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Cavity-enhanced frequency comb spectroscopy for molecule detection in the mid-infrared powerfully combines high resolution, high sensitivity, and broad spectral coverage. However, this technique, and essentially all spectroscopic methods,…

Dual-comb spectroscopy allows for the rapid, multiplexed acquisition of high-resolution spectra without the need for moving parts or low-resolution dispersive optics. This method of broadband spectroscopy is most often accomplished via…

A high-resolution broad-spectral-bandwidth spectrometer on a chip would create new opportunities for gas-phase molecular fingerprinting, especially in environmental sensing. A resolution high enough to observe transitions at atmospheric…

Multiheterodyne techniques using frequency combs -- light sources whose lines are perfectly evenly-spaced -- have revolutionized optical science. By beating an unknown signal with the many lines of a comb, its spectrum is recovered.…

Optics · Physics 2020-04-23 David Burghoff

We describe a possible new technique for precise wavelength calibration of high-resolution astronomical spectrographs using femtosecond-pulsed mode-locked lasers controlled by stable oscillators such as atomic clocks. Such `frequency combs'…

Molecular diagnostics are a primary tool of modern chemistry, enabling researchers to map chemical reaction pathways and rates to better design and control chemical systems. Many chemical reactions are complex and fast, and existing…

Two frequency combs can be used to measure the full complex response of a sample in a configuration which can be alternatively viewed as the equivalent of a dispersive Fourier transform spectrometer, infrared time domain spectrometer, or a…

Optics · Physics 2015-05-18 I. Coddington , W. C. Swann , N. R. Newbury

Joint spectral measurements are a powerful tool for characterising biphoton spectral correlation, which is crucial for quantum information and communication technologies. In these applications, highly pure biphoton states are essential in…

Spectroscopy in the molecular fingerprint spectral region (6.5-20 $\mu$m) yields critical information on material structure for physical, chemical and biological sciences. Despite decades of interest and effort, this portion of the…

It was recently demonstrated that broadband quantum cascade lasers can operate as frequency combs. As such, they operate under direct electrical pumping at both mid-infrared and THz frequencies, making them very attractive for dual-comb…

Two kinds of spectral control over $\gamma$-ray echo using a nuclear frequency comb system are theoretically investigated. A nuclear frequency comb system is composed of multiple nuclear targets under magnetization (hyperfine splitting),…

Quantum Physics · Physics 2019-07-08 Chia-Jung Yeh , Po-Han Lin , Xiwen Zhang , Olga Kocharovskaya , Wen-Te Liao

An optical frequency comb generated with an electro-optic phase modulator and a chirped radiofrequency waveform is used to perform saturation and pump-probe spectroscopy on the $D_1$ and $D_2$ transitions of atomic potassium. With a comb…

Atomic Physics · Physics 2016-12-21 David A. Long , Adam J. Fleisher , David F. Plusquellic , Joseph T. Hodges

Optical frequency combs paved the way for fast and compact multi-component optical chemical analysis due to their broadband spectra. Dual-comb spectrometers embody this technology, but their design requires a pair of matched combs, adding…

Optics · Physics 2025-09-25 Ina Heckelmann , Davide Pinto , Uwe Schmitt , Mattias Beck , Jérôme Faist

Dual-comb interferometry utilizes two optical frequency combs to map the optical field's spectrum to a radio-frequency signal without using moving parts, allowing improved speed and accuracy. However, the method is compounded by the…

Measuring the spectral properties of an optical frequency comb is among the most fundamental tasks of precision metrology. In contrast to general single-parameter measurement schemes, we demonstrate here single shot multiparameter…

Quantum Physics · Physics 2020-03-16 Y. Cai , J. Roslund , V. Thiel , C. Fabre , N. Treps

The introduction of nonlinear nanophotonic devices to the field of optical frequency comb metrology has enabled new opportunities for low-power and chip-integrated clocks, high-precision frequency synthesis, and broad bandwidth…

We demonstrated the observation of Rb two-photon absorption directly excided by an optical frequency comb at fiber communication bands. A chain of comb spectral control is elaborately implemented to increase the power of the second harmonic…

Optics · Physics 2015-06-16 Jiutao Wu , Dong Hou , Xiaoliang Dai , Zhengyu Qin , Zhigang Zhang , Jianye Zhao

We have carried out dual-comb spectroscopy and observed in a simultaneous acquisition a 140-THz-wide spectrum from 1.0 to 1.9 {\mu}m using two fiber-based frequency combs phase-locked to each other. This ultra-broad wavelength bandwidth is…

Frequency comb spectroscopy provides broadband access to molecular fingerprints with mode-defined spectral resolution. However, its deployment in non-cooperative gas sensing remains challenging because conventional implementations require…

Tunable mid-infrared lasers are essential for optical sensing and imaging. Existing technologies, however, face challenges in simultaneously achieving broadband spectral tunability and ultra-rapid scan rates, limiting their utility in…

Optics · Physics 2025-01-20 Xiaoshuai Ma , Tianjian Lv , Xudong Zhu , Ming Yan , Heping Zeng
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