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Related papers: Structural criterion for the onset of rigidity in …

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Determining the onset of rigidity in gels is a fundamental challenge with significant practical implications across different applications. Limited-valence, or patchy-particle systems have proven to be a valuable model to study the…

Soft Condensed Matter · Physics 2025-04-04 J. C. Neves , J. M. Tavares , N. A. M. Araújo , C. S. Dias

Dispersed colloidal particles within a suspension can aggregate and spontaneously self-organize into a robust, percolating structure known as a gel. These network-like structures are prevalent in nature and play a critical role in many…

Soft Condensed Matter · Physics 2025-04-29 David Richard , Mehdi Bouzid

Rigidity percolation (RP) occurs when mechanical stability emerges in disordered networks as constraints or components are added. Here we discuss RP with structural correlations, an effect ignored in classical theories albeit relevant to…

Soft Condensed Matter · Physics 2019-08-07 Shang Zhang , Leyou Zhang , Mehdi Bouzid , D. Zeb Rocklin , Emanuela Del Gado , Xiaoming Mao

The effects of particle roughness and short-ranged non-central forces on colloidal gels are studied using computer simulations in which particles experience a sinusoidal variation in energy as they rotate. The number of minima $n$ and…

Soft Condensed Matter · Physics 2019-09-05 Hong T. Nguyen , Alan L. Graham , Peter H. Koenig , Lev D. Gelb

Colloidal gels constitute an important class of materials found in many contexts and with a wide range of applications. Yet as matter far from equilibrium, gels exhibit a variety of time-dependent behaviours, which can be perplexing, such…

Soft Condensed Matter · Physics 2021-09-22 C. Patrick Royall , Malcolm A. Faers , Sian L. Fussell , James E. Hallett

The formation of colloidal gels is strongly dependent on the volume fraction of the system and the strength of the interactions between the colloids. Here we explore very dilute solutions by the means of numerical simulations, and show…

Soft Condensed Matter · Physics 2017-09-13 Samuel Griffiths , Francesco Turci , C. Patrick Royall

We sandwich a colloidal gel between two parallel plates and induce a radial flow by lifting the upper plate at a constant velocity. Two distinct scenarios result from such a tensile test: ($i$) stable flows during which the gel undergoes a…

Soft Condensed Matter · Physics 2020-08-10 Thibaut Divoux , Asheesh Shukla , Badis Marsit , Yacouba Kaloga , Irmgard Bischofberger

In composite materials composed of soft polymer matrix and stiff, high-aspect-ratio particles, the composite undergoes a transition in mechanical strength when the inclusion phase surpasses a critical density. This phenomenon (rheological…

Soft Condensed Matter · Physics 2021-03-24 Samuel Heroy , Dane Taylor , Feng Shi , M. Gregory Forest , Peter J. Mucha

We study the self-assembly of colloidal microgel particles at a quasi-two-dimensional air-water interface of a drying droplet. Using bright-field microscopy, we demonstrate that increasing particle elasticity drives interfacial organization…

Soft Condensed Matter · Physics 2026-03-10 Vaibhav Raj Singh Parmar , Sayantan Chanda , Rituparno Mandal , Ranjini Bandyopadhyay

We discuss a class of models for particulate gels in which the particle contacts are described by an effective interaction combining a two-body attraction and a three-body angular repulsion. Using molecular dynamics, we show how varying the…

Soft Condensed Matter · Physics 2021-08-05 Minaspi Bantawa , Wayan A. Fontaine-Seiler , Peter D. Olmsted , Emanuela Del Gado

We present a detailed numerical study of multi-component colloidal gels interacting sterically and obtained by arrested phase separation. Under deformation, we found that the interplay between the different intertwined networks is key.…

Soft Condensed Matter · Physics 2020-06-11 Claudia Ferreiro-Cordova , Mehdi Bouzid , Emanuela Del Gado , Giuseppe Foffi

Colloidal gels are out of equilibrium soft solids composed of attractive Brownian particles that form a space-spanning network at low volume fractions. The elastic properties of these systems result from the network microstructure, which is…

Colloidal gels are widely applied in industry due to their rheological character -- no flow takes place below the yield stress. Such property enables gels to maintain uniform distribution in practical formulations; otherwise, solid…

Soft Condensed Matter · Physics 2023-05-17 Yujie Jiang , Ryohei Seto

Attractive colloidal particles can form a disordered elastic solid or gel when quenched into a two-phase region, if the volume fraction is sufficiently large. When the interactions are comparable to thermal energies the stress-bearing…

Soft Condensed Matter · Physics 2014-03-13 Lisa J. Teece , James M. Hart , Kerry Yen Ni Hsu , Stephen Gilligan , Malcolm A. Faers , Paul Bartlett

Colloidal gels consist of percolating networks of interconnected arms. Their mechanical properties depend on the individual arms, and on their collective behaviour. We use numerical simulations to pull on a single arm, built from a model…

Soft Condensed Matter · Physics 2023-01-31 Kristian Thijssen , T. B. Liverpool , C. Patrick Royall , Robert L. Jack

Attractive colloids diffuse and aggregate to form gels, solid-like particle networks suspended in a fluid. Gravity is known to strongly impact the stability of gels once they are formed. However, its effect on the process of gel formation…

Soft Condensed Matter · Physics 2023-04-12 Joost de Graaf , Kim William Torre , Wilson C. K. Poon , Michiel Hermes

Colloidal gels are a prototypical example of a heterogeneous network solid whose complex properties are governed by thermally-activated dynamics. In this Letter we experimentally establish the connection between the intermittent dynamics of…

Soft Condensed Matter · Physics 2017-05-10 Jan Maarten van Doorn , Jochem Bronkhorst , Ruben Higler , Ties van de Laar , Joris Sprakel

Using computer simulations, we identify the mechanisms causing aggregation and structural arrest of colloidal suspensions interacting with a short-ranged attraction at moderate and high densities. Two different non-ergodicity transitions…

Condensed Matter · Physics 2009-11-07 Antonio M. Puertas , Matthias Fuchs , Michael E. Cates

Many biological tissues feature a heterogeneous network of fibers whose tensile and bending rigidity contribute substantially to these tissues' elastic properties. Rigidity percolation has emerged as a important paradigm for relating these…

Attractive colloidal gels exhibit solid-like behavior at vanishingly small fractions of solids, owing to ramified space-spanning networks that form due to particle-particle interactions. These networks give the gel its rigidity, and as the…

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