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Electron-electron thermalization and electron-phonon relaxation processes in laser-excited solids are often assumed to occur on different timescales. This is true for the majority of the conduction band electrons in a metal. However,…

Mesoscale and Nanoscale Physics · Physics 2019-06-05 Sebastian T. Weber , Baerbel Rethfeld

Electron-phonon coupling, being one of the most important parameters governing the material evolution after ultrafast energy deposition, yet remains the most unexplored one. In this work, we applied the dynamical coupling approach to…

Materials Science · Physics 2020-08-05 N. Medvedev , I. Milov

The rate of energy transfer between electrons and phonons is investigated by a first principles framework for electron temperatures up to $T_e=50000$ K while considering the lattice at ground state. Two typical but differently complex…

Other Condensed Matter · Physics 2022-03-08 Jia Zhang , Rui Qin , Wenjun Zhu , Jan Vorberger

This paper describes the effects of electronic nonequilibrium in a simulation of ultrafast laser irradiation of materials. The simulation scheme based on tight-binding molecular dynamics, in which the electronic populations are traced with…

Materials Science · Physics 2023-12-29 Nikita Medvedev

Understanding of the energy exchange between electrons and phonons in metals is important for micro- and nano-manufacturing and system design. The electron-phonon (e-ph) coupling constant is to describe such exchange strength, yet its…

Mesoscale and Nanoscale Physics · Physics 2021-03-17 Wuli Miao , Moran Wang

The electronic behavior of various solid metals (Al, Ni, Cu, Au, Ti, and W) under ultrashort laser irradiation is investigated by means of density functional theory. Successive stages of extreme nonequilibrium on picosecond time scale…

Materials Science · Physics 2014-04-04 Emile Bévillon , Jean-Philippe Colombier , Vanina Recoules , Razvan Stoian

A nonperturbative dynamical coupling approach based on tight-binding molecular dynamics is used to evaluate the electron-ion (electron-phonon) coupling parameter in irradiated semiconductors as a function of the electronic temperature up to…

Materials Science · Physics 2023-10-25 Nikita Medvedev

The out-of-equilibrium dynamics of electrons and phonons upon laser excitation are often described by the two-temperature model, which assumes that both subsystems are separately in thermal equilibrium. However, recent experiments show that…

Materials Science · Physics 2021-01-04 Ulrike Ritzmann , Peter M. Oppeneer , Pablo Maldonado

The electronic and electrical properties of crystalline organic semiconductors, such as the dispersions of the electronic bands and the dependence of charge-carrier mobility on temperature, are greatly impacted by the nonlocal…

Materials Science · Physics 2012-06-06 Yuan Li , Yuanping Yi , Veaceslav Coropceanu , Jean-Luc Brédas

Solid He is studied in the pressure and temperature ranges 1-40 TPa and 0-10,000 K using first-principles methods. Anharmonic vibrational properties are calculated within a self-consistent field framework, including the internal and free…

Materials Science · Physics 2014-02-11 Bartomeu Monserrat , N. D. Drummond , Chris J. Pickard , R. J. Needs

The strength of the electron-phonon coupling parameter and its evolution throughout a solid's phase diagram often determines phenomena such as superconductivity, charge- and spin-density waves. Its experimental determination relies on the…

The periods of the harmonic oscillations of the ion core of charged sodium clusters around the equilibrium shapes are considered. It is found that these periods are of the order of magnitude of the experimentally measured relaxation times…

Atomic and Molecular Clusters · Physics 2009-11-10 F. F. Karpeshin , J. da Providencia , C. Providencia , J. da Providencia

Strong electron-electron interactions are known to significantly modify the electron-phonon coupling relative to the predictions of density functional theory, but this effect is challenging to calculate with realistic theories of strongly…

Strongly Correlated Electrons · Physics 2025-07-21 David J. Abramovitch , Jennifer Coulter , Sophie Beck , Andrew Millis

We analyze Cooper pairing instabilities in strongly driven electron-phonon systems. The light-induced non-equilibrium state of phonons results in a simultaneous increase of the superconducting coupling constant and the electron scattering.…

Superconductivity · Physics 2016-12-16 Michael Knap , Mehrtash Babadi , Gil Refael , Ivar Martin , Eugene Demler

In the present work, a theoretical study of electron-phonon (electron-ion) coupling rates in semiconductors driven out of equilibrium is performed. Transient change of optical coefficients reflects the band gap shrinkage in covalently…

Materials Science · Physics 2017-02-22 Nikita Medvedev , Zheng Li , Victor Tkachenko , Beata Ziaja

Metals exhibit nonequilibrium electron and lattice subsystems at transient times following femtosecond laser excitation. In the past four decades, various optical spectroscopy and time-resolved diffraction methods have been used to study…

Chemical Physics · Physics 2024-05-17 Xing He , Mithun Ghosh , Ding-Shyue Yang

We have studied the effect of nonequilibrium longitudinal optical phonons on hot-electron spin relaxation in $n$-type GaAs quantum wells. The longitudinal optical phonons, due to the finite relaxation rate, are driven to nonequilibrium…

Materials Science · Physics 2010-12-13 P. Zhang , M. W. Wu

We recently developed an approach for calculation of the electron-phonon (electron-ion in a more general case) coupling in materials based on tight-binding molecular dynamics simulations. In the present work we utilize this approach to…

Materials Science · Physics 2023-02-17 Nikita Medvedev , Igor Milov

Understanding nonequilibrium electron-phonon interactions at the microscopic level and on ultrafast timescales is a central goal of modern condensed matter physics. Combining time- and angle-resolved extreme ultraviolet photoemission…

We study the role of the superconducting proximity effect on the electron-phonon energy exchange in diffusive normal metals (N) attached to superconductors (S). The proximity effect modifies the spectral response of the normal metal, in…

Mesoscale and Nanoscale Physics · Physics 2009-03-16 T. T. Heikkila , F. Giazotto
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