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High-harmonic generation (HHG) is a coherent optical process in which the incident photon energy is up-converted to the multiples of its initial energy. In solids, under the influence of a strong laser field, electron-hole (e-h) pairs are…

We present theoretical studies of high-order harmonic generation (HHG) produced by non-homogeneous fields as resulting from the illumination of plasmonic nanostructures with a short laser pulse. We show that both the inhomogeneity of the…

Atomic Physics · Physics 2012-04-27 M. F. Ciappina , J. Biegert , R. Quidant , M. Lewenstein

We propose a real-time time-dependent ab__initio approach within a configuration-interaction-singles ansatz to decompose the high-harmonic generation (HHG) signal of molecules in terms of individual molecular-orbital (MO) contributions.…

Chemical Physics · Physics 2025-12-11 Marco Marchetta , Chiara Morassut , Julien Toulouse , Emanuele Coccia , Eleonora Luppi

High-order harmonic generation (HHG) in gases leads to short-pulse extreme ultraviolet (XUV) radiation useful in a number of applications, for example, attosecond science and nanoscale imaging. However, this process depends on many…

High harmonic generation (HHG) is an extreme nonlinear frequency up-conversion process during which extremely short duration optical pulses at very short wavelengths are emitted. A major concern of HHG is the small conversion efficiency at…

We confirm the existence of a new bulk medium quasiparticle with transverse orbital angular momentum (tOAM) and elucidate its physical origin. The tOAM structure is driven by torques induced by the ponderomotive force of the light in the…

Plasma Physics · Physics 2026-03-17 M. S. Le , S. W. Hancock , N. Tripathi , H. M. Milchberg

Plasmonic vortices (PV) excited by a highly focused radially polarized optical vortex (RPOV) beam on a metal surface are investigated experimentally and theoretically. The proposed method reveals a direct phase singularity and orbital…

Optics · Physics 2011-10-11 X. -C. Yuan , Z. J. Hu , G. H. Yuan , Z. Shen

Recent advancements in ultrafast laser systems and high harmonic generation (HHG) techniques have enabled time-resolved photoemission spectroscopy on femtosecond timescales, opening up unprecedented opportunities to explore quantum…

Strongly Correlated Electrons · Physics 2025-11-03 Takeshi Suzuki , Kozo Okazaki

We use a vortex retarder-based approach to generate few optical cycles light pulses carrying orbital angular momentum (known also as twisted light or optical vortex) from a Yb:KGW oscillator pumping a noncollinear optical parametric…

Spin angular momentum of a photon corresponds to a polarisation degree of freedom of lights, and such that various polarisation properties are coming from macroscopic manifestation of quantum-mechanical properties of lights. An orbital…

Optics · Physics 2024-06-07 Shinichi Saito

The solid-state harmonic generation (SSHG) derives from photocurrent coherence. The crystal symmetry, including point-group symmetry and time-reversal symmetry, constrains the amplitude and phase of the photocurrent, thus manipulates the…

Optics · Physics 2024-01-17 Chen Qian , Shicheng Jiang , Tong Wu , Hongming Weng , Chao Yu , Ruifeng Lu

High-harmonic generation (HHG) in solids has rapidly emerged as a promising platform for creating compact attosecond sources and probing ultrafast electron dynamics. Resonant metasurfaces are essential for enhancement of the otherwise small…

Vector beams with spatially structured polarization and intertwined spin-orbital angular momentum (SAM-OAM) provide powerful degrees of freedom for tailoring light-matter interactions. While such structured beams are well established in the…

The observation of non-perturbative harmonic emission in solids from ultrashort laser pulses [1] sparked a wave of studies [2,3] as a probe of charge carrier dynamics in solids under strong fields and a route to extreme ultraviolet (XUV)…

Parametric oscillation is a fundamental concept that underlies nonlinear wave-matter interactions, leading to generation or amplification of new frequency components. Using a temporal modulation generated by the heterodyne interference of a…

Optics · Physics 2020-01-10 Xuexue Guo , Xingjie Ni

High harmonic generation (HHG) has unleashed the power of strong laser physics in solids. Here we investigate HHG from a large system, solid C$_{60}$, with 240 valence electrons engaging harmonic generation at each crystal momentum, the…

Materials Science · Physics 2020-12-23 G. P. Zhang , Y. H. Bai

In the realm of open quantum systems, steady states and high-harmonic generation (HHG) existing far from equilibrium have become core pillars of ultrafast science. Most solid-state research explores charge HHG with limited investigations…

Strongly Correlated Electrons · Physics 2024-08-20 Negin Moharrami Allafi , Michael H. Kolodrubetz , Marin Bukov , Vadim Oganesyan , Mohsen Yarmohammadi

The generation of coherent light pulses in the extreme ultraviolet (XUV) spectral region with attosecond pulse durations constitutes the foundation of the field of attosecond science. Twenty years after the first demonstration of isolated…

Intense, single-cycle terahertz (THz) pulses offer a promising approach for understanding and controlling the properties of a material on an ultrafast time scale. In particular, resonantly exciting phonons leads to a better understanding of…

Strongly Correlated Electrons · Physics 2016-10-05 P. Bowlan , J. Bowlan , S. A. Trugman , R. Valdes Aguilar , J. Qi , X. Liu , J. Furdyna , M. Dobrowolska , A. J. Taylor , D. A. Yarotski , R. P. Prasankumar

In fluids, vortices form at boundaries between flows of different velocities. Here, we show that pulsed electromagnetic waves form spatiotemporal vortices when light straddles media of different phase velocities. When the resulting relative…

Optics · Physics 2025-11-17 Jordan M. Adams , Daniel Heligman , Rajind Mendis , Josh Wetherington