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Because of their strong excitonic photoluminescence (PL) and electroluminescence (EL), together with an excellent electronic tunability, transition metal dichalcogenide (TMD) semiconductors are promising candidates for novel optoelectronic…

Mesoscale and Nanoscale Physics · Physics 2019-03-08 Lukas Dobusch , Simone Schuler , Vasili Perebeinos , Thomas Mueller

We present a general picture of the exciton properties of layered materials in terms of the excitations of their single-layer building blocks. To this end, we derive a model excitonic hamiltonian by drawing an analogy with molecular…

Optical dynamics in van der Waals heterobilayers is of fundamental scientific and practical interest. Based on a time-dependent adiabatic GW approach, we discover a new many-electron (excitonic) channel for converting photoexcited…

Materials Science · Physics 2023-05-30 Chen Hu , Mit H. Naik , Yang-Hao Chan , Steven G. Louie

Statistics of photons emitted by mobile excitons in individual carbon nanotubes are investigated. Photoluminescence spectroscopy is used to identify the chiralities and suspended lengths of air-suspended nanotubes, and photon correlation…

Mesoscale and Nanoscale Physics · Physics 2017-11-28 A. Ishii , T. Uda , Y. K. Kato

By stacking various two-dimensional (2D) atomic crystals [1] on top of each other, it is possible to create multilayer heterostructures and devices with designed electronic properties [2-5]. However, various adsorbates become trapped…

Mesoscale and Nanoscale Physics · Physics 2012-09-06 S. J. Haigh , A. Gholinia , R. Jalil , S. Romani , L. Britnell , D. C. Elias , K. S. Novoselov , L. A. Ponomarenko , A. K. Geim , R. Gorbachev

In the last decade atomically thin 2D materials have emerged as a perfect platform for studying and tuning light-matter interaction and electronic properties in nanostructures. The optoelectronic properties in layered materials such as…

Mesoscale and Nanoscale Physics · Physics 2024-10-07 Roberto Rosati , Ioannis Paradisanos , Ermin Malic , Bernhard Urbaszek

Strongly bound excitons confined in two-dimensional (2D) semiconductors are dipoles with a perfect in-plane orientation. In a vertical stack of semiconducting 2D crystals, such in-plane excitonic dipoles are expected to efficiently couple…

The interaction between off-resonant laser pulses and excitons in monolayer transition metal dichalcogenides is attracting increasing interest as a route for the valley-selective coherent control of the exciton properties. Here, we extend…

Electric field-controlled, two-dimensional (2D) exciton dynamics in transition metal dichalcogenide monolayers is a current research focus in condensed matter physics. We have experimentally investigated the spectral and temporal properties…

Mesoscale and Nanoscale Physics · Physics 2019-12-11 Michael Engel , Mathias Steiner

The resonance energy and the transition rate of atoms, molecules and solids were understood as their intrinsic properties in classical electromagnetism. With the development of quantum electrodynamics, it is realized that these quantities…

Mesoscale and Nanoscale Physics · Physics 2020-05-07 Jason Horng , Yu-Hsun Chou , Tsu-chi Chang , Chu-Yuan Hsu , Tien-chang Lu , Hui Deng

Controlling matter-light interactions with cavities is of fundamental importance in modern science and technology. It is exemplified in the strong-coupling regime, where matter-light hybrid modes form, with properties controllable via the…

Mesoscale and Nanoscale Physics · Physics 2021-11-03 Long Zhang , Fengcheng Wu , Shaocong Hou , Zhe Zhang , Yu-Hsun Chou , Kenji Watanabe , Takashi Taniguchi , Stephen R. Forrest , Hui Deng

The photoluminescence dynamics of a microscopic gas of indirect excitons trapped in coupled quantum wells is probed at very low bath temperature (approximately 350 mK). Our experiments reveal the non linear energy relaxation characteristics…

Strongly Correlated Electrons · Physics 2015-05-20 Mathieu Alloing , Aristide Lemaitre , Francois Dubin

Excitons in two-dimensional semiconductors are directly exposed to the environment and are sensitive to the dielectric properties of their surrounding. Here, we show that the Rydberg series of excited states of excitons in a monolayer…

Twisted van der Waals heterostructures and the corresponding superlattices, moire superlattices, are remarkable new material platforms, in which electron interactions and excited-state properties can be engineered. Particularly, the band…

Mesoscale and Nanoscale Physics · Physics 2019-11-13 Xiaobo Lu , Xiaoqin Li , Li Yang

Despite the weak, van-der-Waals interlayer coupling, photoinduced charge transfer vertically across atomically thin interfaces can occur within surprisingly fast, sub-50fs timescales. Early theoretical understanding of the charge transfer…

Two-dimensional (2D) van der Waals (vdW) heterostructures consist of different 2D crystals with diverse properties, constituting the cornerstone of the new generation of 2D electronic devices. Yet interfaces in heterostructures inevitably…

Materials Science · Physics 2024-09-04 Yuxiang Gao , Fenglin Deng , Ri He , Zhicheng Zhong

Van der Waals heterostructures obtained by artificially stacking two-dimensional crystals represent the frontier of material engineering, demonstrating properties superior to those of the starting materials. Fine control of the interlayer…

Atoms start behaving as waves rather than classical particles if confined in spaces commensurate with their de Broglie wavelength. At room temperature this length is only about one angstrom even for the lightest atom, hydrogen. This…

Mesoscale and Nanoscale Physics · Physics 2018-03-20 S. Hu , K. Gopinadhan , A. Rakowski , M. Neek-Amal , T. Heine , I. V. Grigorieva , S. J. Haigh , F. M. Peeters , A. K. Geim , M. Lozada-Hidalgo

Controlling excitons and their transport in two-dimensional (2D) transition metal dichalcogenides (TMDs) heterostructures is central to advancing photonics and electronics on-chip integration. We investigate the controlled generation and…

Moir\'e superlattices open an unprecedented opportunity for tailoring interactions between quantum particles and their coupling to electromagnetic fields. Strong superlattice potential generates moir\'e minibands of excitons -- bound pairs…

Materials Science · Physics 2020-02-25 Yanhao Tang , Jie Gu , Song Liu , Kenji Watanabe , Takashi Taniguchi , James Hone , Kin Fai Mak , Jie Shan
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