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We theoretically propose a multidimensional high-harmonic echo spectroscopy technique which utilizes strong optical fields to resolve coherent electron dynamics spanning an energy range of multiple electron Volts. Using our recently…

The interplay of nuclear and electronic dynamics characterizes the multi-dimensional electronic spectra of various molecular and solid-state systems. Theoretically, the observable effect of such interplay can be accounted for by response…

Quantum Physics · Physics 2023-02-07 Filippo Troiani

Recent progress in the field of molecular electronics has revealed the fundamental importance of the coupling between the electronic degrees of freedom and specific vibrational modes. Considering the examples of a molecular dimer and a…

Mesoscale and Nanoscale Physics · Physics 2017-02-22 Jakub K. Sowa , Jan A. Mol , G. Andrew D. Briggs , Erik M. Gauger

We study resonant optical excitations of strongly-interacting Rydberg states of atoms in the presence of relaxations. We employ the quantum stochastic (Monte Carlo) wavefunctions to simulate the dissipative dynamics of tens of atoms in…

Quantum Physics · Physics 2013-06-25 David Petrosyan

The Wigner-crystal phase of two-dimensional electrons interacting via the Coulomb repulsion and subject to a strong Rashba spin-orbit coupling is investigated. For low enough electronic densities the spin-orbit band splitting can be larger…

Mesoscale and Nanoscale Physics · Physics 2014-08-12 P. G. Silvestrov , O. Entin-Wohlman

We discuss the electronic transport through molecules in the Kondo regime. We concentrate here on the influence of molecular vibrations. Two types of vibrations are investigated: (i) the breathing internal molecular modes, where the…

Mesoscale and Nanoscale Physics · Physics 2009-12-21 J. Mravlje , A. Ramsak

Orbital-lattice coupled excitation dynamics in orbitally degenerate correlated systems are examined. We present a theoretical framework, where both local vibronic excitations and superexchange-type inter-site interactions are dealt with on…

Strongly Correlated Electrons · Physics 2015-06-16 Joji Nasu , Sumio Ishihara

We consider the model of quantum dots interacting with coherent radiation when the relaxation processes may be neglected. The system under investigation consists of two discrete energy levels of the quantum dots in the presence of strong…

Pattern Formation and Solitons · Physics 2007-05-23 Andrey Maimistov , Elena Kazantseva , Sergei Elyutin

Multi-electron giant dipole resonances of atoms in crossed electric and magnetic fields are investigated. Stationary configurations corresponding to a highly symmetric arrangement of the electrons on a decentered circle are derived, and a…

Atomic Physics · Physics 2011-02-24 Sascha Zoellner , Hans-Dieter Meyer , Peter Schmelcher

In this preprint I propose that the non local discrete-state-in-continuum model previously successfully used to describe the inelastic electron molecule collisions can also be used to model the electron photo-detachment from the molecular…

Chemical Physics · Physics 2023-09-13 Martin Čížek

With advanced fabrication techniques it is possible to make nanoscale electronic structures that have discrete energy levels. Such structures are called artificial atoms because of analogy with true atoms. Examples of such atoms are quantum…

Mesoscale and Nanoscale Physics · Physics 2012-06-07 David Gunnarsson , Jani Tuorila , Antti Paila , Jayanta Sarkar , Erkki Thuneberg , Yuriy Makhlin , Pertti Hakonen

The correlated motion of electrons in a one dimensional system with an externally applied longitudinal electric field is discussed. Within the tight binding model we show that in addition to the well known Bloch oscillations the…

Condensed Matter · Physics 2009-11-10 F. Claro , J. F. Weisz , S. Curilef

The spectral properties of up to four interacting electrons confined within a quasi one--dimensional system of finite length are determined by numerical diagonalization including the spin degree of freedom. The ground state energy is…

Condensed Matter · Physics 2009-10-22 Wolfgang Haeusler , Bernhard Kramer , PTB Braunschweig

A variational model for the infra-red spectrum of VO is presented which aims to accurately predict the hyperfine structure within the VO $\mathrm{X}\,^4\Sigma^-$ electronic ground state. To give the correct electron spin splitting of the…

Chemical Physics · Physics 2022-10-25 Qianwei Qu , Sergei N. Yurchenko , Jonathan Tennyson

We examine the one-dimensional spinless Falicov-Kimball model extended by a hybridization potential between the localized and itinerant electron states. Below half-filling we find a crossover from a mixed-valence metal to an integer-valence…

Strongly Correlated Electrons · Physics 2009-01-26 P. M. R. Brydon , M. Gulacsi , A. R. Bishop

We study a class of exactly solvable models for strongly correlated electrons, defined on a set of N cells, and with infinite on-site repulsion on part of the sites of each cell. For 2N or more electrons the exact ground state is known. We…

Condensed Matter · Physics 2009-10-28 Andreas Giesekus , Uwe Brandt

In strongly correlated systems the strength of Coulomb interactions between electrons, relative to their kinetic energy, plays a central role in determining their emergent quantum mechanical phases. We perform resonant x-ray scattering on…

Singlet fission, the molecular process through which photons are effectively converted into pairs of lower energy triplet excitons, holds promise as a means of boosting photovoltaic device efficiencies. In the preceding article of this…

Materials Science · Physics 2017-05-12 Roel Tempelaar , David R. Reichman

Multi-electron giant dipole resonances of atoms in crossed electric and magnetic fields are investigated. Stationary configurations corresponding to a highly symmetric arrangement of the electrons on a decentered circle are derived, and a…

Atomic Physics · Physics 2011-02-24 S. Zöllner , H. -D. Meyer , P. Schmelcher

Resonant vibrational and rotation-vibration excitation cross sections for electron-CO scattering are calculated in the 0-10 eV energy range for all 81 vibrational states of CO, assuming that the excitation occur via the 2{\Pi} shape…

Chemical Physics · Physics 2012-08-14 V. Laporta , C. M. Cassidy , J. Tennyson , R. Celiberto