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Strong coupling between electronic excitations in materials and photon modes results in the formation of polaritons, which display larger nonlinearities than their photonic counterparts due to their material component. We theoretically…

Chemical Physics · Physics 2023-08-29 Sindhana Pannir-Sivajothi , Nathaniel P. Stern , Joel Yuen-Zhou

We create exciton-polaritons in a zero-dimensional (0D) microcavity filled with organic ladder-type conjugated polymer in the strong light-matter interaction regime. Photonic confinement at wavelength scale is realized in the longitudinal…

Mesoscale and Nanoscale Physics · Physics 2019-01-23 Fabio Scafirimuto , Darius Urbonas , Ullrich Scherf , Rainer F. Mahrt , Thilo Stöferle

We study the resonant electronic excitation dynamics for ultracold atoms trapped in a deep optical lattice prepared in a Mott insulator state. Excitons in these artificial crystals are similar to Frenkel excitons in Noble atom or molecular…

Quantum Physics · Physics 2009-08-11 Hashem Zoubi , Helmut Ritsch

We study the elastic response of a stationarily driven system of a cavity field strongly coupled with molecular excitons, taking into account the main dissipation channels due to the finite cavity linewidth and molecular vibrations. We show…

Quantum Physics · Physics 2021-02-24 Kalle S. U. Kansanen , J. Jussi Toppari , Tero T. Heikkilä

We propose a practical scheme to observe the polaritonic quantum phase transition (QPT) from the superfluid (SF) to Bose-glass (BG) to Mott-insulator (MI) states. The system consists of a two-dimensional array of photonic crystal…

Quantum Physics · Physics 2013-05-29 Y. C. Neil Na , Shoko Utsunomiya , Lin Tian , Yoshihisa Yamamoto

Nonperturbative coupling of light with condensed matter in an optical cavity is expected to reveal a host of coherent many-body phenomena and states. In addition, strong coherent light-matter interaction in a solid-state environment is of…

Two-dimensional semiconductors inside optical microcavities have emerged as a versatile platform to explore new hybrid light-matter quantum states. The strong light-matter coupling leads to the formation of exciton-polaritons, which in turn…

Mesoscale and Nanoscale Physics · Physics 2021-11-05 Miguel Angel Bastarrachea-Magnani , Jannie Thomsen , Arturo Camacho-Guardian , Georg M. Bruun

We introduce a prototypical model for cavity polaritonic control of ultracold photochemistry by considering the resonant vibrational strong coupling of a rubidium dimer to a terahertz cavity. We demonstrate that at avoided crossings between…

Quantum Gases · Physics 2023-11-21 Vasil Rokaj , Simeon I. Mistakidis , H. R. Sadeghpour

Recent experiments have observed that the chemical and photophysical properties of molecules can be modified inside an optical Fabry-Perot microcavity under collective vibrational strong coupling (VSC) conditions, and such modification is…

Mesoscale and Nanoscale Physics · Physics 2021-03-09 Tao E. Li , Abraham Nitzan , Joseph E. Subotnik

Strong light-matter coupling is a quantum process in which light and matter are coupled together, generating hybridized states. This is similar to the notion of molecular hybridization, but one of the components is light. Here, we utilized…

Applied Physics · Physics 2024-02-20 Jhuma Dutta , Pooja Bhatt , Kuljeet Kaur , Daniel E. Gómez , Jino George

Understanding the quantum dynamics of strongly coupled molecule-cavity systems remains a significant challenge in molecular polaritonics. This work develops a comprehensive self-consistent model simulating electromagnetic interactions of…

Chemical Physics · Physics 2025-01-29 Maxim Sukharev , Joseph E. Subotnik , Abraham Nitzan

We theoretically study circular dichroism of chiral molecules embedded inside a helicity-preserving Fabry-P\'erot cavity. We find an increase of the intrinsic chiroptical response of the molecules by 2 orders of magnitude and report the…

Optics · Physics 2023-02-22 L. Mauro , J. Fregoni , J. Feist , R. Avriller

Microcavity polaritons are strongly interacting hybrid light-matter quasiparticles, which are promising for the development of novel light sources and active photonic devices. Here, we report polariton lasing in the UV spectral range in…

We consider a one-dimensional topological superconductor hosting Majorana bound states at its ends coupled to a single mode cavity. In the strong light-matter coupling regime, electronic and photonic degrees of freedom hybridize resulting…

Mesoscale and Nanoscale Physics · Physics 2023-10-11 Olesia Dmytruk , Marco Schirò

Following experimental evidence that vibrational polaritons, formed from collective vibrational strong coupling (VSC) in optical microcavities, can modify ground-state reaction rates, a spate of theoretical explanations relying on…

Chemical Physics · Physics 2023-04-14 Matthew Du , Yong Rui Poh , Joel Yuen-Zhou

Using carefully designed hybrid metal-dielectric resonators, we study molecular optomechanics in the strong coupling regime ($g_{\rm }^2/\omega_m {>} \kappa$), which manifests in anharmonic emission lines in the sideband-resolved region of…

Mesoscale and Nanoscale Physics · Physics 2019-11-28 Mohsen Kamandar Dezfouli , Reuven Gordon , Stephen Hughes

When the interaction between a molecular system and confined light modes in an optical or plasmonic cavity is strong enough to overcome the dissipative process, hybrid light-matter states (polaritons) become the fundamental excitations in…

Mesoscale and Nanoscale Physics · Physics 2020-01-08 Yu Zhang , Tammie Nelson , Sergei Tretiak

Exciton-polaritons in semiconductors are quasi-particles which have recently shown the capability to undergo phase transition into a coherent hybrid state of light and matter. The observation of such quasi-particles in organic microcavities…

Control is exerted over the exciton-polariton physics in metal - Poly(9,9-dioctyl fluorene) - metal microcavities via conformational changes to the polymer backbone. Using thin-film samples containing increasing fractions of $\beta$-phase…

Soft Condensed Matter · Physics 2018-11-21 F. Le Roux , D. D. C. Bradley

Resonant coupling of a vibration to a cavity mode has been reported to dramatically modify spontaneous Raman scattering, but subsequent studies have produced conflicting results. In this Letter, we develop a microscopic quantum framework…

Mesoscale and Nanoscale Physics · Physics 2025-11-04 Maxime Dherbécourt , Joël Bellessa , Clémentine Symonds , Guillaume Weick , David Hagenmüller