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Direct imaging of molecular dynamics is a long-standing goal in physics and chemistry. As an emerging tool, high-harmonic spectroscopy (HHS) enables accessing molecular dynamics on femtosecond to attosecond time scales. However, decoding…

We perform a detailed analysis of how high-order harmonic generation (HHG) and above-threshold ionization (ATI) can be controlled by a time-delayed attosecond-pulse train superposed to a strong, near-infrared laser field. In particular we…

Atomic Physics · Physics 2009-11-11 C. Figueira de Morisson Faria , P. Salieres , P. Villain , M. Lewenstein

High-harmonic generation (HHG), which is generation of multiple optical harmonic light, is an unconventional nonlinear optical phenomenon beyond perturbation regime. HHG, which was initially observed in gaseous media, has recently been…

We investigate the high harmonic generation (HHG) from solids by simulating the dynamics of a single active electron in periodic potentials. The corresponding time-dependent Schr\"odinger equations (TDSE) are solved numerically by using…

Atomic Physics · Physics 2016-03-31 Zhong Guan , Xiao-Xin Zhou , Xue-Bin Bian

We explore the impact of spatiotemporal couplings (STCs) on high-order harmonic generation (HHG) driven by spatiotemporal vortex beams. Our investigation demonstrates how STCs shape key properties of the generated harmonic beams, including…

Atomic Physics · Physics 2025-03-31 C. Granados , Bikash K. Das , M. Ciappina , W . Gao

Spin-orbital coupling and interaction as intrinsic light fields characteristics have been extensively studied. Previous studies involve the spin angular momentum (SAM) carried by circular polarization and orbital angular momentum (OAM)…

Optics · Physics 2021-03-18 Jian Chen , Lihua Yu , Chenhao Wan , Qiwen Zhan

High-order harmonic generation (HHG) in aligned linear molecules can offer valuable information about strong-field interactions in lower-lying molecular orbitals, but extracting this information is difficult for three-dimensional molecular…

High-order harmonic generation (HHG) from aligned acetylene molecules interacting with mid infra-red (IR), linearly polarized laser pulses is studied theoretically using a mixed quantum-classical approach in which the electrons are…

Atomic Physics · Physics 2018-05-18 Peter Mulholland , Daniel Dundas

This paper presents the method for the first time to generate intense high-order optical vortices that carry orbital angular momentum in the extreme ultraviolet region. In three-dimensional particle-in-cell simulation, both the reflected…

We theoretically investigate correlated electron dynamics in high-harmonic generation (HHG), using all-electron \emph{ab initio} simulations for three-dimensional real alkali-metal atoms. The resulting harmonic spectra exhibit a plateau…

Atomic Physics · Physics 2019-04-10 Yang Li , Takeshi Sato , Kenichi L. Ishikawa

The influence of large permanent dipoles on molecular orbital tomography via high-order harmonic generation (HHG) is investigated in this work. It is found that, owing to the modification of the angle-dependent ionization rate resulting…

Atomic Physics · Physics 2013-02-27 Xiaosong Zhu , Meiyan Qin , Qingbin Zhang , Yang Li , Zhizhan Xu , Peixiang Lu

Spatiotemporal optical vortex (STOV) carrying transverse orbital angular momentum (OAM) enriches the family of vortex beams and exhibit unique properties. Typically, a high-order STOV with an intensity null degrades into multiple…

Optics · Physics 2025-02-18 Shunlin Huang , Xiong Shen , Renjing Chen , Jun Liu , Ruxin Li

Accelerating and colliding particles has been a key strategy to explore the texture of matter. Strong lightwaves can control and recollide electronic wavepackets, generating high-harmonic (HH) radiation which encodes the structure and…

Mesoscale and Nanoscale Physics · Physics 2016-04-14 M. Hohenleutner , F. Langer , O. Schubert , M. Knorr , U. Huttner , S. W. Koch , M. Kira , R. Huber

We theoretically study high-harmonic generation (HHG) from solids driven by intense laser pulses using a one-dimensional model periodic crystal. By numerically solving the time-dependent Schr\"{o}dinger equation directly on a real-space…

High-order harmonic generation (HHG) enables the up-conversion of intense infrared or visible femtosecond laser pulses into extreme-ultraviolet attosecond pulses. However, the highly nonlinear nature of the process results in low conversion…

An intuitive physical mechanism for single attosecond pulse generation in multi-cycle pulse regime is proposed. We suggest that the continuum spectra of HHG can be controlled through the modulation of carrier wave, while keeping the…

Optics · Physics 2011-11-01 Xiang Yang , Yueping Niu , Shangqing Gong

High harmonic generation (HHG) opens a window on the fundamental science of strong-field light-mater interaction and serves as a key building block for attosecond optics and metrology. Resonantly enhanced HHG from hot spots in…

The high-order harmonic generation (HHG), if phase matched, opens a unique way to produce coherent ultrafast extreme-UV (XUV) or soft x-ray light sources. Here we describe a robust and tunable method for scaling and narrowing the bandwidth…

Optics · Physics 2017-10-03 L. Mashhadi , G. Shayeganrad

Today, it is well known that light possesses a linear momentum which is along the propagation direction. Besides, scientists also discovered that light can possess an angular momentum (AM), a spin angular momentum (SAM) associated with…

Optics · Physics 2020-07-15 Andy Chong , Chenhao Wan , Jian Chen , Qiwen Zhan

Light intensity control of the orbital angular momentum of the fundamental beam in a quadratic nonlinear process is theoretically and numerically presented. In particular we analyzed a seeded second harmonic generation process in presence…

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