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Under vibrational strong coupling (VSC), the formation of molecular polaritons may significantly modify the photo-induced or thermal properties of molecules. In an effort to understand these intriguing modifications, both experimental and…

Chemical Physics · Physics 2022-04-07 Tao E. Li , Abraham Nitzan , Joseph E. Subotnik

We study the elastic response of a stationarily driven system of a cavity field strongly coupled with molecular excitons, taking into account the main dissipation channels due to the finite cavity linewidth and molecular vibrations. We show…

Quantum Physics · Physics 2021-02-24 Kalle S. U. Kansanen , J. Jussi Toppari , Tero T. Heikkilä

A model describing amplification and quantum statistics of the exciton polaritons with k=0 in a non-resonantly excited semiconductor quantum well embedded in a microcavity is presented. Exploiting the bottleneck effect for exciton…

Other Condensed Matter · Physics 2009-11-11 Paolo Schwendimann , Antonio Quattropani

We develop an approach based on stochastic quantum trajectories for an incoherently pumped system of interacting bosons relaxing their energy in a thermal reservoir. Our approach enables the study of the versatile coherence properties of…

Quantum Gases · Physics 2015-09-17 H. Flayac , I. G. Savenko , M. Möttönen , T. Ala-Nissila

We present a formulation of measurement-based feedback control of a single quantum particle in one spatial dimension. An arbitrary linear combination of the position and momentum of the particle is continuously monitored, and feedback…

Quantum Physics · Physics 2022-12-26 Amy Rouillard , Anirudh Reddy , Humairah Bassa , Shamik Maharaj , Lajos Diosi , Thomas Konrad

We theoretically and experimentally investigate quantum features of an interacting light-matter system from a multidisciplinary perspective, unifying approaches from semiconductor physics, quantum optics, and quantum information science. To…

We report on the study of a polariton gas confined in a quasi-periodic one dimensional cavity, described by a Fibonacci sequence. Imaging the polariton modes both in real and reciprocal space, we observe features characteristic of their…

We present an alternative approach to finite-size effects around the synchronization transition in the standard Kuramoto model. Our main focus lies on the conditions under which a collective oscillatory mode is well defined. For this…

Adaptation and Self-Organizing Systems · Physics 2018-04-04 Franziska Peter , Arkady Pikovsky

Spectral and temporal mode matching are required for the efficient interaction of photons and quantum memories. In our previous work, we proposed a new route to spectrally compress broadband photons to achieve spectral mode matching with…

Quantum Physics · Physics 2022-03-23 Karthik V. Myilswamy , Andrew M. Weiner

We propose a scheme to implement a supersensitive estimation of the coupling strength in a hybrid optomechanical system which consists of a cavity-Bose-Einstein condensate system coupled to an impurity. This method can dramatically improve…

Quantum Physics · Physics 2020-09-22 Qing-Shou Tan , Ji-Bing Yuan , Jie-Qiao Liao , Le-Man Kuang

Recent experimental evidence for collective protein vibrations in the terahertz (THz) domain indicates that energy in biomolecular systems can self-organize in an orderly manner, as anticipated by Fr\"ohlich's theory of condensates within a…

Biological Physics · Physics 2026-03-18 Jordane Preto , Vania Calandrini , Elena Floriani , Gergely Katona , Marco Pettini

It has been experimentally demonstrated that reaction rates for molecules embedded in microfluidic optical cavities are altered when compared to rates observed under "ordinary" reaction conditions. However, precise mechanisms of how strong…

Quantum Physics · Physics 2022-04-22 Eric W. Fischer , Janet Anders , Peter Saalfrank

We introduce a theory of chemical equilibrium in optical microcavities, which allows us to relate equilibrium reaction quotients in different electromagnetic environments. Our theory shows that in planar microcavities under strong coupling…

Chemical Physics · Physics 2023-05-02 Kaihong Sun , Raphael F. Ribeiro

Recent experiments have observed that the chemical and photophysical properties of molecules can be modified inside an optical Fabry-Perot microcavity under collective vibrational strong coupling (VSC) conditions, and such modification is…

Mesoscale and Nanoscale Physics · Physics 2021-03-09 Tao E. Li , Abraham Nitzan , Joseph E. Subotnik

A nonequilibrium statistical operator method is developed for ensembles of particles obeying non-Hamiltonian equations of motion in classical phase space. The main consequences of non-zero compressibility of phase space are examined in…

Statistical Mechanics · Physics 2007-05-23 Alexander V. Zhukov , Jianshu Cao

The energy and wave function of a harmonically confined two-electron system coupled to light is calculated by separating the wave functions of the relative and center of mass (CM) motions. The relative motion wave function has a known…

Mesoscale and Nanoscale Physics · Physics 2021-11-10 Chenhang Huang , Alexander Ahrens , Matthew Beutel , Kalman Varga

In this tutorial-style review we discuss basic concepts of coupled cluster theory and recent developments that increase its computational efficiency for calculations of molecules, solids and materials in general. We will touch upon the…

Materials Science · Physics 2020-04-15 Igor Ying Zhang , Andreas Grüneis

An analytical solution of the Helmholtz equation for electromagnetic field distribution in a resonant cavity with elliptic cross-section is found. We compare the frequencies of the eigenmodes with numerical and experimental values for a…

Classical Physics · Physics 2019-11-22 Mihael S. Grbić

Long-term quantum coherence constitutes one of the main challenges when engineering quantum devices. However, easily accessible means to quantify complex decoherence mechanisms are not readily available, nor are sufficiently stable systems.…

We present a microscopic theory for nonlinear optical spectroscopy of N molecules in an optical cavity. A quantum Langevin analytical expression is derived for the time- and frequency-resolved signals accounting for arbitrary numbers of…

Quantum Physics · Physics 2023-03-29 Zhedong Zhang , Xiaoyu Nie , Dangyuan Lei , Shaul Mukame