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We present terahertz spectroscopic measurements of quantum spin dynamics in the honeycomb magnet K$_2$Co$_2$TeO$_6$ as a function of temperature, polarization and in an external magnetic field applied in the honeycomb plane. Magnetic…

Strongly Correlated Electrons · Physics 2025-08-01 Patrick Pilch , Laur Peedu , Urmas Nagel , Toomas Rõõm , Changqing Zhu , Yurii Skourski , Xianghan Xu , Robert J. Cava , Zhe Wang

Spin-orbit coupled honeycomb magnets with the Kitaev interaction have received a lot of attention due to their potential of hosting exotic quantum states including quantum spin liquids. Thus far, the most studied Kitaev systems are…

The honeycomb magnet Na$_3$Co$_2$SbO$_6$ recently emerged as a promising candidate for realizing Kitaev quantum spin liquid with relatively low levels of structural disorder. While the precise spin Hamiltonian remains controversial, the…

Strongly Correlated Electrons · Physics 2025-07-16 Rongsheng Li , Liyu Shi , Yuchen Gu , Yue Chen , Xintong Li , Qiong Wu , Shuxiang Xu , Dong Wu , Yuan Li , Fa Wang , Tao Dong , Nanlin Wang

One of the most important issues in modern condensed matter physics is the realization of fractionalized excitations, such as the Majorana excitations in the Kitaev quantum spin liquid. To this aim, the 3d-based Kitaev material Na2Co2TeO6…

Quantum fluctuations endow spin systems with surprisingly enriched magnetic phase diagrams. In frustrated magnets, strong quantum fluctuations boosted by either geometrical incompatibility or competitive exchange interactions stabilize…

We report on the results of 23Na NMR in the honeycomb lattice magnet Na2Co2TeO6 which has been nominated as a Kitaev material. Measurements of magnetic shift and width of the NMR line as functions of temperature and magnetic field show that…

Strongly Correlated Electrons · Physics 2022-12-21 Jun Kikuchi , Takayuki Kamoda , Nobuyoshi Mera , Yodai Takahashi , Kouji Okumura , Yukio Yasui

Spin systems with honeycomb structures have recently attracted a great deal of attention in connection with the Kitaev quantum spin liquid state (QSL) predicted theoretically. One possible Kitaev QSL candidate is Na$_2$Co$_2$TeO$_6$…

Strongly Correlated Electrons · Physics 2023-12-11 A. K. Bera , S. M. Yusuf , F. Orlandi , P. Manuel , L. Bhaskaran , S. A. Zvyagin

Kitaev interactions, arising from the interplay of frustration and bond anisotropy, can lead to strong quantum fluctuations and, in an ideal case, to a quantum-spin-liquid state. However, in many nonideal materials, spurious non-Kitaev…

Magnetic excitations in cycloidal magnet LiCu$_2$O$_2$ are explored using THz absorption spectroscopy in magnetic fields up to 12 T. Below the spin ordering temperature we observe eight optically active transitions in the spin system of…

Strongly Correlated Electrons · Physics 2015-05-13 D. Hüvonen , U. Nagel , T. Rõõm , Y. J. Choi , C. L. Zhang , S. Park , S. -W. Cheong

We present a comprehensive study of single crystals of Na2Co2TeO6, a putative Kitaev honeycomb magnet, focusing on its low-temperature phase behaviors. A new thermal phase transition is identified at 31.0 K, below which the system develops…

Strongly Correlated Electrons · Physics 2021-05-26 Wenjie Chen , Xintong Li , Zhenhai Hu , Ze Hu , Li Yue , Ronny Sutarto , Feizhou He , Kazuki Iida , Kazuya Kamazawa , Weiqiang Yu , Xi Lin , Yuan Li

The honeycomb cobaltate Na$_2$Co$_2$TeO$_6$ has recently been proposed as a candidate material for hosting field-induced quantum spin liquid (QSL) behavior. Here, we present a comprehensive thermodynamic study of its low-temperature,…

In the quest to find quantum spin liquids, layered cobalt oxides Na2Co2TeO6 and Na3Co2SbO6 have been proposed as promising candidates for approximating the Kitaev honeycomb model. Yet, their suitability has been thrown into question due to…

Strongly Correlated Electrons · Physics 2024-04-25 Ping Miao , Xianghong Jin , Weiliang Yao , Yue Chen , Akihiro Koda , Zhenhong Tan , Wu Xie , Wenhai Ji , Takashi Kamiyama , Yuan Li

Na$_2$Co$_2$TeO$_6$ has recently been proposed to be a Kitaev-like honeycomb magnet. To assess how close it is to realizing Kitaev quantum spin liquids, we have measured magnetization and specific heat on high-quality single crystals in…

Strongly Correlated Electrons · Physics 2020-02-19 Weiliang Yao , Yuan Li

We report on terahertz spectroscopy of quantum spin dynamics in $\alpha$-RuCl$_3$, a system proximate to the Kitaev honeycomb model, as a function of temperature and magnetic field. An extended magnetic continuum develops below the…

Strongly Correlated Electrons · Physics 2017-11-30 Zhe Wang , S. Reschke , D. Hüvonen , S. -H. Do , K. -Y. Choi , M. Gensch , U. Nage , T. Rõõm , A. Loidl

Na2Co2TeO6 is a proposed approximate Kitaev magnet, yet its actual magnetic interactions are elusive due to a lack of knowledge on the full excitation spectrum. Here, using inelastic neutron scattering and single crystals, we determine the…

Strongly Correlated Electrons · Physics 2022-10-04 Weiliang Yao , Kazuki Iida , Kazuya Kamazawa , Yuan Li

Despite exhibiting magnetic long-range order below $T_\mathrm{N} = 26.7\,\mathrm{K}$, the honeycomb cobaltate Na$_2$Co$_2$TeO$_6$ is predicted to enter a Kitaev spin liquid state when subjected to small external perturbations. While most of…

Strongly Correlated Electrons · Physics 2026-03-04 J. Arneth , R. Kalaivanan , R. Sankar , K. -Y. Choi , R. Klingeler

We have investigated the magnetic properties and mapped out the phase diagram of the honeycomb magnet Na2Co2TeO6 with Co 3d7 in out-of-plane magnetic fields. This material has previously been proposed to show nearest-neighbor Kitaev…

Strongly Correlated Electrons · Physics 2024-06-03 Shengzhi Zhang , Sangyun Lee , Eric Brosha , Qing Huang , Haidong Zhou , Vivien S. Zapf , Minseong Lee

Magnetoelectric effects in honeycomb antiferromagnet Co4Nb2O9 are investigated on the basis of symmetry analyses of Co ions in trigonal P-3c1 space group. For each Co ion, the possible spin dependence is classified by C3 point-group…

Strongly Correlated Electrons · Physics 2020-07-16 Masashige Matsumoto , Mikito Koga

Measurements are reported of the magnetic field dependence of excitations in the quantum critical state of the spin S=1/2 linear chain Heisenberg antiferromagnet copper pyrazine dinitrate (CuPzN). The complete spectrum was measured at k_B…

Strongly Correlated Electrons · Physics 2009-11-10 M. B. Stone , D. H. Reich , C. Broholm , K. Lefmann , C. Rischel , C. P. Landee , M. M. Turnbull

Two-dimensional high-spin bipartite honeycomb networks, where anisotropy, competing exchange interactions, and spin fluctuations interplay, provide an alternative platform to test theoretical models that distinguish between classical and…

Strongly Correlated Electrons · Physics 2026-05-05 M. Barik , Q. Faure , F. Damay , J. P. Embs , S. Petit , P. Khuntia
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