applicability is limited by computational costs. Empirical methods are cheaper, but come with inherent approximations and are…

Chemical Physics · Physics 2023-11-16 Moritz Thürlemann , Sereina Riniker